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Activated Complex in the Decomposition of N2O over Cu

Polie S., Senegaenik M., Kobal I., Zieliński M.

Polish Journal of Chemistry

2001

Vol. 75, nr 11

1729-1729

Decomposition of N2O over Cu wire, at initial N2O pressures 40–60 kPa and temperatures 675–875 K, showed first order kinetics inN2Owith an apparent activation energy of 110 š 16 kJ mol–1. The 15N and 18O kinetic isotope effects under these experimental conditions were determined and interpreted following the Bigeleisen’s formalism. A bent NNO activated complex satisfactorily accounts for the experimental results.