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Counterion effects on the alkali dissolution mechanism of quartz

Yao Yu-yun, Tang Yun, Yang Yong, Li Guo-hui, Wu Bo, Dai Wen-zhi

Physicochemical Problems of Mineral Processing

2023

Vol. 59, iss. 1

art. no. 160038

In gold ore, quartz plays an important role in mineral formation by acting as the follower. Understanding counterion release, transport, and deposition in alkali solution is a prerequisite for evaluating the potential role of gold separate from quartz deposits in pretreatment. In this work, the aggregation, retention, and release of counterion in alkali solution media were investigated by kinetic research and pure mineral experiments, the correlation and mechanism of these processes were revealed by combining geochemical theory, interaction energy calculation, and quantum chemistry. The results showed that the retention and release of counterion were closely related to the dissolution and corrosion rate of quartz. The NH4+ and Fe2+ with higher mineral affinity reduced the quartz stability, and the dispersion stability and mobility of the quartz were greatly improved by an alkaline substance due to the enhancement of steric hindrance effects. Quantum chemical calculation results show that ammonium ion promotes the dissolution of quartz stronger than ferrous ion, which is mainly reflected in reducing the activation energy required for the formation of transition state (TS1), which can be verified by kinetic calculation. These findings provide essential insight into the extraction of gold coated by quartz as well as a vital reference for the experiment of gold-loaded quartz leaching in mineral processing.

Study on the three-phase flow of the water transfer export elbow of natural gas hydrate

Chen Wei, Xu Hai-Liang, Wu Bo, Yang Fang-Qiong

Archives of Mining Sciences

2022

Vol. 67, no. 2

239--258

The Euler multiphase flow and population equilibrium model were used to simulate the three-phase flow field in the bubble expansion stage of the outlet curved pipe section. The influence of the ratio of the bending diameter and the volume fraction of the gas phase on the pressure loss is revealed, and the safety range of the optimum bending diameter ratio and the volume fraction of the outlet gas phase is determined. The results show that the three-phase flow in the tube is more uniformly distributed in the vertical stage, and when the pipe is curved, the liquid-phase close to the pipe wall gathers along the pipe flank to the outside of the pipe, the solid phase is transferred along the pipe flank to the inside of the pipe, and the gas phase shrinks along the pipe flank to the inner centre. The maximum speed of each phase of the three-phase flow in the elbow is at the wall of the tube from 45° to 60° inside the elbow, and the distribution law along the axial direction of the pipe is about the same as the distribution law of volume fraction. The pressure loss of the elbow decreases with the increase of the bend diameter ratio, when the bend diameter ratio increases to 6, the pressure loss of the pipe decreases sharply, and the pressure loss decreases slowly with the increase of the bend diameter ratio. When the gas phase volume score in the elbow reaches 70%, there will be an obvious wall separation phenomenon, to keep the system in a stable working state and prevent blowout, the gas phase volume score should be controlled within 60%.