Characterization of the effects of acetic acid on the recovery of valuable contents from flotation tailings of non-sulfide metals

• Autorzy: Yoğurtcuoğlu Emine

Identyfikatory

DOI

10.37190/ppmp/185168

• Języki publikacji: EN

Abstrakty

EN

Non-sulfide lead flotation tailings draw attention in terms of their valuable contents. Dissolution studies have been carried out with strong inorganic acids, especially in ore form, but these acids have been unfavorable in removal in the context of metal recovery processes. Organic acids, on the other hand, are notable for their environmentally friendly properties and selective metal recovery opportunities. In this study, the effects of acetic acid on metal recovery from oxidized waste were investigated with different experimental parameters at a laboratory scale. Optimal conditions were determined depending on the increase in acetic acid concentration. At 0.75-1.0 M acid concentrations, 49-55% Pb and 49-54% Zn recovery efficiencies were obtained with grades of 7.0-7.2% and 19.5-19.7%, respectively. The recovery of Pb/Zn by the leaching process with acetic acid and the selective nonrecovery of iron were also observed through characterization studies. With the Rietveld XRD method, an increase in iron minerals such as goethite and a decrease in smithsonite-hydrozincite minerals were determined. These changes were seen as a decrease in the contents of these minerals in SEM/EDX analysis and as a decrease in smithsonite mineral bond structures in the FT-IR analysis. This study showed that acetic acid has many advantages in the utilization of zinc-lead-containing oxide flotation tailings, which have high economic value, such as selective metal recovery, easy biodegradability, environmental friendliness, and non-corrosiveness.

Słowa kluczowe

EN

flotation tailing; acetic acid; recovery; zinc; lead; characterization

• Wydawca: Oficyna Wydawnicza Politechniki Wrocławskiej
• Czasopismo: Physicochemical Problems of Mineral Processing
• Rocznik: 2024
• Tom: Vol. 60, iss. 1
• Strony: art. no. 185168
• Opis fizyczny: Bibliogr. 67 poz., rys., tab., wykr.

Twórcy

autor

Yoğurtcuoğlu Emine

• Faculty of Engineering, Department of Mining Engineering, Niğde Ömer Halisdemir University, 51240, Niğde, Turkey

Bibliografia

• AHMED, S.H., GAMMAL, E.M. EL, AMIN, M.I., YOUSSEF, W.M., 2021. Studying the effect of potassium amyl xanthate surfactant on fe, cu and u ions for the pretreatment of abu zeneima sulphate leach liquor. Periodica Polytechnica Chemical Engineering 65, 408–415.
• AKYILDIRIM, O., YUKSEK, H., MANAP, S., 2019. Synthesis and Characterization of New 3-Alkyl(Aryl)-4-[3-ethoxy-4-(2- furylcarbonyloxy)-benzylidenamino]-4,5-dihydro-1H-1,2,4-triazol-5-ones. International Turkic World Congress on Science and Engineering. Niğde, Turkiye, 230–236.
• ALKAN, M.S., RÜŞEN, A., TOPÇU, M.A., 2023. Recovery of Lead and Zinc from Complex Industrial Waste of Zinc Process with Ammonium Acetate. JOM 75, 1158–1168.
• APARAJITH, B., MOHANTY, D.B., GUPTA, M.L., 2010. Recovery of enriched lead-silver residue from silver-rich concentrate of hydrometallurgical zinc smelter. Hydrometallurgy 105, 127–133.
• ASLAN, Y., GUROCAK, Z., 2022. Investigation of the textural changes after the stabilization of bentonite with lime and tuff by Fourier Transform Infrared (FT-IR) Spectroscopy method (in Turkish). DUJE (Dicle University Journal of Engineering) 13, 599–610.
• AYDOǦAN, S., ARAS, A., UÇAR, G., ERDEMOǦLU, M., 2007. Dissolution kinetics of galena in acetic acid solutions with hydrogen peroxide. Hydrometallurgy 89, 189–195.
• BARRETT, E.C., NENNIGER, E.H., DZIEWINSKI, J., 1992. A hydrometallurgical process to treat carbon steel electric arc furnace dust. Hydrometallurgy 30, 59–68.
• DIKMEN, G., ALVER, Ö., 2021. Vibrational studies of monomer, dimer and trimer structures of 4-carboxy phenylboronic acid. Eskişehir Technical University Journal of Sciences and Technology A- Applied Science and Engineering 22, 134–147.
• DREISINGER, D.B., PETERS, E., MORGAN, G., 1990. The hydrometallurgical treatment of carbon steel electric arc furnace dusts by the UBC-Chaparral process. Hydrometallurgy 25, 137–152.
• EL OUARDI, M., LAABD, M., ABOU OUALID, H., BRAHMI, Y., ABAAMRANE, A., ELOUAHLI, A., AIT ADDI, A., LAKNIFLI, A., 2019. Efficient removal of p-nitrophenol from water using montmorillonite clay: insights into the adsorption mechanism, process optimization, and regeneration. Environmental Science and Pollution Research 26, 19615–19631.
• FREDD, C.N., FOGLER, H.S., 1998. The kinetics of calcite dissolution in acetic acid solutions. Chemical Engineering Science 53, 3863–3874.
• GUO, X., ZHANG, B., WANG, Q., LI, Z., TIAN, Q., 2021. Recovery of Zinc and Lead from Copper Smelting Slags by Chlorination Roasting. JOM 73, 1861–1870.
• HALLI, P., HAMUYUNI, J., REVITZER, H., LUNDSTRÖM, M., 2017. Selection of leaching media for metal dissolution from electric arc furnace dust. Journal of Cleaner Production 164, 265–276.
• HAMUYUNI, J., HALLI, P., TESFAYE, F., LEIKOLA, M., LUNDSTRÖM, M., 2018. A sustainable methodology for recycling electric arc furnace dust. Miner. Metals Mater. Ser. 133–240.
• HANILÇI, N., ÖZTÜRK, H., 2005. Mississippi Valley Type Zn-Pb Deposits In The Aladağlar-Zamanti (Eastern Taurus) Regio: Ayrakli and Denizovası Zn-Pb Deposits, Turkey (in Turkish). İTU Journal 18, 23–43.
• HAVLIK, T., FRIEDRICH, B., 2004. Pressure Leaching of EAF Dust. World of Metallurgy - ERZMETALL 2. HENRIQUE, P., FERREIRA, T., MALENA, R., LIMA, F., 2022. Concentration of oxidized Brazilian zinc ore by flotation: comparative study between anionic and cationic routes. Separation Science and Technology 57, 2625–2634.
• HOSSEINI, S.H., FORSSBERG, E., 2007. Physicochemical studies of smithsonite flotation using mixed anionic/cationic collector. Minerals Engineering 20, 621–624.
• HOSSEINI, S.H., FORSSBERG, E., 2006. Adsorption studies of smithsonite flotation using dodecylamine and oleic acid. Minerals and Metallurgical Processing 23, 87–96.
• HOSSEINI, S.H., TAJI, M., 2015. Flotation behavior of iranian oxidized zinc ore using different types of collectors (cationic, anionic and mixed (cationic/anionic)). International Journal of Mining Engineering and Mineral Processing 4, 18–27.
• HU, M., XIE, N., GAO, S., HUANG, Y., YU, Y., 2023. A super-efficient polyquaternium gel that can remove over-10-times masses of lignins from wastewater for resourcefulness. Npj Clean Water 6, 1–14.
• HU, W., NIU, Y., ZHU, H., DONG, K., WANG, D., LIU, F., 2021. Remediation of zinc-contaminated soils by using the two-step washing with citric acid and water-soluble chitosan. Chemosphere 282, 131092.
• HURŞIT, M., LAÇIN, O., SARAÇ, H., 2009. Dissolution kinetics of smithsonite ore as an alternative zinc source with an organic leach reagent. Journal of the Taiwan Institute of Chemical Engineers 40, 6–12.
• HUSSAINI, S., TITA, A.M., KURSUNOGLU, S., TOP, S., ICHLAS, Z.T., KAR, U., KAYA, M., 2021. Pb-Zn recovery from a malic leach solution of a carbonate type ore flotation tailing by precipitation and solvent extraction. Separation and Purification Technology 272, 118963.
• HUSSAINI, S., TITA, A.M., KURSUNOGLU, S., TOP, S., KAYA, M., 2023. Recovery of Lead and Zinc from a Citric Leach Solution of a Non-sulfide Type Ore Flotation Tailing via Precipitation Followed by Solvent Extraction. JOM 75, 1569–1580.
• JHA, M.K., KUMAR, V., SINGH, R.J., 2001. Review of hydrometallurgical recovery of zinc from industrial wastes. Resources, Conservation and Recycling 33, 1–22.
• JIAO, B.C., ZHANG, X.D., WEI, C.C., SUN, J., HUANG, Q., ZHAO, Y., 2011. Effect of acetic acid on ZnO:In transparent conductive oxide prepared by ultrasonic spray pyrolysis. Thin Solid Films 520, 1323–1329.
• KAYA, M., HUSSAINI, S., KURSUNOGLU, S., 2020. Critical review on secondary zinc resources and their recycling technologies. Hydrometallurgy 195, 105362.
• KIEFER, J., STRÄK, A., KIEFER, A.L., GLADE, H., 2018. Infrared spectroscopic analysis of the inorganic deposits from water in domestic and technical heat exchangers [WWW Document], Energies.
• LAÇIN, O., DÖNMEZ, B., DEMIR, F., 2005. Dissolution kinetics of natural magnesite in acetic acid solutions. International Journal of Mineral Processing 75, 91–99.
• LUO, W., SI, Y., WANG, H., QIN, Y., HUANG, F., WANG, C., 2011. Leather material found on a 6th B.C. Chinese bronze sword: A technical study. Spectrochimica Acta - Part A: Molecular and Biomolecular Spectroscopy 79, 1630–1633.
• MAGELA, G., DUARTE, P., MALENA, R., LIMA, F., 2021. Mineral Processing and Extractive Metallurgy Review Quartz and Hematite Activation by Zn, Ca and Mg Ions in the Cationic Flotation Route for Oxidized Zinc Ore Quartz and Hematite Activation by Zn, Ca and Mg Ions in the Cationic Flotation Route for Oxidize. Mineral Processing and Extractive Metallurgy Review 43, 720–727.
• MALLIGARJUNA RAO, S., KOTTEESWARAN, S., VISAGAMANI, A.M., 2021. Green synthesis of zinc oxide nanoparticles from camellia sinensis: Organic dye degradation and antibacterial activity. Inorganic Chemistry Communications 134, 108956.
• MIKULA, K., SKRZYPCZAK, D., IZYDORCZYK, G., BAŚLADYŃSKA, S., SZUSTAKIEWICZ, K., GORAZDA, K., MOUSTAKAS, K., CHOJNACKA, K., WITEK-KROWIAK, A., 2022. From hazardous waste to fertilizer: Recovery of high-value metals from smelter slags. Chemosphere 297. https://doi.org/10.1016/j.chemosphere.2022.134226
• MORADI, S., MONHEMIUS, A.J., 2011. Mixed sulphide–oxide lead and zinc ores: Problems and solutions. Minerals Engineering 24, 1062–1076.
• NAGIB, S., INOUE, K., 2000. Recovery of lead and zinc from fly ash generated from municipal incineration plants by means of acid and/or alkaline leaching. Hydrometallurgy 56, 269–292.
• NANDA, S., KUMAR, S., MANDRE, N.R., 2022. Flotation behavior of a complex lead-zinc ore using individual collectors and its blends for lead sulfide [WWW Document], Journal of Dispersion Science and Technology. URL https://www.tandfonline.com/doi/abs/10.1080/01932691.2022.2036185 (accessed 7.3.22).
• NANDIYANTO, A.B.D., OKTIANI, R., RAGADHITA, R., 2019. How to read and interpret ftir spectroscope of organic material. Indonesian Journal of Science and Technology 4, 97–118.
• NAYAK, A., JENA, M.S., MANDRE, N.R., 2021. Beneficiation of Lead-Zinc Ores-A Review. Mineral Processing and Extractive Metallurgy Review 43, 564–583.
• NISKANEN, J., LAHTINEN, M., PERÄMÄKI, S., 2022. Acetic acid leaching of neodymium magnets and iron separation by simple oxidative precipitation [WWW Document], Cleaner Engineering and Technology. https://doi.org/10.1016/j.clet.2022.100544
• OJIMA, J., 2003. Determining of crystalline silica in respirable dust samples by Infrared Spectrophotometry in the presence of interferences. Journal of Occupational Health 45, 94–103.
• ÖNAL, G., BULUT, G., GÜL, A., KANGAL, O., PEREK, K.T., ARSLAN, F., 2005. Flotation of Aladaǧ oxide lead-zinc ores. Minerals Engineering 18, 279–282.
• ONOL, K., SARIDEDE, M.N., 2013. Investigation on microwave heating for direct leaching of chalcopyr- ite ores and concentrates. International Journal of Minerals, Metallurgy and Materials 20, 228–233.
• ONUKWULI, O.D., NNANWUBE, I.A., 2022. Optimization of zinc recovery from sphalerite using response surface methodology and particle swarm optimization. Periodica Polytechnica Chemical Engineering 66, 20–29.
• RASHCHI, F., DASHTI, A., ARABPOUR-YAZDI, M., ABDIZADEH, H., 2005. Anglesite flotation: A study for lead recovery from zinc leach residue. Minerals Engineering 18, 205–212. https://doi.org/10.1016/j.mineng.2004.10.014
• ŞAHIN, M., ERDEM, M., 2015. Cleaning of high lead-bearing zinc leaching residue by recovery of lead with alkaline leaching. Hydrometallurgy 153, 170–178.
• SBIHI, K., CHERIFI, O., BERTRAND, M., EL GHARMALI, A., 2014. Biosorption of metals (Cd, Cu and Zn) by the freshwater diatom Planothidium lanceolatum: A laboratory study. Diatom Research 29, 55–63.
• ŞENTÜRK, B., ÖZBAYOĞLU, G., ATALAY, Ü., 1993. Flotation of Lead-Zinc Carbonate Ore of Kayseri̇-Zamanti District (in Turkish). Türkiye XIII . Madencilik Kongresi. 459–466.
• SETHURAJAN, M., HUGUENOT, D., JAIN, R., LENS, P.N.L., HORN, H.A., FIGUEIREDO, L.H.A., VAN HULLEBUSCH, E.D., 2017. Leaching and selective zinc recovery from acidic leachates of zinc metallurgical leach residues. Journal of Hazardous Materials 324, 71–82.
• SINHA, M.K., PRAMANIK, S., SAHU, S.K., PRASAD, L.B., JHA, M.K., PANDEY, B.D., 2016. Development of an efficient process for the recovery of zinc and iron as value added products from the waste chloride solution. Separation and Purification Technology 167, 37–44.
• SMITH, A.M.L., DUBBIN, W.E., WRIGHT, K., HUDSON-EDWARDS, K.A., 2006. Dissolution of lead- and lead–arsenic-jarosites at pH 2 and 8 and 20 ℃: Insights from batch experiments. Chemical Geology 229, 344–361.
• STEER, J.M., GRIFFITHS, A.J., 2013. Investigation of carboxylic acids and non-aqueous solvents for the selective leaching of zinc from blast furnace dust slurry. Hydrometallurgy 140, 34–41.
• TANG, S., LI, R., HAN, X., MIAO, X., GUO, M., ZHANG, M., 2020. Selective and efficient extraction of lead from mixed sulfide-oxide lead and zinc ore by the in-situ self-reduction method. Hydrometallurgy 193, 105297.
• TOPÇU, M.A., KALEM, V., RÜŞEN, A., 2021A. Processing of anode slime with deep eutectic solvents as a green leachant. Hydrometallurgy 205. https://doi.org/10.1016/j.hydromet.2021.105732
• TOPÇU, M.A., RÜŞEN, A., KÜÇÜK, Ö., 2021B. Treatment of copper converter slag with deep eutectic solvent as green chemical. Waste Management 132, 64–73.
• TURAN, M.D., ALTUNDOǦAN, H.S., TÜMEN, F., 2004. Recovery of zinc and lead from zinc plant residue. Hydrometallurgy 75, 169–176.
• VIDRA, A., NÉMETH, Á., 2018. Bio-produced acetic acid: A review. Periodica Polytechnica Chemical Engineering 62, 245–256.
• XIAO, X., HOOGENDOORN, B.W., MA, Y., ASHOKA SAHADEVAN, S., GARDNER, J.M., FORSBERG, K., OLSSON, R.T., 2021. Ultrasound-assisted extraction of metals from Lithium-ion batteries using natural organic acids. Green Chemistry 23, 8519–8532.
• XUE, Y., HAO, X., LIU, X., ZHANG, N., 2022. Recovery of Zinc and Iron from Steel Mill Dust—An Overview of Available Technologies. Materials 15, 1–17.
• YARLUĞKAL ALTINIŞIK, A. C., CEBECİ, Y., SİS, H., C., KALENDER, L., 2022. A Process Mineralogy Approach to the Flotation of Complex Lead – Zinc Ores from Görgü ( Malatya ) Region. Mining, Metallurgy & Exploration 39, 1219–1232.
• YOĞURTCUOĞLU, E., 2023A. The citric acid leaching of boron process wastes. Canadian Metallurgical Quarterly 62, 773-790.
• YOĞURTCUOĞLU, E., 2023B. Multi-Metal Recovery from Flotation Tailings with Citric Acid on the NaCl Media. Journal of Scientific Reports-A 59–73.
• YOĞURTCUOĞLU, E., 2023C. Investigation of the effect of cyanidation after microwave roasting treatment on refractory gold / silver ores by characterization studies. Physicochem. Probl. Miner. Process. 59, 1–14.
• YOĞURTCUOĞLU, E., 2022A. Evaluation of flotation wastes of oxidised ores (in Turkish). IV . International Turkic World Congress on Science and Engineering (TURK-COSE). 1098–1104.
• YOĞURTCUOĞLU, E., 2022B. Usage of acetic acid for boric acid production from boron wastes. Niğde Ömer Halisdemir University Journal of Engineering Sciences 11, 819–825.
• ZHENG, Y. XING, LIU, W., QIN, W. QING, JIAO, F., HAN, J. WEI, YANG, K., LUO, H. LIN, 2015. Sulfidation roasting of lead and zinc carbonate with sulphur by temperature gradient method. Journal of Central South University 22, 1635–1642.
• ZHU, X., HE, X., YANG, J., GAO, L., LIU, J., YANG, D., SUN, X., ZHANG, W., WANG, Q., KUMAR, R.V., 2013. Leaching of spent lead acid battery paste components by sodium citrate and acetic acid. Journal of Hazardous Materials 250–251, 387–396.
• ZVIAGINA, B.B., DRITS, V.A., DORZHIEVA, O. V., 2020. Distinguishing features and identification criteria for Kdioctahedral 1M micas (Illite-aluminoceladonite and illite-glauconite-celadonite series) from middle-infrared spectroscopy data. Minerals 10. https://doi.org/10.3390/min10020153