FTIR and Raman spectroscopic study of a complex perovskite: Ca0.91-xCe0.09Rb0.04Csx [(Zr0.50Ti0.45)Al0.05]O3, x=0.2 to 0.4, dedicated for radioactive waste confinement

Hasnat, K.; Kamel, N.; Moudir, D.; Mouheb, Y.; Kamariz, S.; Arabi, A.

doi:10.2478/adms-2020-0012

Artykuł - szczegóły

Tytuł artykułu

FTIR and Raman spectroscopic study of a complex perovskite: Ca0.91-xCe0.09Rb0.04Csx [(Zr0.50Ti0.45)Al0.05]O3, x=0.2 to 0.4, dedicated for radioactive waste confinement

Autorzy

Hasnat K. , Kamel N. , Moudir D. , Mouheb Y. , Kamariz S. , Arabi A.

Wybrane pełne teksty z tego czasopisma

http://content.sciendo.com/view/journals/adms/adms-overview.xml

Identyfikatory

DOI

10.2478/adms-2020-0012

Warianty tytułu

Języki publikacji

Abstrakty

Perovskite is able to sequester simultaneously, in its structure, both actinides and alkaline-earth elements. This study is an attempt to synthesize a complex perovskite Ca_0.91-xCe_0.09Rb_0.04Cs_x [(Zr_0.50Ti_0.45)Al_0.05]O₃ (0.2≤x≤0.4), doped in the same time, with Ce, Cs and Rb. The synthesis is conducted by sintering at 1150°C during 16h. XRX analysis confirms the perovskite formation. SEM observations show a less porous microstructure. FTIR analysis reveals TiO₆, Ti-O-Ti, Ti-O and Zr-O vibrations. Raman spectroscopy indicates many orthorhombic perovskite active modes, as: Ti-O₆ and Ti-O₃ torsions, ZrO₇, CaO₈ vibrations, the totally symmetric oxygen, and the O-octahedron cage rotation.

Słowa kluczowe

perovskite radioactive waste XRD X-ray diffraction FTIR Fourier transform infrared spectroscopy Raman spectroscopy

perowskit odpady radioaktywne XRD dyfrakcja rentgenowska FTIR spektroskopia fourierowska w podczerwieni spektroskopia ramanowska

Wydawca

Politechnika Gdańska

Czasopismo

Advances in Materials Science

Rocznik

2020

Tom

Vol. 20, nr 2(64)

Strony

81--94

Opis fizyczny

Bibliogr. 73 poz., wykr., rys.

Twórcy

autor

Hasnat K.

Chahid Abderrahmane Taleb Military Polytechnique School, Algiers, Algeria

autor

Kamel N.

h.kamel@crna.dz

Algiers Nuclear Research Center, Division of Environment, Safety, and Radioactive Waste, Algiers, Algeria

autor

Moudir D.

Algiers Nuclear Research Center, Division of Environment, Safety, and Radioactive Waste, Algiers, Algeria

autor

Mouheb Y.

Algiers Nuclear Research Center, Division of Environment, Safety, and Radioactive Waste, Algiers, Algeria

autor

Kamariz S.

Algiers Nuclear Research Center, Division of Environment, Safety, and Radioactive Waste, Algiers, Algeria

autor

Arabi A.

Algiers Nuclear Research Center, Division of Environment, Safety, and Radioactive Waste, Algiers, Algeria

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Uwagi

Opracowanie rekordu ze środków MNiSW, umowa Nr 461252 w ramach programu "Społeczna odpowiedzialność nauki" - moduł: Popularyzacja nauki i promocja sportu (2021).

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Bibliografia

Identyfikator YADDA

bwmeta1.element.baztech-e8b8373f-1087-469b-86de-4938529c3c2c