Synthesis and characterization of metastable CeO2-ZrO2 solid solution obtained by polymerized complex method

• Autorzy: Miśta, W. , Rayment, T. , Hanuza, J. , Macalik, L.
• Języki publikacji: EN

Abstrakty

EN

The paper describes the preparation and characterization of nano-size metastable tetragonal CeO2–ZrO2 mixed oxides prepared by a polymerized complex method. A glycine–ethylene glycol solution containing Ce3+ and Zr4+ ions was polymerized at 80–110 °C to form a viscous transparent resin without any visible precipitation. After heat-treatment at relatively low temperature (ca 250 °C) on a hot plate in static air, the solid precursor ignited in part due to self-combustion, resulting in the formation of a nanocrystalline, compositionally-homogeneous solid solution. Its structure was confirmed using X-ray diffraction, HRTEM and Raman spectroscopy. The phase separation in CeO2–ZrO2 system on a subsequent heat-treatment in air and in a mixture of H2 and He was also investigated up to 1100 °C.

Słowa kluczowe

EN

ceria-zirconia; polymerized complex method; Raman spectroscopy; X-ray diffraction

• Czasopismo: Materials Science Poland
• Rocznik: 2004
• Tom: Vol. 22, No. 2
• Strony: 153--170
• Opis fizyczny: Bibliogr. 65 poz.

Twórcy

autor

Miśta, W.

• Institute of Low Temperature and Structure Research, Polish Academy of Sciences, P.O. Box 1410, 50-950 Wrocław 2, Poland,

autor

Rayment, T.

• Chemistry Department, Cambridge University, Cambridge CB2 1EW, UK

autor

Hanuza, J.

• Institute of Low Temperature and Structure Research, Polish Academy of Sciences, P.O. Box 1410, 50-950 Wrocław 2, Poland

autor

Macalik, L.

• Institute of Low Temperature and Structure Research, Polish Academy of Sciences, P.O. Box 1410, 50-950 Wrocław 2, Poland

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