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Dynamics of Molecular Hydrogen Exchange in Hydrogen-Bonded Systems

Identyfikatory
Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
The kinetics of hydrogen exchange in molecular systems with H-bonds studied by kinetic IR spectroscopy and low-temperatureNMRspectroscopy methods is critically reviewed. The experimental rate constants and activation energies obtained so far for molecules capable of forming H-bonds as both proton donors and proton acceptors are collected and analyzed from the point of view of the influence of H-bond formation ability of the molecules- partners. The evidence available testifies to a molecular mechanism of the H-exchange reactions in inert solvents and in the gas phase via the formation of cyclic, mostly bimolecular, intermediates. The different mechanisms of the molecular H-exchange process in inert media are discussed and the possible paths of experimental elucidation of reaction mechanism are offered.
Rocznik
Strony
1177--1190
Opis fizyczny
Bibliogr. 57 poz., rys.
Twórcy
autor
  • Institute of Physics, St. Petersburg State University,Ulianovskaya 1, Petrodvorets, St. Petersburg, 198504, Russia
  • Institute of Physics, St. Petersburg State University,Ulianovskaya 1, Petrodvorets, St. Petersburg, 198504, Russia
Bibliografia
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Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-article-BUJ1-0023-0032
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