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Development of crystals based on cesium iodide for measurements of gamma radiation and alpha particles

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Identyfikatory
Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
During the past 50 years, scintillators have been among the most important nuclear radiation detectors. Inorganic scintillators are widely used in experimental nuclear physics, high energy physics, nuclear medicine, nuclear tomography, environmental studies and many other fields of use. Scintillation crystals based on cesium iodide (CsI) are matters of relatively low hygroscopy, high atomic number, easy handling and low cost, characteristics that favor their use as radiation detectors. In this work, the growth of pure CsI crystals, CsI:Br and CsI:Pb, using the Bridgman technique, is described. Ions of divalent lead (Pb2+) doped in the crystal structures are efficient emission centers and their application as scintillators is still the reason for intensive studies. Recently, promising results have been found for crystals of CsI doped by bromine (Br) for their use as radiation detectors. The concentration of the bromine doping element (Br) was studied in the range from 1.5 × 10–1 M to 10–2 M and the lead (Pb) in the range from 10–2 M to 5 × 10–4 M. To evaluate the scintillators developed, systematic measurements were carried out for luminescence emission and luminescence decay time for gamma radiation, Vickers microhardness assays, and analysis of crystals response to the gamma radiation, in the energy range from 350 keV to 1330 keV, and alpha particles from a 241Am source, with energy of 5.54 MeV. The obtained values for luminescence decay time for CsI:Br and CsI:Pb crystals, were from 13 to 19 ns.
Czasopismo
Rocznik
Strony
151--155
Opis fizyczny
Bibliogr. 10 poz., rys.
Twórcy
autor
autor
  • Instituto de Pesquisas Energéticas e Nucleares (IPEN/CNEN-SP), 2242 Professor Lineu Prestes Ave., Cidade Universitária – CEP: 05508-000, Săo Paulo – SP, Brazil, Tel.: +55 11 3133 9845, Fax: +55 11 3133 9765, macoper@ipen.br
Bibliografia
  • 1. Amsler C, Grogler D, Foffrain W et al. (2002) Temperature dependence of pure CsI: scintillation light yield and decay time. Nucl Instrum Methods Phys Res 480:494–500
  • 2. Astakhov MV, Belanov GS, Vasil’chenko VG, Rodin AO, Samoilenko VD, Solov’ev AS (2006) Properties of severely deformed CsI-based scintillators. Instrum Exp Tech 49:637–644
  • 3. Britvich GI, Britvich IG, Vasilchenko VG et al. (2001) New heavy scintillating materials for precise heterogeneous EM-calorimeters. Nucl Instrum Methods Phys Res 469:77–88
  • 4. Ishii M, Kobayashi M (1991) Single crystals for radiation detectors. Prog Cryst Growth Charact Mater 23:245–311
  • 5. Novotny R (2005) Inorganic scintillators – a basic material for instrumentation in physics. Nucl Instrum Methods Phys Res 537:1–5
  • 6. Schotanus P, Kamermans R, Dorenbos P (1990) Scintillation characteristics of pure and Tl-doped CsI crystals. IEEE Trans Nucl Sci 37:177–182
  • 7. Shannon RD (1976) Revised effective ionic radii and systematic studies of interatomic distances in halides and chalcogenides. Acta Crystallogr 32:751–767
  • 8. Shwartz B (2000) Eletromagnetic calorimeters based on CsI crystals. Nucl Instrum Methods Phys Res 453:205–209
  • 9. Sirdeshmukh DB, Swamy TK, Krishna PG, Subhadra KG (2003) Systematic hardness measurements on mixed and doped crystals of rubidium halides. Bull Mater Sci 26:261–265
  • 10. Zaslavsky BG, Vasetsky AM, Kudin AM et al. (2001) Scintillation and mechanical properties of CsI(Tl, Br) crystals pulled from melt. J Cryst Growth 212:751–754
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-article-BUJ7-0008-0015
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