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EN
This study focusses on dose rate determination in complex settings in two drill cores from the site of Niederweningen, northern Switzerland. A crosscheck with a certified standard material and neutron activation analyses (NAA) reveals an overall good performance of high-resolution gamma spectrometry (HR-GS) when determining dose rate-relevant elements. A second focus is on average water content during burial, by comparing measured sediment moisture with water uptake capability. Furthermore, layer models are used to investigate the impact of inhomogeneous stratification on dose rate. Finally, different scenarios to correct for radioactive disequilibrium in the uranium decay chain are investigated. While most of the applied corrections appear to have only a minor to moderate effect on age calculation, the results for one core are contradictory. Possibly, some of the applied correction scenarios are not reflecting the complex natural setting sufficiently, in particular average sediment moisture during burial and the timing of radioactive disequilibrium might be incorrectly estimated. While deposition in one core can be quite securely attributed to the period 100–70 ka, assigning the sediment sequence in the other core to the time between ca. 130 ka and 90 ka remains to some extent insecure.
EN
This work considers the impact of the internal alpha and beta dose rates in quartz grains obtained from sandy sediments on the results of luminescence dating. The internal dose rates reported here (ca. 0.01–0.21 Gy · ka−1) play a particularly important role, because of low (ca. 0.8–0.9 Gy · ka−1) or very low (ca. 0.4–0.6 Gy · ka−1) external dose rates. In these cases, the internal dose rates form a significant fraction of the total dose rates, often exceeding 10%. Ignoring this contribution would have made the considered luminescence ages artificially older. In our study, we measure both the internal alpha and beta contributions as the latter is usually neglected in the case of quartz. The dose rate measurements were performed using the innovative μDose system.
3
Content available remote Luminescence dating procedures at the Gliwice Luminescence Dating Laboratory
EN
The Gliwice Luminescence Laboratory (GLL) is a part of the Institute of Physics – Centre for Science and Education at the Silesian University of Technology, which has gradually evolved since the 1980s. To date, nearly 3500 samples have been dated using luminescence from materials such as ceramics, bricks, and sediments from archaeological and geological sites. Currently, the laboratory is equipped with four luminescence readers and three gamma spectrometers, allowing luminescence dating of approximately 300 samples annually for the needs of research projects. This article focuses on the laboratory procedures used in GLL to obtain luminescence ages. Recent improvements of the GLL's facilities and new equipment, as well as the performance spanning the Laboratory's 30 years of activity, are discussed in terms of obtained results and the involvement in national and international projects.
EN
In terms of fine-grain luminescence dating applications, the efficiency of α-radiation in producing luminescence is an important issue when determining environmental dose rates. Efficiency is usually assessed by measuring the ratio of luminescence intensities induced by known α and β laboratory doses. Consequently, most thermoluminescence (TL)/optically stimulated luminescence (OSL) readers besides the standard 90Sr/90Y β-source can also be equipped with a 241Am α-source. A crucial point is, however, the calibration of these sources. The calibration of β-sources is routinely performed using standard quartz samples previously irradiated by a known γ-dose, though, in the case of α-sources, the procedure is less standardised, partly because there are no calibration materials with a known α-efficiency value. In this study, we aimed to cross-calibrate the built-in α-source of a RISØ TL/OSL DA-20 luminescence reader by testing and comparing five procedures, applying different samples (quartz and polymineral), different protocols multiple aliquot regeneration (MAR) and single aliquot regeneration (SAR) and different calibration sources. Throughout the tests, the performance of the fine-grain RISØ calibration quartz was also assessed. Regardless of the applied procedure, the calculated α-dose rates with one exception gave similar results. On the one hand, the applied polymineral sample due to potential fading, fairly high residuals after bleaching and relatively low infrared stimulated luminescence (IRSL) sensitivity proved to be the least optimal choice for cross-calibration. On the other hand, the tested natural fine grain quartz gave almost identical results when using different types of bleaching and different calibration α-sources. The mean dose rate determined for the source was 0.080 ± 0.004 Gy/s. The cross-calibration by using the RISØ fine grain quartz yielded somewhat higher but at the apparent uncertainty of luminescence dating still not significantly different dose rate for the source under calibration. Tests showed that the calibration quartz saturates at a relatively low α-dose, and the shape of α- and β-dose-response curves also depart from each other quite early, suggesting that cross-calibration with this material seems to be reliable only at low doses. For the first time, the a-value of the fine-grain calibration quartz was also determined using the freshly calibrated α-source, and the measurement yielded a 0.054 ± 0.003 value. We propose that after further validation of this result, the RISØ calibration quartz can ease the dose rate assessment of uncalibrated α-sources in the future.
EN
The stratigraphy of Late Pleniglacial and Late Glacial fluvio-to-aeolian succession was investigated in two sites located at the Niemodlin Plateau, SW Poland. Lithofacial analysis was used for the reconstruction of sedimentary environments. An absolute chronology for climatic change and the resulting environmental changes were determined based on optically stimulated luminescence (OSL – nine samples) and radiocarbon (three samples) dating methods. Four phases of changes in sedimentary environments were established. The first depositional phase correlates with the Last Permafrost Maximum (24−17 ka) based on the type and size of the periglacial structures, which aggraded under continuous permafrost conditions. During 17.5−15.5 ka (upper Late Pleniglacial), a stratigraphic gap was detected, owing to a break in the deposition on the interfluve area. The second depositional phase took place during 15.5−13.5 ka. During this phase, the first part of the dune formation (Przechód site) and fluvio-aeolian cover (Siedliska site) was deposited. The sedimentary processes continued throughout the entire Bølling interstadial and Older Dryas. In the third phase (Allerød interstadial), soil formation took place. At the Siedliska site, palaeosol represented Usselo soil type, whereas at the Przechód site, there was a colluvial type of soil. The last phase (Younger Dryas) is represented by the main phase of dune formation in both sites. After the Younger Dryas, no aeolian activity was detected. High compliance with both absolute dating methods was noticed.
EN
Luminescence dating is based mainly on the dosimetric properties of quartz and feldspar. These minerals are among the most popular found on Earth, resulting in the possibility of using luminescence methods in practically any environment. Currently, quartz remains the best recognized mineral in terms of dosimetric properties, particularly with regards to results obtained for quartz grains, which are regarded as being the most reliable in luminescence dating. Supporters of luminescence methods are constantly growing, however, these groups do not always have sufficient knowledge to avoid even the most basic of issues that may be encountered overall – from the process of sampling through to the awareness of what a single luminescence result represents. The present paper provides an overview of several practical aspects of luminescence dating such as correct sampling procedures and all necessary information regarding the calculation of the dose rate and equivalent dose with particular reference to potential problems that occur when the age of the sample is being determined. All these aspects are crucial for obtaining a reliable dating result, on the other hand, they remain a potential source of uncertainty.
EN
South-Eastern coastal plains of India experience some of the major delta formations of the Indian subcontinent majorly affected by fluctuations of the Indian summer monsoon (ISM) and sea level. Past shoreline signatures in the form of palaeo beach ridges in Kaveri delta (Tamil Nadu, India), suggest a wave-dominated delta and thus past sea-level variations affecting directly the sedimentary dynamics of the Kaveri river forcing the river to either aggrade or prograde. Chronostratigraphic and foraminiferal study of the 25 m deep sediment core taken 2.5 km onshore from Tamil Nadu coast, Kaveri delta shows evidence of changing coastline over the last 150 ka. Various units in the core reflect eight major phases of increased sea level (~3.4 ka, ~5.0 ka, 9–6 ka, 60–57 ka, 89–81 ka, ~102 ka,~121 ka and 143–140 ka) partly coinciding with the global climate cycles MIS 1, MIS 3, MIS 5, MIS 6 respectively during the late Quaternary period. During ~121 ka and 9–6 ka, direct signature of marine transgression is observed by the presence of foraminifera in the core location. The study also shows that the sea transgression during ~121 ka was much longer-lasting and higher than during 9–6 ka, even though not revealed in the Quaternary sea level curve given by previous authors. Depositional breaks are observed in the core during periods of lower sea levels as the river responded by incision. Total organic matter of the deposition between 9–6 ka was observed as high as 2.5–6% suggesting oxygen stressed conditions during the period.
EN
Litho-, pedo- and palynological analyses constrained by radiometric dating of two loess-palaeosol sequences, Nahirne and Velyka Andrusivka, exposed in a cliff at the eastern edge of the Dnieper Upland, Ukraine, document regional environmental changes in the western marginal zone of the Dnieper lobe. The postglacial loess sedimentation cycle was initiated during MIS 8, immediately after the ice sheet recession. On the basis of palaeorelief analysis, subsequent morphogenetic stages of the original postglacial relief, associated with the modifying and masking role of the loess, and destructive slope processes were reconstructed. Periglacial steppe with consistently present scattered trees formed the Pleistocene landscape in the Middle Dniester area during the last three glacial periods. In such an environment, the following loess beds, correlated with marine isotope stages (MIS), were deposited: Dnieper (dn) - MIS 8, Tyasmyn (ts) - MIS 6, Uday (ud) - MIS 4 and Bug (bg) - MIS 2. During the last two warm periods: Kaydaky (kd) - MIS 7 and Pryluky (pl) - MIS 5, the landscape was not fully forested. As a result, the individual palynological features of these soils show a diverse character. The TL and OSL dates form a sequence with numerous inversions that are difficult to interpret. Although these data do not significantly influence the interpretation, they show that: 1) there are loesses that undoubtedly formed after the maximum extent of the ice sheet by short-distance transport of dust material from local fresh glacial deposits and the underlying Paleogene rocks; 2) date distortions result from the activities of an exceptionally rich pedofauna that has contaminated the material not only in the soil sections of the profile but also in the adjacent loess. It is possible to delimit a few stages of pedofaunal activity in each of the soil units.
EN
The Volochysk site belongs to important and unique loess sites in the Podolia Upland (W Ukraine) because it contains relatively well-developed loess deposits representing the last and penultimate glacial cycles. This loess-palaeosol sequence consists of pedocomplex S1 (MIS 5) developed on loess L2, and loess L1 (MIS 4-2) with the palaeosols of lower, interstadial rank. In this sequence, different periglacial structures were found, including the largest ones of ice-wedge cast type. Different quartz and polymineral fractions separated from the samples collected in the Volochysk site were dated using luminescence methods (SAR OSL, post-IR IRSL and TL) in three Polish luminescence laboratories in Gdańsk, Gliwice and Lublin. In total, 69 luminescence dating results were obtained for 18 samples. The methodological and research aims were to carry out mutual verification of the obtained dating results as well as to analyse and interpret the differences between them, and to determine the age of distinguished deposit layers and the period of cryogenic activities. The luminescence dates of the sediments, which were deposited during MIS 2, 3 and 4, corresponded fairly well to the ages attributed to these stages. They also indicate the age of periglacial phenomena. However, the TL dates were generally older than the OSL ones, especially those obtained for the sediments deposited during MIS 5 and 6. The results of the research of the Volochysk sequence were compared with those obtained in past years for the loess deposits of the Volhynian Upland (north of Podolia) during similar inter-laboratory analyses conducted to determine their age. The results of OSL datings of the older deposits (MIS 5 and MIS 6) are underestimated irrespective of the used method, and the type (quartz, polymineral) and size of grains. Numerous attempts were made to explain this phenomenon, which, however, give no answer. It was only found that this underestimation corresponded to the equivalent dose value of ~150 Gy.
10
Content available remote Luminescence chronostratigraphy for the loess deposits in Złota, Poland
EN
Loess formations in Poland display a close relationship with cooling and warming trends of the Northern Hemisphere during the Pleistocene. Loess sequences sensitively record regional palaeoclimatic and palaeoecological changes. The Złota loess profile (21°39’E, 50°39’N) provides a unique opportunity to reconstruct climate conditions in the past in this part of Poland. This continuous sequence of loess and palaeosol deposits allows to distinguish between warmer and more humid climate which is favourable for soil development and much colder and dry periods which are conducive to loess accumulation. The silty and sandy aeolian material originates mainly from weathered rock surfaces affected by frost shattering or from glaciofluvial/fluvial deposits of river flood plains. In Poland, loess and loess-like formations occur in the southern part of the country, mostly in the south polish uplands, i.e. in the Lublin, Sandomierz, and Cracow Uplands. We used different techniques to establish a chronological framework for this site. 21 samples for luminescence dating were collected from the investigated loess profile in Złota. Infrared post-IR IRSL dating method was applied to the polymineral fine grains (4–11µm). The dating results are accompanied by detailed analyses of the geochemical composition, organic carbon and carbonate. Also, analysis of magnetic susceptibility and grain-size distribution were investigated. Based on such a large stratigraphic dataset an age-depth model using OxCal has also been constructed for this site.
EN
Recent developments in the use of more stable feldspar signals in the luminescence dating of sediments offer the possibility of obtaining accurate feldspar luminescence ages for ceramic artefacts; this is especially interesting in locations which do not provide suitable quartz extracts. Here we examine the application of the stable infrared stimulated luminescence signal measured at elevated temperature (in this case 290°C; pIRIR290) after stimulation at about room temperature to Levantine pottery samples. A total of 52 potsherds were collected from three superimposed iron-age units at Pella (Jordan); based on 14C dating, typology and seriation these units were deposited between 700 and 900 BCE. Sand-sized quartz extracts were unsuitable, and there was insufficient sand-sized feldspar, and so polymineral fine grains were chosen for dating. Various tests for reliability were undertaken (dose recovery, dependence of De on first stimulation temperature etc.). The pIRIR signals are weak, and 14 potsherds were rejected on this basis. Of the remainder, 3 were confidently identified as outliers. Based on those sherds for which IR signals were sufficiently intense, we use the ratio of the IR50 to pIRIR290 signals to argue that these outliers do not arise from incomplete resetting during manufacture. The ages from each layer are considerably over dispersed (typically by ~25%) but average ages for each unit are consistent with each other and with the expected age range. The average OSL age for the site is 2840 ± 220 years (n = 35), with the overall uncertainty dominated by systematic uncertainties; this average is consistent with the range of 14C ages from 970–1270 BCE reported from across the destruction horizon. We conclude that the pIRIR290 signal is delivering accurate ages, but that the variability in age from shard to shard is much greater than would be expected from known sources of uncertainty. This demonstrates the need for site ages to be based on multiple samples; individual shard ages are unlikely to be sufficiently accurate.
12
Content available remote OSL chronostratigraphy for loess deposits from Tyszowce – Poland
EN
The presented work concerns a loess profile located in Tyszowce, in the eastern part of Poland on the Volyn Upland, close to the Ukrainian border. The investigated loess formation is well preserved and is characterised by clear stratigraphic units providing an opportunity to refine the loess chronostratigraphy in Poland. In the paper, we present luminescence ages of loess from the last glacial cycle in SE Poland (up to about 100 ka) together with seven radiocarbon ages. Twenty-one samples were collected and dated using infrared (post-IR IRSL) and blue light stimulated luminescence dating. Two fractions were used, namely polymineral fine grains (4–11 μm) and medium sized quartz grains (45–63 μm). The obtained luminescence ages show very good agreement of both methods in relation to loess deposits, however for the fossil soil units the post-IR IRSL method yields older ages. Radiocarbon dates also confirm luminescence chronostratigraphy for younger units. Moreover, the luminescence results are supported by detailed analyses of grain size distribution, carbonate content and magnetic susceptibility variations allowing to create a comprehensive picture of chronological evolution of this site.
EN
Presented are the results of research into the fluvio-aeolian sedimentary succession at the site of Postolin in the Żmigród Basin, southwest Poland. Based on lithofacies analysis, textural analysis, Thermoluminescence and Infrared-Optical Stimulated Luminescence dating and GIS analysis, three lithofacies units were recognised and their stratigraphic succession identified: 1) the lower unit was deposited during the Pleni-Weichselian within a sand-bed braided river functioning under permafrost conditions within the central part of the alluvial fan; 2) the middle unit is the result of aeolian deposition and fluvial redeposition on the surface of the fan during long-term permafrost and progressive decrease of humidity of the climate at the turn of the Pleni to the Late Weichselian; 3) the upper unit accumulated following the development of longitudinal dunes at the turn of the Late Weichselian to the Holocene; the development of dunes was interrupted twice by the form being stabilised by vegetation and soil development.
EN
This study describes the luminescence characteristics of quartz of Upper Pleistocene loess of the Middle Rhine area. The loess/palaeosol sequence of the Schwalbenberg near Remagen comprises a multitude of interstadial soils and soil sediments that have been dedicated to the Marine Isotope Stage 3 (MIS 3). These weak calcaric cambisols and their derivates are underlain by loess and soil sediments of MIS 4 to MIS 5 and covered by loess sediments and intercalated gelic gleysols of MIS 2. We applied luminescence dating of quartz and feldspar of drill core samples and observed an age discrepancy within both data sets. The quartz ages were clearly younger than the feldspar ages, because of thermally unstable signal components of the quartz luminescence signal. Therefore, we regarded the quartz samples of the lower parts of the drill core as unsuitable for luminescence dating. This underestimation did not affect the quartz samples of the upper part of the drill core which was indicated by age control that was provided by the Eltville tephra layer. Geochemical analysis based on X-ray fluorescence showed that the sediments in the upper part and the lower part of the drill core have different geogenic finger prints most likely due to changing source areas of dust and sediment allocation. We assumed that these different facies types were the reason for the luminescence behavior of the quartz samples.
EN
Following the luminescence system lexsyg research, which was designed for research, the luminescence reader lexsyg smart for the application of luminescence detection was developed by Freiberg Instruments. It is suited for routine measurements of luminescence (thermoluminescence, photoluminescence, photon-stimulated, optically stimulated and infrared stimulated luminescence) for a wide range of materials because of the availability of several stimulation sources. The possibility for user definition and change of most parameters provides a great deal of flexibility and also allows research applications. While detection is limited to a single unit and sample storage to 40 positions, the lexsyg smart is much faster in aliquot transportation compared to the lexsyg research, and allows fast mass measurements in luminescence dating, retrospective and personal dosimetry, etc. Cross talk of optical stimulation is absent and cross-irradiation is negligible from the single radioactive source (α, β or x-ray) because of a disconnected sample storage wheel from the measurement chamber, which has a small volume and therefore gas consumption is small. Thermoluminescence measurements and pre-heatings are possible with a versatile heater, which can be programmed for linear/non-linear heating at varying rates and durations for an almost unlimited number of steps. Optical excitation for up to three wavelength bands (violet, blue, green, yellow, infrared) is provided from high power LEDs or laser diodes, with an optional filter wheel to vary detection wavelength bands according the material specific requirements. Either can be programmed to change at almost any time within measurement sequences.
16
Content available remote Performance tests using the Lexsyg luminescence reader
EN
This study presents test measurements on a Lexsyg luminescence reader, acquired by the Giessen luminescence group. The reader is of the type Standard, hence designed for routine determi-nation of palaeodoses using quartz or K-feldspars. The tests include measurements of the stimulation powers, preheat temperatures, OSL- and TL-curves, as well as dose recovery tests and calibration measurements using highly sensitised calibration quartz. A comparison of De values determined using a Lexsyg reader with single grain De -values, which have been previously obtained on a Risø reader, is also presented. The results imply that the Lexsyg reader is a highly reliable measurement device with high reproducibility, yielding instrumental uncertainties of around 0.3%.
17
Content available remote Different approaches to date bricks from historical buildings
EN
The application of Thermally (TL) and Optically (OSL) Stimulated Luminescence on bricks used as building material has allowed solving an chronological issue in the field of historical building dating. The possibility to use one or more methodologies of dating is closely related to the luminescent and granulometric characteristics of the sample. Using some brick samples collected in the church of Sain Seurin in Bordeaux (France), this paper discusses the implications and the possibility to use different approaches and techniques for dating. With this aim luminescence measurements were performed on both polymineral fine grain and quartz inclusion phases extracted from each brick. For Equivalent Dose (ED) and consequently age determination, TL on mixed fine grain fraction (FG), OSL on quartz inclusions (QI) and on mixed fine grain (FG*) fraction, were used. The results obtained suggest the advantage of using OSL technique on fine grain fraction cleaned up by IR stimulation (FG*), but the use of quartz inclusion represents indeed a good alternative.
EN
The morphogenesis and inner structure of the Holocene foredune plain in the Narva-Joesuu area, eastern Gulf of Finland, were studied using optically stimulated luminescence (OSL) dating, ground-penetrating radar (GPR) study and interpretation of airborne LIDAR elevation data. The results show that the Narva-Joesuu foredune plain consists of ca. 100 parallel coastal foredune ridges built of well-sorted fine sand underlain by gently (~7°) seaward-dipping sandy beach deposits. The distal part of the plain, which consists of at least 15 ridges, formed during the regressive phase of the Ancylus Lake/Early Litorina Sea, serving as a barrier for the lagoon behind it. A larger portion of ridges, with an average progradation rate of 0.26 m a-1, formed under conditions of falling relative sea level during the Litorina regression and was separated from the older foredune succession by a hiatus related to the Litorina transgression at 8.5-7.3 cal. ka BP. In the highest central part of the plain the foredune growth was interrupted by foredune instability and a re-blowing episode dated to 5.4 ± 0.9 ka BP which may correlate with a larger regional cooling at 5.8-5.1 cal. ka BP in the North Atlantic and central Europe. During the last 3000 years, the foredune progradation rate decreased to 0.19 m a-1, most probably because of decelerated land-uplift and increased human impact due to coastal protection.
EN
This study investigates the potential of luminescence to date deposits from different fluvial sedimentary environments; namely point bar deposits, sandy and silty channel fills and floodplain sediments. Samples were taken from Holocene (<5 ka) terraces of the Lech and Danube rivers, for which independent age constraint is available through 14C ages, archaeological data and historical maps. OSL-ages were obtained using small aliquots of coarse grain quartz for the majority of sam-ples. Two further samples were dated by the IRSL-signals of polymineral fine grain extracts, as no sufficient number of coarse grains could be extracted from these sediments. In order to detect and ac-count for incomplete bleaching, we used the decision process suggested by Bailey and Arnold [Statis-tical modelling of single grain quartz De distributions and an assessment of procedures for estimating burial dose. Quaternary Science Reviews 25, 2475-2502, 2006]. Although their model was designed for single grains of quartz, our study shows that it is also applicable to multiple grains of quartz, pro-vided that a low number of luminescent grains is present on one aliquot. Luminescence ages of point bar deposits and a sandy channel fill correspond most closely to the independent age control. In the floodplain, sand-striped floodplain channel deposits were incompletely bleached to a moderate de-gree, yielding ages with acceptable overestimations, while fine-grained floodplain deposits were worst bleached. One crevasse splay deposit was so severely incompletely bleached that none of the age models was able to yield accurate ages.
20
Content available remote Lexsyg – a new system for luminescence research
EN
The newly developed lexsyg system by Freiberg Instruments is a versatile luminescence reader, suited for research on the luminescence of materials, fundamental research in luminescence dating, but also for routine mass measurements in retrospective dosimetry as well as in dating application. The 80 sample storage wheel is disconnected from the measurement chamber and therefore crosstalk of optical stimulation is absent and cross-irradiation is negligible from the α- and β-sources, which are providing very uniform irradiations, with the latter especially designed for radiofluorescence (RF) measurement. Optical excitation sources and filter wheels to vary detection wavelengths can be programmed to change at almost any time within measurement sequences, including the auto-mated change of an optional wheel holding up to four different detectors. Thermoluminescence measurements and preheating are possible with a versatile heater, which can be programmed for linear or non-linear heating or cooling, as well as holding a temperature constant. Rates as well as durations can be varied, together with individual ramping, staging and cooling for an almost unlimited number of steps. Violet- and IR-lasers, green and blue LED-arrays can be operated in continuous (CW) or modulated mode (linear/non-linear), and optionally for pulsed as well as time resolved luminescence detection. Six arrays of power LEDs allow the simulation of different bleaching regimes (‘solar simulator’), while luminescence detection can be achieved by a variety of photomultiplier tubes and by CCD cameras for spatially resolved measurements and luminescence spectra.
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