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Adsorption of 4-aminopyrimidine at the R-AgLAFE/chlorate(VII) interface. Comparison of the adsorption properties of various water activity as well as different surfactants

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Języki publikacji
EN
Abstrakty
EN
The results of 4-aminopyrimidine (4-APM) impact studies on the double layer parameters at the R-AgLAFE/ chlorates(VII) interface in the solutions with different water activity as well as different properties of the mixed adsorption layer of 4-aminopirimidine - sodium 1-decanesulfonate (SDS) and 4- aminopyrimidine - hexadecyltrimethylammonium bromide (CTAB) at the electrode/solution interface are discussed.The differential capacity of the double layer (Cd) at the R-AgLAFE/ basic solution interface was measured using the electrochemical impedance spectroscopy. The zero charge potential (Ez) was determined using a streaming electrode, while the surface tension at the zero charge potential (Yz) was measured using the largest pressure method inside the mercury drop. It was proved that both the 4-aminopirymidine concentration and water activity have an essential effect on the doublelayer parameters on the R-AgLAFE/ chlorates(VII) interface. In the studied systems: 4-APM - SDS and 4-APM - CTAB, 4-aminopyrimidine dominance was observed.
Słowa kluczowe
Rocznik
Strony
art. no. 170204
Opis fizyczny
Bibliogr. 28 poz., rys., wykr., tab.
Twórcy
  • Faculty of Chemistry, Maria Curie-Sklodowska University, Maria Curie-Sklodowska Sq. 3, 20-031 Lublin, Poland
  • Faculty of Chemistry, Maria Curie-Sklodowska University, Maria Curie-Sklodowska Sq. 3, 20-031 Lublin, Poland
  • Faculty of Chemistry, Maria Curie-Sklodowska University, Maria Curie-Sklodowska Sq. 3, 20-031 Lublin, Poland
  • Faculty of Chemistry, Adam Mickiewicz University in Poznań, Uniwersytetu Poznańskiego 8, 61-614 Poznań, Poland
  • Faculty of Chemistry, Adam Mickiewicz University in Poznań, Uniwersytetu Poznańskiego 8, 61-614 Poznań, Poland
  • Faculty of Chemistry, Maria Curie-Sklodowska University, Maria Curie-Sklodowska Sq. 3, 20-031 Lublin, Poland
Bibliografia
  • AKYUZ, S., AKYUZ, T., 2004. FT-IR spectroscopic investigations adsorption of pyrazinamide and 4-aminopyrimidine by clays.J. Incl. Phenom., 48, 75-80.
  • ARYAN, R., BEYZAEI, H., SADEGHI, F., 2016. Facile Synthesis of Some Novel Tetrasubstituted 2, 4‐Diaminopyrimidine Derivatives in Aqueous Glucose Solution as a Fully Green Medium and Promoter.J.Heterocycl.Chem. 53(6), 1963-1969.
  • BALAKRISHNAN, A., GAO, Y., MOORJANI, P., NEMERIA, N. S., TITTMANN, K., JORDAN, F., 2012. Bifunctionality of the thiamindiphosphate cofactor: Assignment of tautomeric/ionizationstates of the 4′-aminopyrimidine ring when various intermediates occupy the active sites during the catalysis of yeast pyruvatedecarboxylase.J.Am.Chem.Soc. 134(8), 3873-3885.
  • BATANA, A., FILHO, R. R., AVACA, L. A., GONZÁLEZ, E. R., 1981. Determination of electrical double‐layer parameters for the adsorption of neutral molecules at the electrode–solution interface. J.Comput.Chem. 2(3), 221-224.
  • BRYCHT, M., SKRZYPEK, S., NOSAL-WIERCIŃSKA, A., SMARZEWSKA, S., GUZIEJEWSKI, D., CIESIELSKI, W., BURNAT, B., LENIART, A., 2014. The new application of renewable silver amalgam film electrode for the electrochemical reduction of nitrile, cyazofamid, and its voltammetric determination in the real samples and in a commercial formulation. Electrochim. Acta. 134, 302–308.
  • DUEVA, E. V., TUCHYNSKAYA, K. K., KOZLOVSKAYA, L. I., OSOLODKIN, D. I., SEDENKOVA, K. N., AVERINA, E. B., KARGANOVA, G. G. 2020. Spectrum of antiviral activity of 4-aminopyrimidine N-oxides against a broad panel of tick-borne encephalitis virus strains.Antivir.Chem.Chemother. 28, 2040206620943462.
  • FARIAS, P. A., WAGENER, A. D. L. R., CASTRO, A. A., 2001. Ultratrace determination of adenine in the presence of copper by adsorptive stripping voltammetry.Talanta. 55(2), 281-290.
  • GUGAŁA-FEKNER, D., NIESZPOREK, J., SIEŃKO, D., 2015. Adsorption of anionic surfactant at the electrode–NaClO 4 solutioninterface.Monatsh.Chem. 146, 541-545.
  • GUGALA-FEKNER, D., 2021. Adenine adsorption in different pH acetate buffer. Available at SSRN 3881627. IKEDA, O., JIMBO, H., TAMURA, H., 1982. Adsorption of tetramethylthiourea at the mercury/water interface.J. Electroanal. Chem. Interfacial Electrochem., 137(1), 127-141.
  • KLIN, M., NIESZPOREK, J., SIEŃKO, D., GUGAŁA-FEKNER, D., SABA, J., 2011. Adsorption of tetramethylthioureain the presence of cationic detergent at interface electrode/aqueous perchlorate solutions. Croat. Chem. Acta. 84, 475–480.
  • KUMAR, D., RUB, M.A., 2019. Role of cetyltrimethylammonium bromide (CTAB) surfactant micelles on kinetics of [Zn (II)-Gly-Leu]+ and ninhydrin. J. Mol. Liq. 274, 639-645.
  • MARTÍN-YERGA, D., GONZÁLEZ-GARCÍA, M. B., COSTA-GARCÍA, A., 2013. Electrochemical determination of mercury: A review.Talanta. 116, 1091-1104.
  • MARTYNA, M., GROCHOWSKI, M., URBAN, T., NOSAL-WIERCIŃSKA, A., 2022. Study of 2–thiocytosine/surfactant adsorption at the R-AgLAFe/chlorate (VII) interface–impact of surfactant ionic character. Physicochem. Probl. Miner. Process. 58(2).
  • NEMERIA, N. S., CHAKRABORTY, S., BALAKRISHNAN, A., JORDAN, F., 2009. Reaction mechanisms of thiamin diphosphate enzymes: defining states of ionization and tautomerization of the cofactor at individual steps.FEBS J. 276(9), 2432-3446.
  • NOSAL-WIERCIŃSKA, A., 2010. Adsorption of cystine at mercury/ aqueous solution of chlorate (VII) interface in solutions of different water activity. Cent. Europ. J. Chem. 10, 1290–1300.
  • NOSAL‐WIERCIŃSKA, A., DALMATA, G., 2010. Adsorption of methonine at mercury/aqueous solution of chlorate (VII) interface; dependence on the supporting electrolyte concentration.Electroanalysis. 22(17‐18), 2081-2086.
  • NOSAL-WIERCIŃSKA, A., GROCHOWSKI, M., WIŚNIEWSKA, M., TYSZCZUK-ROTKO, K., YILMAZ, S., YAGMUR, S., YANIK, S. 2015. Adsorption of selected amino acids at the mercury/aqueous solution interface from the chlorate (VII) and its dependence on the supporting electrolyte concentration.Adsorp. Sci. Technol. 33(6-8), 553-558.
  • NOSAL-WIERCIŃSKA, A., WIŚNIEWSKA, M., GROCHOWSKI, M., KALISZCZAK, W., SKRZYPEK, S., BRYCHT, M., FRANUS, W., 2017. The effect of homocysteine and homocystine protonation on double-layer parameters at the electrode/chlorates (VII) interface.Adsorp. Sci. Technol. 35(5-6), 396-402.
  • NOSAL-WIERCIŃSKA, A., KALISZCZAK, W., GROCHOWSKI, M., WIŚNIEWSKA, M., KLEPKA, T., 2018. Effects of mixed adsorption layers of 6-mercaptopurine–Triton X-100 and 6-mercaptopurine–Tween 80 on the double layer parameters at the mercury/chlorates (VII) interface. J. Mol. Liq. 253, 143-148.
  • NOSAL-WIERCIŃSKA, A., MARTYNA, M., GROCHOWSKI, M., BAŚ, B., 2021. First electrochemical studies on “CAP—PAIR” effect for Bi (III) ion electroreduction in the presence of 2-Thiocytosine on novel cyclically renewable liquid silver amalgam film electrode (R-AgLAFE).J. Electrochem. Soc. 168(6), 066504.
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  • PALECˇEK, E., JELEN, F., 2005. Electrochemistry of nucleicacids. In: Palecˇek E, Scheller F, Wang J (eds) Perspectives in Bioanalysis, vol 1. Elsevier, Amsterdam, 73
  • RACZYŃSKA, E. D., KOLCZYŃSKA, K., STĘPNIEWSKI, T. M., 2012. Consequences of one-electron oxidation and one-electron reduction for 4-aminopyrimidine—DFT studies. J. Mol. Model. 18, 3523-3533.
  • RASTOGI, S. C., 2007. Essentials of animal physiology. New Age International
  • SKOMPSKA, M., 1991. The effect of LiClO4 concentration on the adsorption behaviour of thiourea at the mercury-ethanolic solution interface.J. Electroanal. Chem. Interfacial Electrochem. 319(1-2), 331-339.
  • VAZ-DOMINGUEZ, C., ESCUDERO-ESCRIBANO, M., CUESTA, A., PRIETO-DAPENA, F., CERRILLOS, C., RUEDA, M., 2013. Electrochemical STM study of the adsorption of adenine on Au (111) electrodes. Electrochem.commun. 35, 61-64.
  • VENTURINI FILHO, E., PINHEIRO, E. M., PINHEIRO, S., GRECO, S. J., 2021. Aminopyrimidines: Recent synthetic procedures and anticancer activities. Tetrahedron. 92, 132256.
  • ZHOU, Z., ZHOU, X., WANG, X., JIANG, B., LI, Y., CHEN, J., XU, J., 2017. Ultrafast excited-state dynamics of cytosine aza-derivative and analogues. J. Phys. Chem. 121(14), 2780-2789.
Uwagi
Opracowanie rekordu ze środków MNiSW, umowa nr SONP/SP/546092/2022 w ramach programu "Społeczna odpowiedzialność nauki" - moduł: Popularyzacja nauki i promocja sportu (2024).
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-ea215736-d3e4-44be-84ff-20638806a1c5
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