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Progowa spektroskopia fotoelektronowa cząsteczek

Zubek Mariusz

Postępy Fizyki

2021

T. 72, z. 2

2--8

Spektroskopia fotoelektronowa stosowana jest w badaniach struktury i dynamiki zewnętrznych i wewnętrznych powłok elektronowych atomów, cząsteczek oraz klasterów w fazie gazowej. W artykule przedstawiono progową spektroskopię fotoelektronową, w której rejestruje się fotoelektrony z prawie zerową energią kinetyczną. Zilustrowano ją omawiając progowe widma fotoelektronowe cząsteczek azotu i furanu otrzymane w pomiarach z wykorzystaniem promieniowania synchrotronowego. Widma te wskazują na znaczny udział stanów autojonizacyjnych w procesach fotojonizacji progowej.

Photoelectron spectroscopy is applied to investigate electronic structure and electron dynamics in outer and inner shells of atoms, molecules and clusters in the gas phase. he article presents threshold photoelectron spectroscopy is presented, in which photoelectrons with near zero kinetic energy are detected. It is illustrated by describing the photoelectron spectra of nitrogen and furan obtained in the measurements using synchrotron radiation. These spectra show signifcant contributions of the autoionizing states to the processes of threshold photoionization.

Electromagnetically induced transparency for A-like systems with degenerate autoionizing levels and a broadband coupling laser

Khoa D. Q., Van C. L., Lanh C. V., Phuc H. V.

Optica Applicata

2016

Vol. 46, nr 1

93--102

In our previous paper (DOAN QUOC K. et al., Physica Scripta T147, 2012, article 014008), electromagnetically induced transparency for A-like systems consisting of two lower bound states and a flat continuum coupled to an autoionization state embedded in it has been considered, in which the laser coupling light is modeled by white noise. In this paper, we investigate a similar scheme, where the continuum involved in the problem is replaced by one with so-called the double-A system, when instead of one autoionization state we have two autoionization states of the same energy embedded in the continuum. For such a system containing degenerate autoionization levels we derive a set of coupled stochastic integro-differential equations which can be averaged exactly. This leads to the exact formula determining the stationary solution for the electric susceptibility. Dispersion and absorption spectra for electromagnetically induced transparency are found and compared with those obtained previously by us and other authors.

Electromagnetically induced transparency in systems with degenerate autoionizing levels in Λ-configuration

Dinh T. B., Leoński W., Perina J., Long V. C.

Optica Applicata

2013

Vol. 43, nr 3

471--484

We discuss a Λ-like model of atomic levels involving two autoionizing (AI) states of the same energy. The system is irradiated by two external electromagnetic fields (strong – driving and weak – probing). For such a system containing degenerate AI levels we derive the analytical formula describing the medium susceptibility. We show that the presence of the second AI level leads to the additional electromagnetically induced transparency (EIT) window appearance. We show that the characteristics of this window can be manipulated by changes of the parameters describing the interactions of AI levels with other ones. This is a new mechanism which leads to additional transparency windows in EIT model, that differs from the mechanism where a bigger number of Zeeman sublevels is taken into account.