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Natlenianie zanieczyszczonych osadów dennych podczas tymczasowego składowania

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Warianty tytułu
EN
Oxygenation of contaminated dredged sediments during temporary upland disposal
Języki publikacji
PL
Abstrakty
PL
Dla badanych osadów określono indeks dojrzewania, stopień kurczenia, współczynnik dyfuzji oraz dystrybucję tlenu. W celu odwodnienia osadów i uzyskania różnych etapów fizycznego dojrzewania osadów zastosowano potencjały matrycowe w zakresie od -100 do -1 000 000 hPa. Sprawdzono wpływ zastosowanego potencjału matrycy na występowanie miejsc pozbawionych tlenu w agregatach osadowych. Przeprowadzone badania pozwoliły na wypracowanie efektywnej metody pomiaru centrów tlenowych w osadach dennych. Dostarczyły one danych o wpływie kurczenia się agregatów na wzrost współczynnika dyfuzji tlenu, a w konsekwencji na wzrost natlenienia, co ma istotne znaczenie dla bioremediacji osadów zanieczyszczonych substancjami organicznymi (np. substancje ropopochodne, WWA) podczas ich tymczasowego składowania.
EN
Temporary disposal is the most widely adopted alternative for sediments dredged annually in some countries (e.g. the Netherlands) for both maintenance and environmental reasons. For good management of disposal sites, knowledge is required about controlling the behaviour of sediments during disposal. A short overview was made about processes that take place during temporary disposal, and how they can affect the biodegradation of organic contaminants. The method of oxygenation measurements within sediments aggregates was developed and improved in order to evaluate the bioremediation potentials during temporary disposal of sediments contaminated with organic compounds. The parameters determined for three studied sediments (I, II and III) included: the ripening index, shrinkage, diffusion coefficient and oxygen distribution in sediment aggregates. To enhance dewatering and to simulate diverse stages of sediment ripening, matrix potentials from -100 to -1,000,000 hPa were applied. The effect of diverse matrix potentials on the formation of oxic and anoxic zones within the aggregates was also determined. The complete transformation of sediments into soil was taking place at matrix potentials between -1000 and -2000 hPa when the ripening indexes for all sediments dropped below 0.7. For lower ripening indexes an increase of pore volumes filled with air was observed. The highest ripening index of 0.5 was for sediment III, in which the highest organic matter content was found. Decreasing matrix potentials resulted in an increase of the O2 penetration depths in sediment aggregates. At the matrix potential of -16,000 and lower, the whole aggregates were fully aerated. Increased organic matter contents limited the depth of O2 penetration. The diffusion coefficients were higher proportionally to the decreased matrix potentials. Shrinkage of aggregates affected the diffusion coefficients and oxygenation, which is an important factor to be considered for bioremediation of sediments contaminated with organic substances (oil hydrocarbons, PAHs) during temporary disposal. Thus, the physical ripening of dredged sediments is a promising technique to enhance aerobic bioremediation of polluted sediments.
Rocznik
Strony
401--419
Opis fizyczny
Bibliogr. 26 poz.
Twórcy
autor
  • Politechnika Częstochowska, Instytut Inżynierii Środowiska, ul. Brzeźnicka 60a, 42-200 Częstochowa
autor
  • Wageningen University and Research Center, Sub-department of Environmental Technology Bomenweg 2, P.O. Box 8129,6700 EV Wageningen, Holandia
autor
  • Politechnika Częstochowska, Instytut Inżynierii Środowiska, ul. Brzeźnicka 60a, 42-200 Częstochowa
  • Wageningen University and Research Center, Sub-department of Environmental Technology Bomenweg 2, P.O. Box 8129,6700 EV Wageningen, Holandia
Bibliografia
  • [1] Bojakowska T., Gliwicz G., Sokołowska, Wyniki monitoringu gechemicznego osadów wodnych Polski w latach 1998-1999, PIOŚ, Warszawa 2000.
  • [2] Klimaszewska K., Występowanie i biodegradacja wielopierścieniowych węglowodorów aromatycznych w osadach dennych, Biotechnologia 1998, 1, 2.
  • [3] Popenda A., Malina G., Hazard from contaminated sediments in Poland, (w:) Pallei et al. (eds) Characterization of contaminated sediments, The 1st Int. Conference on Remediation of Contaminated Sediments, Venice, Italy, Battelle Press 2002, Sl-1,181-187.
  • [4] Rejman W., Zanieczyszczenie środowiska gruntowo-wodnego w Polsce przez WWA, Gospodarka Wodna 1998, 183-184.
  • [5] Vermeulen J., Grotenhuis T., Joziasse J., Rulkens W., Ripening of clayey dredged sediments during temporary upland disposal, A bioremediation technique, J. Soils and Sediments 2003, 3(1), 49-59.
  • [6] Vermeulen J., van Dijk S., Grotenhuis J.T.C., Joziasse J., Rulkens W.H., Accelerated physical ripening of PAH and oil contaminated sediment to distinguish critical steps in remediation, Proc. 7th Int. FZK/TNO Conference on Contaminated Soil, Leipzig, Germany 2000, 1184-1185.
  • [7] Konrad J.M., Ayad R., Dessication of a sensitive clay: field experimental observation, Canadian Geotechnical Journal 1997, 34, 929-942.
  • [8] Dexter A.R., Advances in characterization of soil structure, Soil and Tillage Research 1988, 11, 199-238.
  • [9] Kim D.J., Feyen J., Vereecken H., Prediction of dynamic hydraulic properties in a ripening soil, Geoderma 1993, 57, 231-246.
  • [10] Bronswijk J.J.B., Magnitude, modeling and significance of swelling and shrinkage processes in clay soils, PhD-Thesis, Wageningen Agricultural University, Wageningen, Holandia 1991.
  • [11] Harmsen J., Bioremediation of polluted sediments: a matter of time or effort, (w:) Phytoremediation, Wetlands, and Sediments, Proc. 6 th Int. In Situ and On Site Bioremediation Symposium, San Diego 2001, vol. 5, 279-287, Battelle Press, Columbus OH.
  • [12] Pons L.J., van der Molen W.H., Soil genesis under dewatering regimes during 1000 years of polder development, Soil Science 1973, 116, 228-235.
  • [13] Vermeulen J., van Dijk S.G., Grotenhuis J.T.C., Rulkens W.H., Quantification of physical properties of dredged sediments during physical ripening, Geoderma (przesłane do druku).
  • [14] Kim D.J., Characterization of swelling and shrinkage behaviour, hydraulic properties and modeling of water movement in physically ripening marine clay soil, PhD-thesis, K.U. Leuven, Belgium 1992.
  • [15] Malina G., Biowentylacja (SBV) strefy aeracji zanieczyszczonej substancjami ropopochodnymi, Monografie 69, Wyd. Politechniki Częstochowskiej, Częstochowa 1999.
  • [16] Malina G., Wielofazowa migracja zanieczyszczeń ropopochodnych w strefie aeracji i saturacji, Inż. i Ochr. Śród. 1998, 1, 85-96.
  • [17] Hillel D., Environmental soil physics, Academic Press, San Diego 1998.
  • [18] Blake G.R., Hartage K., Particle density, (w:) A. Klute (Ed.), Methods of soil analysis, Part 1, physical and mineralogical methods - agronomy, monograph no. 9, Am. Soc. Agron., Madison 1986, 377-382.
  • [19] Klute A., Water retention: laboratory methods, (w:) A. Klute (ed.), Methods of soil analysis, Part 1. Physical and mineralogical methods - agronomy, monograph no. 9, Am. Soc. Agron., Madison 1986, 635-662.
  • [20] Koorevaar P., Menelik G., Dirksen C., Elements of soil physics, Developments in Soil Science 13, Elsevier, Amsterdam 1983.
  • [21] Sextone A.J., Revsbech N.P., Parkin T.B., Tiedje J.M., Direct measurement of oxygen profiles and denitrification rates in soil aggregates, Soil Sei. Soc. Am. J. 1985, 49, 645-651.
  • [22] Crank J., The mathematics of diffusion, P. 11-12, Oxford Univ. Press, New York 1956, 189-191.
  • [23] Duursma E.K., Hoede C., Theoretical, experimental and field studies concerning molecular diffusion of radiostopes in sediments and suspended solid particles of the sea. Part A: Theories and mathematical calculations, Netherlands Journal of Sea Research 1967, 3(3), 423-457.
  • [24] Rolston D.E., Gas diffusivity, (w.) A. Klute (Ed.), Methods of soil analysis. Part 1. Physical and mineralogical methods - agronomy, monograph no. 9, Am. Soc. Agron., Madison 1986, 1089-1102.
  • [25] Taylor S.A., Oxygen diffusion in porous media as a measure of soil aeration, Soil Sei. Soc. Am. Proc. 1949, 14, 55-61.
  • [26] Zausig J., Stepniewski W., Horn R., Oxygen concentration and redox potential gradients in unsaturated model soil aggregates, Soil Sei. Soc. Am. J. 1993, 57, 908-916.
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-article-LOD3-0004-0044
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