Computer Simulation of Processes Connected with Electron Donor Fluorescence Quenching in Rigid Matrices. Effect of an External Electric Field

• Autorzy: Gutman M. , Hilczer M.
• Języki publikacji: EN

Abstrakty

EN

Computer simulation of photoexcited electron-donor D* fluorescence quenching in a rigid matrix has been performed. Three processes are assumed to occur: (1) the natural decay of D* excitation, (2) the electron transfer from D* to acceptor A, (3) migration of the excitation energy among D molecules. The effect of an external electric field F on process (2) has been included into considerations. Fluorescence decay curves calculated for various concentrations of D and the field-induced variation in the donor fluorescence intensity have been compared with respective experimental data and the results obtained from the approximate analytical calculations (hop ping model).

Słowa kluczowe

EN

photoinduced electron transfer; energy migration; simulation; hopping model; electric field effect

• Wydawca: Polskie Towarzystwo Chemiczne
• Czasopismo: Polish Journal of Chemistry
• Rocznik: 2008
• Tom: Vol. 82, nr 12
• Strony: 2245--2253
• Opis fizyczny: Bibliogr. 41 poz., rys.

Twórcy

autor

Gutman M.

autor

Hilczer M.

• Institute of Applied Radiation Chemistry, Technical University of Łódź, Wróblewskiego 15, 93-590 Łódź, Poland,

Bibliografia

• 1. Popovic Z.D., Khan M.I., Hor A.-M., Goodman J.L. and Graham I.F., J. Phys. Chem. B, 106, 8625 (2002).
• 2. Weitera M. and Bassler H., J. Lumin., 112, 363 (2005)
• 3. Kalmowski J   Stampor W. and Di Marco P.G., J. Chem. Phys., 96, 4136 (1992)
• 4. Pfefrer N.,Neher D.,Remmers M.,Poga C.,Hopmeier M. and Mahrt R., Chem.Phys.,227,167(1998).
• 5. Hertel D., Scherf U. and Bassler H., Adv. Mater., 10, 1119 (1998)
• 6. Jung J. Głowacki L and Ulański J., J. Chem. Phys., 110, 7000 (1999)
• 7. Pan J., Scherf U., Schreiber A. and Haarer D., J. Chem. Phys., 112, 4305 (2000).
• 8. Karki L., Vance F.W., Hupp J.T., LeCours S.M. and Therien M.J., J. Am. Chem. Soc., 120,2606 (1998).
• 9. Peteanu L.A., The Spectrum, 16, 12 (2003).
• lO. Hush N.S., Wong A.T., Bacskay G.B. and Reimers J.R., J. Am. Chem. Soc., 112, 4192 (1990)
• 11. Senindler R, Lupton J.M., Miiller J., Feldmann J. and Scherf U., Nature Materials, 5, 141 (2006)
• 12. Cupelli D., De Filpo G., Chidichimo G. and Nicoletta F.P., J. Appl Phys., 100, 024508 (2006)
• 13. Boxer S.G., in: Deisenhofer J. and Norris J.R., (Eds.), The Photosynthetic Reaction Center, vol.II Academic Press, San Diego, 1993, p. 179.
• 14. Lockhart D.J., Kirmaier Ch., Holten D. and. Boxer S.G., J. Phys. Chem., 94, 6987 (1990)
• 15. Tanaka S. and Marcus R.A., J. Phys. Chem. B, 101, 5031 (1997).
• 16. Lao K.,Franzen S., Steffen M.,Lambright D., Stanley R and Boxer S.G., Chem. Phys., 197,259(1995).
• 17. Ogrodnik A., Eberl U., Heckmann R., Kappl M., Freick R. and Michel-Beyerle M.E., J. Phys. Chem., 95,2036(1991).
• 18. Evans E.H. and Crofts A.R., Biochim. Biophys. Acta, 357, 89 (1974).
• 19. Ohta N., Koizumi M., Umeuchi S., Nishimura Y. and Yamazaki L., J. Phys. Chem., 100,16466 (1996).
• 20. Ohta N., Umeuchi S., Nishimura Y. and Yamazaki L., J. Phys. Chem. B, 102, 3784 (1998).
• 21. Ohta N., Bull.Chem. Soc. Jap., 75, 1637 (2002).
• 22. Kawabata H., Nishimura Y., Yamazaki L., Iwai K. and Ohta N., J. Phys. Chem. A, 105, 10261 (2001).
• 23. Ito T., Yamazaki I. and Ohta N., J. Phys. Chem. B, 106, 895 (2002).
• 24. Nakabayashi T., Wu B., Morikawa T., Limori T., Rubin M.B., Speiser S. and Ohta N., J. Photochem. Photobiol. A Chemistry, 178, 236 (2006).
• 25. Wahadoszamen Md., Nakabayashi T., Kang S., Imahori H. and Ohta N., J. Phys. Chem. B, 110, 20354 (2006).
• 26. Imori T., Yoshizawa T., Nakabayashi T. and Ohta N., Chem. Phys., 319, 101 (2005).
• 27. Ohta N., Kanada T., Yamazaki L, Ito S. and Suzuka I., J. Luminesc., 79, 177 (1998).
• 28. Kawabata H., Ohta N., Arakawa H., Ashida M., Kohtani S. and Nakagaki R., J. Chem. Phys., 114, 7723 (2001).
• 29. Yoshizawa T., Mizoguchi M., Limori T., Nakabayashi T. and Ohta N., Chem. Phys., 324, 26 (2006).
• 30. Hilczer M., Traytak S. and Tachiya M., J. Chem. Phys., 115, 11249 (2001).
• 31. Bandyopadhyay T., Ghosh S.H. and Tachiya M., Isr. J. Chem., 44, 119 (2004).
• 32. Hilczer M., Bandyopadhyay T. and Tachiya M., J. Photochem. Photobiol. A Chemistry, 166,33 (2004).
• 33. Burshtein A.I., J. Lumin., 34, 167 (1985).
• 34. Burshtein A.I., Sov. Phys. JETP, 35, 882 (1972).
• 35. Logan J. and Newton M.D., J. Chem. Phys., 78, 4086 (1983).
• 36. Newton M.D., Adv. Chem. Phys., 106, 303 (1999).
• 37. Förster Th., Ann. Physik, 2, 55 (1948).
• 38. Gutman M., Hilczer M. and Tachiya M., Nukleonika, 50, S39 (2005).
• 39. The LAPACK (Linear Algebra PACKage) project. http://www.netlib.org/lapack
• 40. Press W.H., Teukolsky S.A., Vetterling W.T. and Flannery B.P., Numerical recipes in C: The art of scientific computing. 2nd ed. Cambridge Univ. Press, 2002.
• 41. Galassi   et  al.,   GNU   Scientific  Library  Reference  Manual  (2nd  Ed.),   ISBN  0954161734, http ://www. gnu. org/software/gsl/