Recent Developments in Thermodynamics of Mixtures Containing 1,3-Dialkylimidazolium Alkylsulfate Ionic Liquids

Domańska, U.

Artykuł - szczegóły

Tytuł artykułu

Recent Developments in Thermodynamics of Mixtures Containing 1,3-Dialkylimidazolium Alkylsulfate Ionic Liquids

Autorzy

Domańska U.

Identyfikatory

Warianty tytułu

Języki publikacji

Abstrakty

Mixtures of ionic liquids, (ILs), with organic solvents exhibit a most interesting research area in thermodynamics. This report presents the ge eral discussion on the solid-liquid equilibria (SLE), high pressure solid-liquid equilibria, binary and ternary liquid-liquid equilibria (LLE), excess molar volumes, Vm E and ac tiv ity co ef fi cients at in finite dilution, gamma 1 Infinity of 1,3-dialkylimidazolium alkylsulfate ionic liquids, in alcohols and hydrocarbons. New sol u bil ity data of 1,3-dimethylimidazolium methylsulfate, [MMIM][CH3SO4] and 1-butyl-3-methylimidazolium octylsulfate, [BMIM][OcSO4] in methanol are presented. The solubilities have been measured by a dynamic method from 220 K to the melting point of the ionic liquid. Solubility of [MMIM][CH3SO4] and [BMIM][OcSO4] in methanol is very similar because of close melting temperatures of these ILs. The data were correlated by means of the NRTL and UNIQUAC equations utilizing parameters derived from the solid-liquid equilibrium. The melting point, the glass transition temperature and the enthalpy of fusion of [BMIM][OcSO4] were determined by the differential scanning calorimetry (DSC). The solubility of 1,3-dialkylimidazolium alkylsulfate ionic liquids in alcohols and hydrocarbons decreases with an in crease of the molecular weight of the solvent. Usually, with the exception of methanol and short chain alcohols, the mutual liquid-liquid equilibrium with the upper critical solution temperature (UCST) is observed in the liquid phase. This review presents a survey of the most recent data material including current developments and aspects of research activities needed in the future.

Słowa kluczowe

green chemistry ionic liquids solid-liquid equilibria liquid-liquid equilibria excess molar volumes activity coefficients at infinite dilution

Wydawca

Polskie Towarzystwo Chemiczne

Czasopismo

Polish Journal of Chemistry

Rocznik

2008

Tom

Vol. 82, nr 10

Strony

1923--1939

Opis fizyczny

Bibliogr. 77 poz., rys.

Twórcy

autor

Domańska U.

Physical Chemistry Division, Faculty of Chemistry, Warsaw University of Technology, Noakowskiego 3, 00-664 Warsaw, Poland phone: +48-22-6213115; Fax: +48-22-6282741, ula@ch.pw.edu.pl

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Typ dokumentu

Bibliografia

Identyfikator YADDA

bwmeta1.element.baztech-article-BUJ6-0024-0149