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2017 | 26 | 4 |
Tytuł artykułu

Mass spectral analysis of the aged 1,3,5-trimethylbenzene secondary organic aerosol in the presence of ammonium sulfate seeds

Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
The ammonium sulfate ((NH₄)₂SO₄) seed aerosols commonly found in the Chinese urban atmosphere could affect the formation and aging of secondary organic aerosols (SOA). Aging of aromatic SOA is performed using UV-irradiation of 1,3,5-trimethylbenzene (135-TMB)/CH₃ONO/NO/air mixtures with high concentrations (~100 μg/m³) of (NH₄)₂SO₄ seeds in the laboratory chamber in this study. The particulate products of SOA were measured using an aerosol laser time-of-flight mass spectrometer (ALTOFMS) in real-time, and fuzzy c-means (FCM) was applied to the mass spectra organic species for clusters. Experimental results indicated that methylglyxoal, 2-methyl-4-oxo-2-pentenal, 4-methyl-1H-imidazole, 4-methyl-imidazole-2-acetaldehyde, and other imidazole derivative compounds are the principal products in the aged particles. Imidazole compounds that can absorb solar radiation effectively were newly detected in the aged 135-TMB SOA with high concentrations of (NH₄)₂SO₄ seed aerosols. These would provide new information for discussing the 135-TMB SOA aging mechanism.
Słowa kluczowe
Wydawca
-
Rocznik
Tom
26
Numer
4
Opis fizyczny
p.1531-1537,fig.,ref.
Twórcy
autor
  • Fujian Provincial Key Laboratory of Modern Analytical Science and Separation Technology, College of Chemistry and Environment, Minnan Normal University, Zhangzhou 363000, China
  • Department of Environmental Science and Engineering, Xiamen University, Tan Kah Kee College, 363105 Zhangzhou, China
autor
  • Fujian Provincial Key Laboratory of Modern Analytical Science and Separation Technology, College of Chemistry and Environment, Minnan Normal University, Zhangzhou 363000, China
autor
  • Fujian Provincial Key Laboratory of Modern Analytical Science and Separation Technology, College of Chemistry and Environment, Minnan Normal University, Zhangzhou 363000, China
autor
  • Department of Environmental Science and Engineering, Xiamen University, Tan Kah Kee College, 363105 Zhangzhou, China
autor
  • Laboratory of Atmospheric Physico-Chemistry, Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 230031, China
autor
  • Laboratory of Atmospheric Physico-Chemistry, Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 230031, China
autor
  • Laboratory of Atmospheric Physico-Chemistry, Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 230031, China
autor
  • Laboratory of Atmospheric Physico-Chemistry, Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 230031, China
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Typ dokumentu
Bibliografia
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Identyfikator YADDA
bwmeta1.element.agro-f8ecbba6-4fcc-4ba5-b80e-908eba5d2229
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