Połączenia lantanowców z niewspółmiernymi strukturami warstwowymi

Palewski, T.

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Artykuł - szczegóły

Czasopismo

Wiadomości Chemiczne

2003 | [Z] 57, 9-10 | 827--854

Tytuł artykułu

Połączenia lantanowców z niewspółmiernymi strukturami warstwowymi

Autorzy

Palewski, T.

Wybrane pełne teksty z tego czasopisma

Warianty tytułu

Rare earth compounds with incommensurate layered structures

Języki publikacji

Abstrakty

In a family of sulfide and selenide compounds are known composite crystals with incommensurate layered crystal structure and with a general formula (MX)_1+n(TX₂)_m where M = Pb, Sn, Sb, Bi and rare earth metals (Ln), T = Ti, V, Cr, Nb and Ta, and X = S and Se which in the English scientific literature are called „misfits". The crystal structure of misfits consist of two types of slabs with strong intra-slab bonding and a weaker interaction between them. One type of slabs (TX₂) is a three-atom-thick sandwich of a transition metal T layer between layers of chalcogenide atoms X, the second one (MX) consists of a two-atom-thick double layer of atoms each with the same number of M and X atoms. The paper presents a description of part of the whole class of misfits compounds, the rare earth misfits (LnX)_1+n (TX₂)_m. Some physical properties of them, mainly the electrical and magnetic properties, originate from the first or the second types of slabs and may be changed independently. The Introduction gives a short history of discovery of the misfits compounds and their location in the family of composite crystals. Then details of the crystal structure of lantanide misfits have been presented, types of slabs and their geometric forms, preffered crystal structures and the direction of incommensurability. Two next parts present the way of determination of their chemical formula and methods of their synthesis. The described physical properties concern the electrical resistivity, superconductivity, magnetism, and some spectral properties. On this basis possible band structures are presented. Particular attention is devoted to the similarities and differences of the physical properties between parent compounds LnX, TX₂ and the misfits (LnX)_1+n (TX₂)_m. Finally, some perspective studies of the rare earth misfits are considered

Słowa kluczowe

struktury modulowane kryształy złożone misfity niewspółmierne struktury warstwowe

composite crystals misfit layered compounds

Wydawca

Czasopismo

Wiadomości Chemiczne

Rocznik

2003

Tom

[Z] 57, 9-10

Strony

827--854

Opis fizyczny

Bibliogr. 70 poz., tab., wykr.

Twórcy

autor

Palewski, T.

Międzynarodowe Laboratorium Silnych Pól Magnetycznych i Niskich Temperatur, ul. Gajowicka 95, 53-421 Wrocław

Międzynarodowe Laboratorium Silnych Pól Magnetycznych i Niskich Temperatur, ul. Gajowicka 95, 53-421 Wrocław

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Bibliografia

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