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Radionuclides of iron (55Fe), nickel (63Ni),polonium (210Po), uranium (234U, 235U, 238U) and plutonium (238Pu, 239+240Pu, 241Pu) in Poland and Baltic Sea environment

Treść / Zawartość
Identyfikatory
Warianty tytułu
Konferencja
Proceedings of the IV All-Polish Conference on Radiochemistry and Nuclear Chemistry9-11 May 2005, Kraków-Przegorzały, Poland
Języki publikacji
EN
Abstrakty
EN
The paper presents the results of determination of natural [polonium (210Po), uranium (234U, 235U, 238U)] and artificial radionuclides [iron (55Fe), nickel (63Ni), and plutonium (238Pu, 239+240Pu, 241Pu)] in Poland and the southern Baltic Sea ecosystem as well as the recognition of their accumulation process in the trophic chain. All presented results is a summary of long lasting studies realized by the present authors. Results of this study indicated that the principal sources of 55Fe and 63Ni in the Baltic Sea environment is the release from Swedish nuclear power plants. Investigation on the polonium 210Po and plutonium 238Pu, 239+240Pu and 241Pu concentration in Baltic and land biota revealed that these radionuclides are strongly accumulated by some species. Moreover, it was found that fish, mushrooms, cigarettes constitutes important sources of 210Po for people. The Baltic Sea algae, benthic animals and fish concentrate uranium only to a small degree. In Baltic sediments, the concentration of uranium increases with core depth and it is connected with the diffusion of 234U, 235U and 238U from sediments. The values of 234U/238U activity ratio in the sediments indicated that the reduction process of U(VI) to U(IV) and the removing of autogenic uranium from seawater to sediments in the Gdańsk Deep constitutes a small part only.
Słowa kluczowe
Czasopismo
Rocznik
Strony
45--51
Opis fizyczny
Bibliogr. 33 poz., rys.
Twórcy
autor
autor
  • Chair of Analytical Chemistry, Faculty of Chemistry, University of Gdańsk, 18/19 Sobieskiego Str., 80-952 Gdańsk, Poland, Tel.: +48 58 345 03 38, Fax: +48 58 345 04 72
Bibliografia
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  • 4. Danielsen EF (1981) Trajectories of the Mount St. Helen plume. Science 221:891−921
  • 5. Hardy EP, Krey PW, Volchok HL (1973) Global inventory and distribution of fallout plutonium. Nature 241:444−445
  • 6. Holm E, Oregoni B, Vas D, Pettersson H, Rioseco J,Nilsson U (1990) Nickel-63: radiochemical separation and measurement with an ion implanted silicon detector. J Radioanal Nucl Chem 138:111−116
  • 7. Holm E, Roos P, Skwarzec B (1992) Radiochemical studies of fallout 63Ni. Appl Radiat Isot 43:371−376
  • 8. Jaworowski Z (1969) Radioactive lead in the environment and in the human body. At Energ Rev 7:3−45
  • 9. Jaworowski Z, Bilkiewicz J, Kownacka L, Włodek S (1972) Artificial sources of natural radionuclides in environment. In: Proc of the 2nd Int Conf: The natural radiation environment, 5 August 1972, Houston, Texas.CONF-720805-P2. Vol. II, pp 809−818
  • 10. Ku TL, Knauss KG, Mathieu GG (1977) Uranium in open ocean: concentration and isotopic composition. Deep Sea Research 24:1005−1017
  • 11. Lambert G, Buisson A, Sanak J, Ardonin B (1979)Modification of the atmospheric polonium-210 to lead-210 ratio by volcanic emissions. Journal Geophysics Research 84:6980−6986
  • 12. Langmuir D (1978) Uranium solution-mineral equilibria at low temperature with applications to sedimentary ore deposits. Geochim Cosmochim Acta 42:547−569
  • 13. Martin JM, Nijampurkar V, Salvadori F (1978) Uranium and thorium isotope behavior in estuarine system. In:Goldberg ED (ed.) Biochemistry of estuarine sediments.UNESCO, pp 111−127
  • 14. McDonald P, Fowler SW, Heyrand MW, Baxter MS (1986) Polonium-210 in mussels and its implications for environmental alpha-autoradiography. J Environ adioact 3:293−303
  • 15. Moore HE, Martell EA, Poet SE (1976) Sources of polonium-210 in the atmosphere. Environ Sci Technol 10:586−591
  • 16. Pietrzak-Flis Z, Chrzanowska S, Dembińska S (1997)Intake of 226Ra, 210Pb and 210Po with food in Poland. Sci Total Environ 203:157−165
  • 17. Rangarajan C, Gopalakrishnam S, Eapen CD (1976)Global variation of 210Po in surface air and precipitation.In: Hardy EP (ed.) Health and safety laboratory environmental quarterly. HASL-298. USERDA, New York, pp 163−182
  • 18. Skwarzec B (1995) Polonium, uranium and plutonium in ecosystem of the southern Baltic Sea. Rozprawy i Monografie no. 6. Instytut Oceanologii PAN, Sopot in Polish)
  • 19. Skwarzec B (1997) Polonium, uranium and plutonium in the southern Baltic Sea. Ambio 26;2:113−117
  • 20. Skwarzec B (2002) Environmental radiochemistry and radiological protection. Wydawnictwo DJ, Gdańsk (in Polish)
  • 21. Skwarzec B, Boryło A, Strumińska DI (2004) Activity disequilibrium between 234U and 238U isotopes in southern Baltic. Water, Air Soil Pollut 159:165−173
  • 22. Skwarzec B, Holm E, Roos P, Pempkowiak J (1994)Nickel-63 in Baltic fish and sediments. Appl Radiat Isot 54:609−611
  • 23. Skwarzec B, Holm E, Strumińska DI (2001)Radioanalytical determination of 55Fe and 63Ni in the environmental samples. Chem Anal (Warsaw) 46:23−30
  • 24. Skwarzec B, Jakusik A (2003) 210Po bioaccumulation by mushrooms from Poland. J Environ Monit 5:791−794
  • 25. Skwarzec B, Strumińska DI, Boryło A (2001) The radionuclides 234U, 238U and 210Po in drinking water in Gdańsk agglomeration (Poland). J Radioanal Nucl Chem 250;2:315−318
  • 26. Skwarzec B, Strumińska DI, Boryło A (2003) Radionuclides of 210Po, 234U and 238U in drinking bottled water in Poland. J Radioanal Nucl Chem 256:361−364
  • 27. Skwarzec B, Strumińska DI, Boryło A, Falandysz J (2004) Intake of radionuclides of 234U and 238U with beer in Poland. J Radioanal Nucl Chem 261;3:661−663
  • 28. Skwarzec B, Strumińska DI, Boryło A, Ulatowski J (2001) Polonium 210Po in cigarettes produced in Poland. J Environ Sci Health A 36:23−30
  • 29. Skwarzec B, Strumińska DI, Prucnal M (2003) Estimates of 239+240Pu inventories in Gdańsk Bay and Gdańsk Basin.J Environ Radioact 70:237−252
  • 30. Skwarzec B, Strumińska DI, Ulatowski J, Gołębiowski M (2001) Determination and distribution of polonium 210Po in tobacco plant from Poland. J Radioanal Nucl Chem 250;2:319−322
  • 31. Skwarzec B, Ulatowski J, Strumińska DI, Boryło A (2001)Inhalation of 210Po and 210Pb from cigarette smoking in Poland. J Environ Radiact 57:221−230
  • 32. Strumińska DI, Skwarzec B (2006) Plutonium 241Pu concentrations in southern Baltic Sea ecosystem. J Radioanal Nucl Chem 268;1:59−63
  • 33. Zatoński W (1996) Development of health situation in Poland after 1988 year. Centrum Onkologii, Instytut im.M. Skłodowskiej-Curie, Zakład Epidemiologii i Prewencji Nowotworów, Warsaw (in Polish)
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-article-BUJ6-0004-0030
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