pH impact on the sol-gel preparation of calcium hydroxyapatite, Ca10(PO4)6(OH)2, using a novel complexing agent, DCTA

• Autorzy: Irma Bogdanoviciene , Kaia Tőnsuaadu , Valdek Mikli , Inga Grigoraviciute-Puroniene , Aldona Beganskiene , Aivaras Kareiva
• Języki publikacji: EN

Abstrakty

EN

Aqueous sol-gel chemistry routes - based on ammonium hydrogen phosphate as the phosphorus precursor, calcium acetate monohydrate as the source of calcium ions, and 1,2-diaminocyclohexanetetraacetic acid monohydrate (DCTA) as the complexing agent - have been used to prepare calcium hydroxyapatite (HA). The sol-gel process was performed in aqueous solution at different pH values followed by calcination of the dry precursor gels for 5 h at 1000°C. Phase transformations, composition, and structural changes in the polycrystalline samples were studied by thermoanalytical methods (TG/DTA), infrared spectroscopy (IR), X-ray powder diffraction analysis (XRD), and scanning electron microscopy (SEM). It was shown that pH adjustment has significant impact on the apatite formation process and on the morphology and phase purity of the ceramic samples.

Słowa kluczowe

EN

Calcium hydroxyapatite; Aqueous sol-gel process; DCTA; Structural features

• Czasopismo: Open Chemistry
• Rocznik: 2010
• Tom: 8
• Numer: 6
• Strony: 1323-1330

Daty

wydano

2010-12-01

online

2010-10-08

Twórcy

autor

Irma Bogdanoviciene

• Department of General and Inorganic Chemistry, Vilnius University, LT-03225, Vilnius, Lithuania

autor

Kaia Tőnsuaadu

• Laboratory of Inorganic Materials, Tallinn University of Technology, 19086, Tallinn, Estonia

autor

Valdek Mikli

autor

Inga Grigoraviciute-Puroniene

• Department of General and Inorganic Chemistry, Vilnius University, LT-03225, Vilnius, Lithuania

autor

Aldona Beganskiene

• Department of General and Inorganic Chemistry, Vilnius University, LT-03225, Vilnius, Lithuania

autor

Aivaras Kareiva

• Department of General and Inorganic Chemistry, Vilnius University, LT-03225, Vilnius, Lithuania,

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Identyfikatory

DOI

10.2478/s11532-010-0113-0