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Self-absorption correction in gamma-ray spectrometry of environmental samples - an overview of methods and correction values obtained for the selected geometries

Autorzy
Treść / Zawartość
Identyfikatory
Warianty tytułu
Konferencja
Proceedings of the IV All-Polish Conference on Radiochemistry and Nuclear Chemistry9-11 May 2005, Kraków-Przegorzały, Poland
Języki publikacji
EN
Abstrakty
EN
Of major concern are the self-absorption correction factors Cs in precise gamma-ray spectrometry of environmental samples. The overview of Cs determination methods (experimental, Monte Carlo calculations, analytical function application) is presented. Among several available methods, the author chose the one proposed by Debertin where the uncertainty level of Cs correction factor is 1÷2%. The point-like detector model is assumed whilst its efficiency is taken to be proportional to the weighted sum (integral) of the number of photons coming from sample volume elements. Computer program was developed to support the computation of Cs by the Debertin's method for samples in cylindrical geometries and Marinelli beakers. The input data are sample dimensions, density and the mass attenuation coefficient. The Cs uncertainty due to an arbitrarily chosen position of a point-like detector would not exceed 1% for the considered photon energies and the sample density range. Utilising this computer program, the relationships Cs(E,ń) were obtained for the applied geometries and a SiO2 matrix to support routine measurements. The SiO2 matrix is widely encountered in environmental spectrometry. This relationship was derived by fitting the computed data with the function Cs(E,ń) in the form proposed by Bolivar. It was shown that while handling this function to samples with the H2O matrix, the error involved in estimations would not exceed 3%.
Czasopismo
Rocznik
Strony
21--25
Opis fizyczny
Bibliogr. 21 poz., rys.
Twórcy
  • Faculty of Physics and Applied Computer Science, AGH University of Science and Technology, 30 A. Mickiewicza Av., 30-059 Kraków, Poland, Tel.: +48 12 617 29 72, Fax: +48 12 634 00 10, jodlowski@novell.ftj.agh.edu.pl
Bibliografia
  • 1. Bolivar JP, García-León M, Garcia-Tenorio R (1997) On self-attenuation corrections in gamma-ray spectrometry. Appl Radiat Isot 48:1125−1126
  • 2. Bolivar JP, García-Tenorio R, García-León M (1996) A method for the determination of counting efficiencies in gamma-spectrometric measurements with HPGe detectors.Nucl Instrum Methods Phys Res A 382:495−502
  • 3. Boshkova T, Minev L (2001) Corrections for self-attenuation in gamma-ray spectroscopy of bulk samples. Appl Radiat Isot 54:777−783
  • 4. Bostock IJ, Taulbee TD (1999) Automated efficiency calibration of HPGe spectrometers for in-vitro soil samples. Nucl Instrum Methods Phys Res A 422:812−816
  • 5. Cutshall N, Larsen IL, Olsen CR (1983) Direct analysis of Pb-210 in sediment samples: a self-absorption corrections. Nucl Instrum Methods Phys Res 206:309−312
  • 6. Debertin K, Helmer RG (1988) Gamma- and X-ray spectrometry with semiconductor detectors. North-Holland Publ, Amsterdam
  • 7. Debertin K, Ren J (1989) Measurement of activity ofr radioactive samples in Marinelli beakers. Nucl Instrum Methods Phys Res A 278:541−549
  • 8. Dryák P, Kováø P, Pilchová L, Šurán J (1989) Corrections for Marinelli geometry. J Radioanal Nucl Chem 135:281−292
  • 9. El-Daoushy F, Garcia-Tenorio R (1995) Photon (20−60keV) self-absorption in small aquatic deposits. Nucl Instrum Methods Phys Res A 359:622−624
  • 10. Haase G, Tait D, Wiechen A (1993) Application of new Monte Carlo method for determination of summation and self-attenuation corrections in gamma spectrometry. Nucl Instrum Methods Phys Res A 336:206−214
  • 11. Hernández F, El-Daoushy F (2002) Semi-empirical method for self-absorption correction of photons with energies as low as 10 keV in environmental samples. Nucl Instrum Methods Phys Res A 484:625−641
  • 12. Joshi SR (1989) Determination of Am-241 in sediments by direct counting of low-energy photons. Int J Radiat Applic Instrum A 40:691−699
  • 13. Korun M (2000) Calculation of self-attenuation factors in gamma-ray spectrometry for samples of arbitrary shape. J Radioanal Nucl Chem 244:685−689
  • 14. Lefèvre O, Bouisset P, Germain P, Barker E, Kerlau G,Cagnat X (2003) Self-absorption correction factor applied to I-129 measurement by direct gamma-X spectrometry for Fucus serratus samples. Nucl Instrum Methods Phys Res A 506:173−185
  • 15. Park TS, Jeon WJ (1995) Measurement of radioactive samples in Marinelli beakers by gamma-ray spectrometry.J Radioanal Nucl Chem 193:133−144
  • 16. Pérez-Moreno JP, San Miguel EG, Bolvar JP, Aguado JL (2002) A comprehensive calibration method of Ge detectors for low-level gamma-spectrometry measurements.Nucl Instrum Methods Phys Res A 491:152−162
  • 17. Ramos-Lerate I, Barrera M, Ligero RA, Casas-Ruiz M (1998) A new method for gamma-efficiency calibration of voluminal samples in cylindrical geometry. J Environ Radioact 38:47−57
  • 18. Sanchez F, Navarro E, Ferrero JL et al. (1991) A Monte Carlo based method of including gamma self-absorption for the analysis of environmental samples. Nucl Instrum Methods Phys Res B 61:535−540
  • 19. Sima O (1992) Photon attenuation for samples in Marinelli beaker geometry: an analytical computation.Health Phys 62:445−449
  • 20. Sima O, Dovlete C (1997) Matrix effects in the activity measurement of environmental samples – implementation of specific corrections in gamma-ray spectrometry analysis program. Appl Radiat Isot 48:59−69
  • 21.Vargas MJ, Timón AF, Diaz NC, Sánchez DP (2002)Monte Carlo simulation of the self-absorption corrections for natural samples in gamma-ray spectrometry. Appl Radiat Isot 57:893−898
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-article-BUJ6-0004-0026
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