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Hybrid white light emitting devices (HWLEDs) from organic polymer and PbS nanocrystals by multiple excitons

Kadim Akeel M.

Materials Science Poland

2020

Vol. 38, No. 4

693--698

Hybrid white light-emitting devices (HWLEDs) were fabricated using FTO/PEDOT: PSS/PbS/Alq3/Ni system and synthesized by phase separation process. In the present study, the multiple excitons generation in lead sulfide (PbS) NCs, which is characteristic of PbS NCs, was used to induce an effective and regulated energy transfer to an HWLED. The HWLED consisted of three layers successively deposited on FTO glass substrate; the first layer consisted of poly (3,4-ethylenedioxythiophene) polystyrene sulfonate (PEDOT: PSS) blended with polymethyl methacrylate (PMMA) organic polymer in the 1:1 ratio, while the second layer consisted of PbS NCs. Finally, above the layer of the PbS NCs, Tris (8-hydroxyquinoline) aluminum (Alq3) layer was deposited. The white light was generated with quite a good efficiency due to the confinement effect that makes the energy gap greater. The characteristics of the current-voltage (I-V) indicate acceptable conditions for the generation of white light by multiple excitons. It was found that the emission levels able to produce white luminescence, classified based on the coordinate system of chromaticity (CIE 1931), are x = 0.31, y = 0.33 while the correlated color temperature (CCT) is about 6250 K. The HWLEDs made from PbS NCs with hole injection from the organic polymer (PEDOT: PSS with PMMA), and electron injection from organic molecules (Alq3) are capable of white light generation.

Interface interactions and optical properties of novel photonic nanocomposites consisting of porous glasses doped with organic luminophore molecules

Antropova T.V., Baran J., Gavrilko T., Gnatyuk I., Morawska-Kowal T., Melnik V., Puchkovska G., Vorobjev V.

Optica Applicata

2005

Vol. 35, nr 4

725-733

Absorption and luminescence spectra of nanocomposites consisting of photonic molecules rhodamine 6G, trishydroxyquinoline aluminum (Alq3) complex and benzophenone adsorbed on soda-borosilicate porous glasses from ethanol and dichloromethane (DCM) solutions are investigated. The effect of sorption interactions at the interface between the glass pore surface and the organic media on luminescent and optical characteristics of the nanocomposites was investigated by NIR spectroscopy. It was shown that spectral changes observed in the absorption and emission spectra of the luminophores in the porous glasses are determined by the balance between physical interaction of the organic molecule with different adsorption centers on the pore walls and solvation effect.

Photoluminescence, optical transmission and reflection of Alq₃ layers obtained by thermal evaporation deposition

Dalasiński P., Łukasiak Z., Rębarz M., Wojdyła M., Bratkowski A., Bała W.

Opto-Electronics Review

2004

Vol. 12, No. 4

429-434

In this paper we present the photoluminescence emission spectra (PL), photoluminescence excitation spectra (PLE), transmission (TS) and reflection (RS) spectra of tris(8-hydroxyquinoline) aluminum(III) (Alq₃) layers grown by thermal evaporation deposition method. All investigated samples exhibit strong luminescence in the wide temperature range from 13 K to room temperature and for different energies of excitation. In our experiments, we have focused on temperature dependence of photoluminescence. The thermal quenching of PL in the measured samples has been found. We have observed also distinct oscillations from reflection and transmission measurements. The energies of thermal activation estimated by means of configuration coordinate diagram and also the layer thickness and refractive index are presented.