0.94Bi0.5Na0.5TiO3-0.06BaTiO3 ceramics were fabricated by sol-gel technique. The XRD results revealed the formation of a single phase perovskite structured Bi0.5Na0.5TiO3-BaTiO3 at 600 °C. The SEM images showed dense microstructure and the optimum density of the ceramics sintered at 1100 °C was 5.2 g/cm3. The saturation polarization (P s ) was found to be increased with increasing temperature while the remnant polarization (P r ) was found to be increased gradually and then decreased abruptly near 85 °C, which could be attributed to the phase transformation. The coercive electric field (E c ) was found to be decreased gradually with increasing temperature. The maximum value of dielectric constant (ɛ r ) at room temperature was 800 and dielectric loss at 1 MHz was 0.07.
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