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Evaluation of the coal combustion input to the 226Ra ground-level air concentration in the Lodz city, Poland

Treść / Zawartość
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Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
The network of high volume aerosol samplers type ASS-500 in Poland, established mainly for monitoring radionuclides of artificial origin, offers also a unique opportunity for measuring natural radionuclide concentrations in ground-level air. Recounting of the closed (sealed) filters after a one month period, necessary for establishing radioactive equilibrium between 226Ra and 222Rn, as well as its short-lived decay products, remarkably improves the accuracy of 226Ra determination. The Currie's average detection and determination limits (with 10% relative accuracy) calculated for 226Ra for 160,000 s counting time and combined with the average filtered air volume of 60,000 m3 were 0.3 and 1.2 mi Bq/m3, respectively. The observed 226Ra concentrations in air in Lodz during the half year collection period, including parts of winter and summer seasons, were always above the detection limit and ranged from 0.76 to 2.75 mi Bq/m3. 226Ra, present in the ground level air mainly as a result of resuspension from the top layer of soil and fly ash emissions from coal burning, was used for rough estimation of the contribution of the coal combustion to the total suspended particulate matter. On the basis of available data for 226Ra content in the soil and fly ashes for the Lodz region of Poland, the calculated coal combustion input to the total air suspended particulate matter ranged from 8 to 39%.
Czasopismo
Rocznik
Strony
167--171
Opis fizyczny
Bibliogr. 17 poz., rys.
Twórcy
autor
  • Institute of Applied Radiation Chemistry, Technical University of Lodz, 36 Żwirki Str., 90-924 Lodz, Poland, Tel.: +48 42/ 631 31 95, Fax: +48 42/ 636 50 08
autor
  • Institute of Applied Radiation Chemistry, Technical University of Lodz, 36 Żwirki Str., 90-924 Lodz, Poland, Tel.: +48 42/ 631 31 95, Fax: +48 42/ 636 50 08
autor
  • Central Laboratory for Radiological Protection, 7 Konwaliowa Str., 03-194 Warsaw, Poland
autor
  • Faculty of Process and Environmental Engineering, Technical University of Lodz, 175 Wólczańska Str., 90-924 Lodz, Poland
Bibliografia
  • 1. Beck HL (1989) Radiation exposures due to the fossil fuel combustion. Radiat Phys Chem 34;2:285−293
  • 2. Bem H, Krzemińska M, Górecka H (2003) Calculation of the trace elements emissions on the basis of their concentration size distribution in fly ashes. Annals of the Polish Chemical Society (Lublin) 2;1:765−769
  • 3. Bem H, Wieczorkowski P, Budzanowski M (2002) Evaluation of technologically enhanced natural radiation near coal-fired power plants in the Lodz region of Poland. J Environ Radioact 61:191−201
  • 4. Bysiek M, Biernacka M, Lipiński P (2001) Radioactivity of ground level air in Poland in 1998−1999. Results from ASS500 stations network. Nukleonika 46;4:171−173
  • 5. Bysiek M, Biernacka M, Lipiński P (2004) Radioactivity of ground level air in Poland in 2002−2003. Results from aerosol sampling stations type ASS-500. In: Report of CLOR 2002−2003, research and operational activities. Central Laboratory for Radiological Protection, Warsaw, pp 52−58
  • 6. Currie LA (1968) Limits for qualitative detection and quantitative determination. Anal Chem 40;3:586−593
  • 7. Gäggeler HW (1995) Radioactivity in the atmosphere. Radiochim Acta 70/71:345−353
  • 8. Hamilton EI (1970) Concentration of uranium in air from contrasted natural environments. Health Phys 19;4:511−520
  • 9. Hötzl H, Winkler R (1987) Activity concentration of Ra-226, Ra-228, Pb-210, K-40 and Be-7 and their temporal variations in surface air. J Environ Radioact 5:445−458
  • 10. Kownacka L, Jaworowski Z, Zając B (1999) Measurement of concentration of 7 Be, 90Sr, 134,137Cs, 210Pb and 226Ra in the tropospheric and lower stratospheric air in 1997 and 1998. Report CLOR no. 138. Central Laboratory for Radiological Protection, Warsaw
  • 11. Lipiński P, Isajenko KA, Biernacka M, Żak A (2001) Integration of Polish monitoring networks (ASS-500 and PMS systems). Nukleonika 46;4:143−146
  • 12. Moore HE, Poet SE (1976) Background levels of radium226 in the lower troposphere. Atmos Environ 10;5:381−383
  • 13. Nowina-Konopka M (1993) Radiological hazard from coal fired power plants in Poland. Radiat Prot Dosim 46;3:171−180
  • 14. Papastefanou C (1996) Radiation impact from lignite burning due to 226Ra in Greek coal-fired power plants. Health Phys 70;2:187−191
  • 15. Report of the state of the environment in the Lodz region in 2002 (2003) Biblioteka Monitoringu Srodowiska, Lodz
  • 16. UNSCEAR (2000) Exposures from natural radiation sources. Vol. I. Report to the General Assembly with Scientific Annexes. United Nations, New York
  • 17. Yunoki E, Kataoka T, Michihiro K, Sugiyama H, Shimizu M, Mori T (1995) Background levels of 238U and 226Ra in atmospheric aerosols. J Radioanal Nucl Chem 189;1:157−164
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-article-BUJ6-0005-0076
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