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Spectroscopic properties of Er3+-doped fluorotellurite glasses modified by Nb2O5 and WO3

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Burtan-Gwizdała B. , Reben M. , Cisowski J. , El Sayed Y. , Lisiecki R. , Grelowska I.

Optica Applicata

2019

tom Vol. 49, nr 3

393--402

We have investigated the spectroscopic properties of Er3+-doped fluorotellurite glasses with the basic molar composition 75%TeO2–10%P2O5–10%ZnO–5%PbF2, modified by replacing 5% TeO2 by a metal oxide, namely WO3 or Nb2O5. The absorption edge of the glasses studied has been described within the Urbach approach, while the absorption and photoluminescence spectra have been analyzed in terms of the standard Judd–Ofelt theory, along with the photoluminescence decay of the 4I13/2 and 4S3/2 levels of the Er3+ ion. The absorption and emission spectra of the 4I15/2↔ 4I13/2infrared transition have been analyzed within the McCumber theory to yield the peak emission cross-section and figure of merit for the amplifier gain. It appears that the fluorotellurite glass containing WO3 as a modifier is characterized by the largest figure of merit, indicating this matrix as a promising new host for doping with Er3+ ions.

Nd3+ or Sm3+ doped oxyfluoride glass based on GeO2-PbO-PbF2. Synthesis and spectroscopic properties

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Klimesz B. , Dominiak-Dzik G. , Ryba-Romanowski W.

Optica Applicata

2005

tom Vol. 35, nr 4

843-850

Glasses with composition 50 GeO2-(45 - x)PbO-5 PbF2-x LnF3 (Ln = Nd or Sm, x = 0.2 and 2 mol%) were synthesised in the bulk form. Phase profiles and temperature characteristics were measured by differential thermal analysis (DTA); glass transition temperature Tg, as well as the b-PbF2 Tb and oxide glass crystallisation Tc temperatures have been derived for each individual system. A study of optical properties (absorption, emission) of the PbF2-Nd3+ and PbF2-Sm3+ was carried out. The oscillator strengths were obtained for several optical transitions and they have been used to calculate phenomenological intensity parameters W2, 4, 6. The probabilities of radiative transitions from fluorescent levels of Nd3+ and Sm3+ ions, as well as branching ratios and radiative lifetimes, were estimated on the basis of the Judd-Ofelt framework. The fluorescence dynamics of studied systems was measured. Experimental lifetimes were compared and discussed with those obtained with the Judd-Ofelt theory.