Synthesis of multi-walled carbon nanotubes with controlled inner and outer diameters by ethylene decomposition over Ni/MgO and Co/MgO catalysts

Lemesh, N. V.; Strizhak, P. E.

doi:10.2478/msp-2018-0089

Artykuł - szczegóły

Tytuł artykułu

Synthesis of multi-walled carbon nanotubes with controlled inner and outer diameters by ethylene decomposition over Ni/MgO and Co/MgO catalysts

Autorzy

Lemesh N. V. , Strizhak P. E.

Wybrane pełne teksty z tego czasopisma

Identyfikatory

DOI

10.2478/msp-2018-0089

Warianty tytułu

Języki publikacji

Abstrakty

In this work, multi-walled carbon nanotubes (MWCNTs) with significantly different mean diameters were produced by catalytic CVD over Ni and Co-based supported catalysts. Our results indicate that Ni nanoparticles in the Ni/MgO catalyst are responsible for controlling the inner diameters of the carbon nanotubes. Contrary, Co nanoparticles in the Co/MgO catalyst control the outer diameters of MWCNTs. The "base-growth" mechanism and smaller diameters of the MWCNTs grown on the Ni/MgO catalyst are associated with a strong metal-support interaction (SMSI) resulting from Ni_xMg_1−xO mixed oxide formation. The concept of the weak metal-support interaction (WMSI) between Co nanoparticles and MgO for the Co/MgO catalyst confirms the "tip-growth" mechanism of the MWCNTs.

Słowa kluczowe

carbon nanotube nanoparticles nickel cobalt metal-support interaction

Wydawca

De Gruyter

Czasopismo

Materials Science Poland

Rocznik

2018

Tom

Vol. 36, No. 4

Strony

739--747

Opis fizyczny

Bibliogr. 39 poz., rys., tab.

Twórcy

autor

Lemesh N. V.

lemeshnataliia@gmail.com

L.V. Pisarzhevskii Institute of Physical Chemistry, National Academy of Sciences of Ukraine Prosp. Nauki 31, Kiev 03028, Ukraine

autor

Strizhak P. E.

L.V. Pisarzhevskii Institute of Physical Chemistry, National Academy of Sciences of Ukraine Prosp. Nauki 31, Kiev 03028, Ukraine

Bibliografia

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Uwagi

Opracowanie rekordu w ramach umowy 509/P-DUN/2018 ze środków MNiSW przeznaczonych na działalność upowszechniającą naukę (2019).

Typ dokumentu

Bibliografia

Identyfikator YADDA

bwmeta1.element.baztech-c7b4b968-aba4-4f0b-8d54-69bbeb6f5a6e