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Photochemical oxidation model of organic pollutants in greywater from a small household

Bielski Andrzej

Environment Protection Engineering

2020

Vol. 46, nr 1

91--115

The treatment of coagulated greywater from a small household was investigated. The processes of oxidation of organic compounds with hydrogen peroxide combined with ultraviolet radiation (H2O2/m3/UV) was described. Greywater with various initial COD and TOC concentrations was used in the H2O2/m3/UV process. The process parameters were hydrogen peroxide doses 0.5–4.0 kg H2O2/m3, UV (254 nm) light intensity 75.5 W/m2 and irradiation time – 1 h. The oxidation efficiency varied broadly from 15 to 98% and higher COD values corresponded to lower oxidation efficiencies. The average hydrogen peroxide consumption per kg of COD w was = 12.2 g H2O2/m3/g O2 COD, while per TOC it was w′ = 69.0 g H2O2/m3/g C. The experiments enabled one to developed mathematical models for coagulation and oxidation kinetics. The models showed that at the initial COD = 859 g O2/m3, the coagulant dose of 100 g Al3+/m3, the hydrogen peroxide dose of 4 kg H2O2/m3 and the UV irradiation time of 3 h it is possible to decrease the COD by 98.4%.