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Zintegrowane oczyszczanie spalin z SO2, NOx i Hg układach mokrego odsiarczania spalin

Autorzy
Krzyżyńska R.
Identyfikatory
Warianty tytułu
EN
Integrated removal of S02, NOx and Hg in the wet flue gas desulphurization systems
Języki publikacji
PL
Abstrakty
PL
W pracy przedstawiono badania nad zintegrowanym oczyszczaniem spalin z dwutlenku siarki, tlenków azotu i rtęci w układach mokrego odsiarczania spalin, które przeprowadzono w skali laboratoryjnej i pilotowej. Wykazano także, że klasyczne układy mokrego odsiarczania spalin zasilane zawiesiną węglanu wapnia mogą pełnić rolę zintegrowanego absorbera, usuwającego nie tylko dwutlenek azotu, lecz także tlenki azotu i rtęć po przeprowadzeniu zabiegów polegających na konwersji nierozpuszczalnego monotlenku azotu znajdującego się w spalinach do rozpuszczalnej formy dwutlenku azotu lub też wyższych form, a także konwersji rtęci metalicznej do formy rozpuszczalnej. Celem badań było dogłębne poznanie i zbadanie procesów zachodzących w zintegrowanym absorberze, które umożliwiłyby zrozumienie mechanizmów usuwania zanieczyszczeń oraz określenie wpływu kluczowych parametrów na przebieg i sprawność tego procesu. Określono więc wpływ: stężeń stosowanych reagentów, stężeń dwutlenku siarki w gazach wyjściowych, stężeń tlenków azotu w gazach wyjściowych, odczynu zawiesiny reakcyjnej, temperatury, miejsca iniekcji roztworu chlorynu sodu w układzie oczyszczania spalin, utworzenia tzw. strefy odsiarczania i utleniania w absorberze kolumnowym z wymuszonym napowietrzaniem, czasu kontaktu gaz-reagent. Ponadto określono rolę, jaką pełnią dwutlenek siarki i jony siarczanowe(IV) i wodorosiarczanowe(IV) w mechanizmie oczyszczania spalin. Zbadano także reemisję rtęci i dwutlenku chloru ze zintegrowanego absorbera zasilanego zawiesiną węglanu wapnia i chlorynu sodu.
EN
This monograph presents the lab- and pilot-scale research on the integrated control of sulphur dioxide, nitrogen oxides and mercury in the wet flue gas desulphurization systems. It is demonstrated that the classical wet limestone scrubbers could be efficient in a removal of sulphur dioxide, nitrogen oxides and mercury simultaneously after the proper modification of chemical processes in the scrubber, which are mainly based on nitrogen oxides and elemental mercury oxidation. The monograph presents the research focusing on better understanding the pollutant removal processes and indicating the key parameters affecting the pollutant removal efficiencies in the integrated scrubber. A series of experiments were performed to evaluate the effect of the most important parameters present in a flue gas cleaning systems on pollutant removals. The following parameters were under study: the effect of reagent concentrations; the effect of initial sulphur dioxide and nitrogen oxides concentrations in flue gas; the pH of reaction medium; temperature; the place of the oxidant injection in the flue gas system; creation of an oxidation and absorption zones in a wet tower working under forced oxidation mode; the effect of reagent-gas contact time. Moreover, the role which the sulfite/bi-sulfite ions may play in a total removal mechanism, and the chlorine dioxide and mercury reemission from the wet integrated absorber were investigated, too.
Słowa kluczowe
PL
EN
Wydawca
Oficyna Wydawnicza Politechniki Wrocławskiej
Czasopismo
Prace Naukowe Instytutu Inżynierii Ochrony Środowiska Politechniki Wrocławskiej. Monografie
Rocznik
2012
Tom
Vol. 93, nr 58
Strony
140--140
Opis fizyczny
Bibliogr. 218 poz., tab., rys.
Twórcy
autor
Krzyżyńska R.
  • Instytut Klimatyzacji i Ogrzewnictwa, Wydział Inżynierii Środowiska, Politechnika Wrocławska, Wybrzeże Wyspiańskiego 27, 50-370 Wrocław.
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