Water-soluble inorganic ions in urban aerosols of the continental part of Balkans (Belgrade) during the summer – autumn (2008)

• Autorzy: Aleksandra Mihajlidi-Zelić , Dragana Đorđević , Dubravka Relić , Ivana Tošić , Ljubiša Ignjatović , Maria A. Stortini , Andrea Gambaro
• Języki publikacji: EN

Abstrakty

EN

Size-segregated aerosol samples were collected using six stages High Volume Cascade Impactor. Aerosol mass and water soluble ions concentrations were determined. The Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model was used to study the origin of air masses arriving to Belgrade in the investigated period. The obtained results of aerosol mass and water-soluble ion concentrations have been divided into six sub-data sets based on air mass categories. The highest average mass concentration of the fine mode (Dp ≤ 0.49 μm) was found for air masses coming to Belgrade from the southeast and northwest directions, and of the coarse mode (3.0 < Dp ≤7.2 μm) for air masses arriving from the northwest direction. The highest concentrations of SO42– were found in the fine particles transported to the investigated area by air masses from southeast direction. The analysis of contribution of marine aerosol components (Na+ and Cl-), the Correlation and Cluster Analysis indicated the influence of marine aerosol on urban aerosol of the central Balkans coming from the Western Mediterranean and northern direction. NH4+ and SO42- and K+ dominated in the fine mode for all air mass categories. PCA demonstrated the dominant impact of secondary aerosol formation processes on urban aerosols.

EN

Słowa kluczowe

EN

Urban aerosol; Size-segregated inorganic ions; Balkan region

• Czasopismo: Open Chemistry
• Rocznik: 2015
• Tom: 13
• Numer: 1

Daty

otrzymano

2013-10-16

zaakceptowano

2014-04-23

online

2014-11-01

Twórcy

autor

Aleksandra Mihajlidi-Zelić

• Institute of Chemistry, Technology and Metallurgy – Centre of Chemistry, University of Belgrade ,11158 Belgrade, Serbia

autor

Dragana Đorđević

• Institute of Chemistry, Technology and Metallurgy – Centre of Chemistry, University of Belgrade ,11158 Belgrade, Serbia

autor

Dubravka Relić

• Faculty of Chemistry, University of Belgrade, 11158 Belgrade, Serbia

autor

Ivana Tošić

• Department of Meteorology, University of Belgrade, 11158 Belgrade, Serbia

autor

Ljubiša Ignjatović

• Faculty of Physical Chemistry, University of Belgrade, 11158 Belgrade, Serbia

autor

Maria A. Stortini

• Institute for the Dynamics of Environmental Processes (CNR-IDPA), 30123 Venice, Italy

autor

Andrea Gambaro

• Environmental Sciences, Informatics, Statistic Department, Ca‘ Foscari University of Venice, 30123 Venice, Italy

Bibliografia

• [1] Seinfeld J.H., Pandis S.N., Atmospheric Chemistry and Physics: From Air Pollution to Climate Change, John Wiley & Sons, Inc, New York, 1998
• [2] Glavas S., Moschonas N., Atmos. Environ., 2002, 36, 3089
• [3] Seinfeld J.H., Atmospheric Chemistry and Physics of Air Pollution, Wiley, New York, 1986
• [4] Putaud J.P., Van Dingenen R., Dell’ Acqua A., Raes F., Matta E., Decesari S. et al., Atmos. Chem. Phys., 2004, 4, 889
• [5] Đorđević D., Mihajlidi-Zelić A., Relić D., Ignjatović Lj., Huremović J., Stortini A.M., Gambaro A., Atmos. Environ., 2012, 46, 309
• [6] Querol X., Alastuey A., Viana M.M., Rodriguez S., Artińano B., Salvador P. et al., Aerosol. Sci., 2004, 35, 1151
• [7] Delalieux F., Van Grieken R., Potgieter J.H., Mar. Pollut. Bull., 2006, 52, 606[Crossref]
• [8] Kishcha P., Ničković S., Starobinetes B., di Sarra A., Udisti R., Becagli S. et al., Atmos. Res., 2011, 100, 28
• [9] Draxler R.R., Hess G.D., Description of the Hysplit_4 modeling system, NOAA Tech. Memo. ERL ARL-224, NOAA Air Resources Laboratory, Silver Spring, MD, 1997, 24
• [10] Draxler R.R., Hess G.D., Aust. Met. Mag., 1998, 47, 295
• [11] Draxler R.R., Rolph G.D., HYSPLIT (HYbrid Single-Particle Lagrangian Integrated Trajectory) Model access via NOAA ARL, NOAA Air Resources Laboratory, Silver Spring, MD, 2011, http://ready.arl.noaa.gov/HYSPLIT.php
• [12] Rolph G.D., Real-time Environmental Applications and Display sYstem (READY), NOAA Air Resources Laboratory, Silver Spring, MD, 2011, http://ready.arl.noaa.gov
• [13] Poissant L., Atmos. Environ., 1999, 33, 2537
• [14] Perkauskas D., Proceedings of Millennium (24th) NATO/CCMS International Technical Meeting on Air Pollution Modelling and its Application, 15-19 May 2000, Boulder, Colorado, USA, 212
• [15] Đorđević D., Tošić I., Unkašević M., Đurašković P., Environ. Sci. Poll. Res., 2010, 17, 1591[Crossref]
• [16] Stortini A.M., Freda A., Cesari D., Cairns W.R.L., Contini D., Barbante C. et al., Atmos. Environ., 2009, 43, 6296
• [17] Kalnay E., Kanamitsu M., Kistler R., Collins W. et al., Bull. Amer. Meteor. Soc., 1996, 77, 437[Crossref]
• [18] Cuccia E., Bernardoni V., Massabò D., Prati P., Valli G., Vecchi R., Atmos. Environ., 2010, 44, 3304
• [19] Espinosa A.J.F., Rodríguez M.T., de la Rosa F.J.B., Sánchez J.C.J., Atmos. Environ., 2001, 35, 2595
• [20] Pikridas M., Bougiatioti A., Hildebrandt L., Engelhart G.J., Kostenidou E., Mohr C. et al., Atmos. Chem. Phys., 2010, 10, 6793
• [21] Wittmaack K., Menzel N., Wehnes H., Heinzmann U., Atmos. Environ., 2002, 36, 5877
• [22] Tsitouridou R., Papazova P., Simeonova P., Simeonov V., J. Environ. Sci. Health A, 2013, 48(14), 1815[Crossref]
• [23] Chrysikou L.P., Samara C.A., Atmos. Environ., 2009, 43, 4557
• [24] Maksimović M., Jovanović M., Nikolić K., Copper, 2007, 32(1), 1
• [25] Đorđević D., Šolević T., Arsić P., Petrović S., Beograd University, Novi Beograd, 2004, (in Serbian) http://archive.rec.org/REC/Programs/REREP/LawDrafting/status/Serbia_and_Montenegro/Serbian/Srbija/Izvestaji/Konacni%20izvestaj_Pancevo.pdf
• [26] Marenco F., Bonasoni P., Calzolari F., Ceriani M., Chiari M., Cristofanelli P. et al., J. Geophys. Res., 2006, 111, D24202 (), DOI: 10.1029/2006JD007145[Crossref]
• [27] Beuck H., Quass U., Klemm O., Kuhlbusch T.A.J., Atmos. Environ., 2011, 45, 5813
• [28] Astel A., Mazerski J., Polkowska Z., Namiesnik J., Adv. Environ. Res., 2004, 8, 337[Crossref]
• [29] Huang S., Rahn K.A., Arimoto R., Atmos. Environ., 1999, 33, 2169

Identyfikatory

DOI

10.1515/chem-2015-0010