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Polynuclear chain complexes of ruthenium(II,III) pivalate dimers linked by 2,5-dimethyl-N,N'-dicyanobenzoquinonediimine, 1,4-benzoquinone, and 1,4-naphthoquinone

Yoshioka D., Hanada M., Mikuriya M., Hiromitsu I.

Materials Science Poland

2005

Vol. 23, No. 3

765--771

Reactions of ruthenium(II,III) pivalate dimer with 2,5-dimethyl-N,N'- dicyanobenzoquinonediimine (2,5-dmdcnqi), 1,4-benzoquinone (1,4-bq), and 1,4- naphthoquinone (1,4-nq) gave polynuclear chain complexes, [Ru2(O2CCMe3)4(L)]nXn, L = 2,5-dmdcnqi, 1,4-bq, and 1,4-nq and X = BF4- and PF6-. It was shown that a weak antiferromagnetic interaction (J = -0.15 cm-1) operates between Ru(II,III) dimers for the 2,5- dmdcnqui complex.