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Capabilities and limits of picosecond vibrational spectroscopy

Seifert G., Graener H.

Bulletin of the Polish Academy of Sciences. Chemistry

1999

Vol. 47, No. 4

397-417

The variety of information about ultrafast processes in condensed matter that can be obtained applying picosecond vibrational spectroscopy is discussed on the example of a quite elaborate experimental setup for infrared double resonance spectroscopy; a novel comprehensive single-shot polarization analysis is described. On the basis of experimental data obtained with this system on simple liquids (CHBr(3), CDBr(3), CS(2), CC(4)) and hydrogen-bonded dimers of acetic acid (dissolved in CC4) the way of distinguishing the desired from non-desired signals and the evaluation of the results is demonstrated.