Elektrogenerowana chemiluminescencja kompleksów lantanowców (III) na elektrodzie Al/Al_20_3

Staninski, K.; Lis, S.

Artykuł - szczegóły

Tytuł artykułu

Elektrogenerowana chemiluminescencja kompleksów lantanowców (III) na elektrodzie Al/Al_20_3

Autorzy

Staninski K. , Lis S.

Wybrane pełne teksty z tego czasopisma

Identyfikatory

Warianty tytułu

Electrogenerated chemiluminescence of lanthanide(III) complexes at Al/Al_20_3 electrode

Języki publikacji

Abstrakty

The aim of this review is to evaluate the electrochemiluminescence (ECL), both, as a method of light emission in certain types of lanthanide complexes by generating species capable of forming excited states, and for its potential use in analytical applications. The electrogenerated ECL in aqueous electrolyte solutions containing organic compounds having structural fragments such as carbonyl groups and conjugated double bonds and an oxide covered aluminum electrode doped with Ln(III) is reported. This specific electrogenerated luminescence can be achieved by producing highly oxidizing and reducing species as: hydrated electrons, hydroxyl and sulfate radicals. Such strong reactants efficiently excite the complexed lanthanide(III) ions [mainly Tb(III) and Dy(III)] by ligand to metal energy transfer, LMET. The experimental setup for ECL measurements (constructed in the Department of Rare Earths, Faculty of Chemistry, Adam Mickiewicz University) is introduced. The ECL generated with aluminium electrodes having chelated lanthanide(III) complexes-doped in their thin oxide coatings is studied following cathodic pulse polarization. The ECL mechanisms induced by hot-electrons leading to the production of light at or near the electrode surface by generating species capable of forming excited states of organic ligands are described.

Słowa kluczowe

electrochemiluminescence lanthanide complexes energy transfer

Wydawca

Polskie Towarzystwo Chemiczne

Czasopismo

Wiadomości Chemiczne

Rocznik

2007

Tom

[Z] 61, 3-4

Strony

279--296

Opis fizyczny

bibliogr. 51 poz., tab., wykr.

Twórcy

autor

Staninski K.

autor

Lis S.

Zakład Ziem Rzadkich, Wydział Chemii, Uniwersytet im. A. Mickiewicza, ul. Grunwaldzka 6, 60-780 Poznań

Bibliografia

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Typ dokumentu

Bibliografia

Identyfikator YADDA

bwmeta1.element.baztech-article-BUS5-0002-0021