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Activity concentration of plutonium in atmospheric precipitation

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Identyfikatory
Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
Activity concentrations of plutonium isotopes (238Pu, 239+240Pu) were determined in atmospheric precipitation samples collected in Kraków from August 2005 to December 2007. The volume of 29 samples varied in the range 14–269 dm3. The method of samples collection, preparation and radiochemical analysis proper for the separation of plutonium are indicated in brief. Monthly plutonium deposition a showed seasonal variation for 239+240Pu the first maximum was observed in August 2005 and amounted to about 2.65±0.31 mBq/m2, the second one in July 2006 – 0.371±0.063 mBq/m2 and the third one in April 2007 – 0.859±0.075 mBq/m2 and for 238Pu in September 2005 – 0.090±0.038 mBq/m2, July 2006 – 0.177±0.074 mBq/m2 and the third maximum in May 2007 – 0.333±0.028 mBq/m2. Similar behaviour of activity concentration of plutonium was also observed in other parts of the earth. Anomalously high deposition of 239+240Pu (2.65±0.31 mBq/m2) was found in August 2005. The 238Pu/239+240Pu activity ratios higher than the global fallout value ~ 0.55 (in Poland) suggested participation from different sources of plutonium.
Czasopismo
Rocznik
Strony
201--204
Opis fizyczny
Bibliogr. 12 poz., rys.
Twórcy
autor
  • The Henryk Niewodniczański Institute of Nuclear Physics, Polish Academy of Sciences, 152 Radzikowskiego Str., 31-342 Kraków, Poland, Tel./Fax: +48 12 662 8392, Renata.Kierepko@ifj.edu.pl
Bibliografia
  • 1. Hirose K, Kim CK, Kim CS, Chang BW, Igarashi Y, Aoyama M (2004) Wet and dry deposition patterns of plutonium in Daejeon, Korea. Sci Total Environ 332:243–252
  • 2. http://amsglossary.allenpress.com/glossary/
  • 3. Katsuragi Y, Hirose K, SugimuraY (1982) A study of plutonium fallout in Tokyo. Pap Met Geophys 33:85–93
  • 4. Kierepko R, Mietelski JW, Borowiec W, Tarasiewicz S, Błażej S, Kapała J (2009) Plutonium traces in atmospheric precipitation and in aerosols from Kraków and Białystok. Radiochim Acta 97;4/5:253–255
  • 5. LaRosa JJ, Cooper E, Ghods-Esphahani A et al. (1992) Radiochemical methods used by the IAEA’s Laboratories at Seibersdorf for the determination of 90Sr, 144Ce and Pu radionuclides in the environment samples collected for the International Chernobyl Project. J Environ Radioactiv 17:183–209
  • 6. Lehto J, Salminen S, Jaakkola T et al. (2006) Plutonium in the air in Kurchatov, Kazakhstan. Sci Total Environ 366:206–217
  • 7. Mietelski JW (2003) Nuclear spectrometry applied to studies of bioavailability of radionuclides from “fuel-like hot particles” in forest environment. (DSc Thesis). IFJ Report no. 1921/B. IFJ, Kraków (in Polish)
  • 8. Mitchell PI, Batlle J Vives i, Downes AB, Condren OM, Leon Vintro L, Sanchez-Cabeza JA (1995) Recent observation on the physico-chemical speciation of plutonium in the Irish Sea and the western Mediterranean. Appl Radiat Isot 46:1175–1190
  • 9. Montero MPR, Sanchez AM (2001) Activity of 239+240Pu and 238Pu in atmospheric deposits. Appl Radiat Isot 55:97–102
  • 10. Pietruszewski A, Bojanowski R (1990) Plutonium in air in Warsaw after Chernobyl accident. In: Proc of the Int Symp on Post-Chernobyl Environmental Radioactivity Studies in East European Countries, Kazimierz nad Wisłą, Poland, 17–19 September 1990. Lublin, pp 118–126
  • 11. Sill CW (1987) Precipitation of actinides as fluorides or hydroxides for high resolution alpha spectrometry. Nucl Chem Waste Mgmt 7:201–215
  • 12.UNSCEAR (1982) Report with annexes. United Nations sales publ. E.82.IX.8. New York
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-article-BUJ7-0014-0033
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