Anew 1-D polymeric coordination compound [Mn(L)2(N(CN)2)2] (L = 4-cyanopyridine N-oxide) has been synthesized and characterized. The crystal structure of this compound was determined by X-ray diffraction analysis. In the crystal structure, the [Mn(L)2]2+ units are linked by [N(CN)2]- _-bridging ligands to form one dimensional structure. The manganese ions display four coordination, with two terminal N atoms of different [N(CN)2]- ligands and twoOatoms of different 4-cyanopyridine N-oxide ligands. Analysis of variable temperature magnetic susceptibility (2-300 K) indicates that the polymer shows weak antiferromagnetic interaction.
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