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Modelling of Mercury Emissions from Large Solid Fuel Combustion and Biomonitoring in CZ-PL Border Region

Identyfikatory
Warianty tytułu
PL
Modelowanie i biomonitoring emisji rtęci z masowego spalania paliwa stałego na pograniczu polsko-czeskim
Języki publikacji
EN
Abstrakty
EN
Tightening of norms for air protection leads to a development of new and significantly more effective techniques for removing particulate matter, SOx and NOx from flue gas which originates from large solid fuel combustion. Recently, it has been found that combinations of these environmental technologies can also lead to the reduction of mercury emissions from coal power plants. Now the greatest attention is paid especially to the coal power plant in Opatovice nad Labem, close to Hradec Kralove. Its system for flue gas dedusting was replaced by a modern type of cloth fabric filter with the highest particle separation efficiency which belongs to the category of BAT. Using this technology, together with modernization of the desulphurisation device and increasing of nitrogen oxides removal efficiency, leads also to a reduction of mercury emissions from this power plant. The University of Hradec Kralove, the Opole University and EMPLA Hradec Kralove successfully cooperate in the field of toxic metals biomonitoring almost 20 years. In the Czech-Polish border region, comprehensive biomonitoring of mercury in bioindicators Xerocomus badius in 9 long-term monitored reference points is done. The values of mercury concentration measured in 2012 and 2016 were compared with values computed by a dispersion model SYMOS′97 (updated 2014). Thanks to modern methods of dedusting and desulphurisation, emissions of mercury from this large coal power plant are now smaller than before and that the downward trends continues. The results indicate that Xerocomus badius is a suitable bioindicator for a long-term monitoring of changes in mercury imissions in this forested border region. This finding is significant because it shows that this region is suitable for leisure, recreation, and rehabilitation.
Rocznik
Strony
593--604
Opis fizyczny
Bibliogr. 24 poz., rys., tab., wykr.
Twórcy
autor
  • Department of Physics, Faculty of Science, University of Hradec Králové, Rokitanského 62, 50003 Hradec Králové, Czech Republic
autor
  • Department of Physics, Faculty of Science, University of Hradec Králové, Rokitanského 62, 50003 Hradec Králové, Czech Republic
  • Department of Physics, Faculty of Science, University of Hradec Králové, Rokitanského 62, 50003 Hradec Králové, Czech Republic
  • Department of Physics, Faculty of Science, University of Hradec Králové, Rokitanského 62, 50003 Hradec Králové, Czech Republic
autor
  • Department of Physics, Faculty of Science, University of Hradec Králové, Rokitanského 62, 50003 Hradec Králové, Czech Republic
autor
  • EMPLA AG spol. s r. o., Za Škodovkou 305, 503 11 Hradec Králové, Czech Republic
  • Independent Chair of Biotechnology and Molecular Biology, Faculty of Natural Sciences and Technology, University of Opole, ul. kard. B. Kominka 6, 45-035 Opole, Poland
autor
  • Independent Chair of Biotechnology and Molecular Biology, Faculty of Natural Sciences and Technology, University of Opole, ul. kard. B. Kominka 6, 45-035 Opole, Poland
autor
  • Independent Chair of Biotechnology and Molecular Biology, Faculty of Natural Sciences and Technology, University of Opole, ul. kard. B. Kominka 6, 45-035 Opole, Poland
autor
  • Independent Chair of Biotechnology and Molecular Biology, Faculty of Natural Sciences and Technology, University of Opole, ul. kard. B. Kominka 6, 45-035 Opole, Poland
autor
  • Independent Chair of Biotechnology and Molecular Biology, Faculty of Natural Sciences and Technology, University of Opole, ul. kard. B. Kominka 6, 45-035 Opole, Poland
Bibliografia
  • [1] Directive 2010/75/EU of the European Parliament and of the Council on industrial emissions (integrated pollution prevention and control). Offic J European Union. 2010;53(L 334):17-119. DOI: 10.3000/17252555.L_2010.334.eng.
  • [2] Pacyna EG, Pacyna JM, Steenhuisen F, Wilson S. Global anthropogenic mercury emission inventory for 2000. Atmos Environ. 2006;40:4048-4063. DOI: 10.1016/j.atmosenv.2006.03.041.
  • [3] Zeng H, Jin F, Guo J. Removal of elemental mercury from coal combustion flue gas by chloride-impregnated activated carbon. Fuel. 2004;83(1):143-146. DOI: 10.1016/S0016-2361(03)00235-7.
  • [4] Kasey P. EPA Air Toxics Rule will close some W.Va. Power Plants by 2015. The State J. 2011. http://www.statejournal.com/story/16321771/epa-air-toxics-rule-will-close-some-wva-powerplants.
  • [5] Pudasainee D, Kim J-H, Seo Y-C. Mercury emission trend influenced by stringent air pollutants regulation for coal-fired power plants in Korea. Atmos Environ. 2009;44(39):6254-6259. DOI: 10.1016/j.atmosenv.2009.06.007.
  • [6] Boening DW. Ecological effects, transport, and fate of mercury: a general review. Chemosphere. 2000;40:1335-1351. DOI: 10.1016/S0045-6535(99)00283-0.
  • [7] Cartridge filters. Donaldson Company, Inc. http://www2.donaldson.com/toritdce/en-gb/replacement-parts-services/pages/filters-donaldson-units/cartridge-filters.aspx.
  • [8] OMD41 Operating Instructions. Germany: SICK MAIHAK GmbH; 2007 (documentation material of SICK MAIHAK GmbH). https://www.yumpu.com/en/document/view/10531842/omd41-operating-instructions-sick.
  • [9] Engel-Cox J, Oanh NTK, van Donkelaar A, Martin RV, Zell E. Toward the next generation of air quality monitoring: Particulate matter. Atmos Environ. 2013; 80:584-590. DOI: 10.1016/j.atmosenv.2013.08.016.
  • [10] Dołhańczuk-Śródka A, Ziembik Z, Kříž J, Hyšplerová L, Wacławek M. Pb-210 isotope as a pollutant emission indicator. Ecol Chem Eng S. 2015;22(1):49-59. DOI: 10.1515/eces-2015-0004.
  • [11] Bubnik J, Keder J, Macoun J, Maňák J. SYMOS’97. System for modeling of stationary sources - methodological guide). Prague: Czech Hydrometeorological Institute; 1998 (updated 2014). https://www.google.cz/search?q=Vach+Air+protection&ie=utf-8&oe=utf-8&clien.
  • [12] Borrego C, Incecik S. Air Pollution Modeling and Its Application. XVI. New York: Springer; 2004. http://www.worldcat.org/title/air-pollution-modeling-and-its-application-xvi/oclc/840276673.
  • [13] Szopka K, Karczewska A, Kabała C. Mercury accumulation in the surface layers of mountain soils: A case study from the Karkonosze Mountains, Poland. Chemosphere. 2011;83:1507-1512. DOI: 10.1016/j.chemosphere.2011.01.049.
  • [14] Melgar MJ, Alonso J, García, MA. Mercury in edible mushrooms and underlying soil: bioconcentration factors and toxicological risk. Sci Total Environ. 2009;407:5328-5334. DOI: 10.1016/j.scitotenv.2009.07.001.
  • [15] Ernst G, Zimmermann S, Christie P, Frey B. Mercury, cadmium and lead concentrations in different ecophysiological groups of earthworms in forest soils. Environ Pollut. 2008;156(3):1304-1313. DOI: 10.1016/j.envpol.2008.03.002.
  • [16] Dołhańczuk-Śródka A, Ziembik Z, Kříž J, Hyšplerová L, Wacławek M. Investigation of committed radiation dose rate and relationships between alkaline metals concentrations in mushroom Xerocomus badius. Ecol Chem Eng S. 2012;19(4):649-664. DOI: 10.2478/v10216-011-0047-2.
  • [17] Rieder SR, Brunner I, Horvat M, Jacobs A, Frey B. Accumulation of mercury and methylmercury by mushrooms and earthworms from forest soils. Environ Pollut. 2011;159(10):2861-9. DOI: 10.1016/j.envpol.2011.04.040.
  • [18] Svoboda L, Havlíčková B, Kalač P. Contents of cadmium, mercury and lead in edible mushrooms growing in a historical silver-mining area. Food Chem. 2006;96(4):580-585. DOI: 10.1016/j.foodchem.2005.03.012.
  • [19] Falandysz J, Kojta AK, Jarzyńska G, Drewnowska M, Dryżałowska A, Wydmańska D, et al. Mercury in Bay Bolete (Xerocomus badius): bioconcentration by fungus and assessment of element intake by humans eating fruiting bodies. Food Addit Contam Part A Chem Anal Control Expo Risk Assess. 2012;29(6):951-61. DOI: 10.1080/19440049.2012.662702.
  • [20] Falandysz J, Zalewska T, Krasińska G, Apanel A, Yuanzhong W, Pankavec S. Evaluation of the radioactive contamination in fungi genus Boletus in the region of Europe and Yunnan Province in China. Appl Microbiol Biotechnol. 2015;99:8217-8224. DOI: 10.1007/s00253-015-6668-0.
  • [21] Zalewska T, Cocchi L, Falandysz J. Radiocaesium in Cortinarius spp. mushrooms in the regions of the Reggio Emilia in Italy and Pomerania in Poland. Environ Sci Pollut Res Int. 2016;23(22):23169-23174. DOI:10.1007/s11356-016-7541-0.
  • [22] Škrkal J, Rulík P, Fantínová K, Burianová J, Helebrant J. Long-term 137Cs activity monitoring of mushrooms in forest ecosystems of the Czech Republic. Radiat Prot Dosimetry. 2013:157(4):579-84. DOI: 10.1093/rpd/nct172.
  • [23] Betti L, Palego L, Lucacchini A, Giannaccini G. 137Caesium in samples of wild-grown Boletus edulis Bull. from Lucca province (Tuscany, Italy) and other Italian and European geographical areas. Food Addit Contam Part A Chem Anal Control Expo Risk Assess. 2016;5:1-7. DOI: 10.1080/19440049.2016.1256502.
  • [24] Zarubina N. The influence of biotic and abiotic factors on (137)Cs accumulation in higher fungi after the accident at Chernobyl NPP. J Environ Radioact. 2016:161:66-72. DOI: 10.1016/j.jenvrad.2015.11.014.
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-c7f7e329-d262-4ad7-8a01-046da84bb6ea
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