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Synthesis and characteristics of titanium silicalite TS-1, Ti-Beta and Ti-MWW catalysts

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Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
The synthesis methods of the following titanium-silicalite catalysts: TS-1, Ti-Beta and Ti-MWW were presented. The results of the analyses of the catalysts by XRD, SEM and IR, UV-vis methods were also shown. A brief description of the catalytic performances of these catalysts in the oxidation process of olefins, alkenes, alcohols and aromatic compounds was presented.
Słowa kluczowe
Rocznik
Strony
64--71
Opis fizyczny
Bibliogr. 33 poz., rys.
Twórcy
autor
autor
  • Institute of Organic Chemical Technology, West Pomeranian University of Technology, ul. Pułaskiego 10, 70-322 Szczecin, agnieszka.wroblewska@ps.pl
Bibliografia
  • 1. Sheldon, R. (1996). Selective catalytic synthesis of fine chemicals: opportunities and trends. J. Mol. Catal. A: Chemical 107(1 - 3), 75 - 83. DOI: 10.1016/1381-1169(95)00229-4.
  • 2. Sheldon, R., Arends, I. & Dijksman, A. (2000). New developments in catalytic alcohol oxidations for fine chemicals synthesis. Catal. Today 57(1 - 3), 157 - 166. DOI: 10,1016/S0920-5861(99)00317-X.
  • 3. Blaser, H. & Studer, M. (1999). The role of catalysis for the clean production of fine chemicals. Appl. Catal.189, 191 - 204. PII: S0926-860X(99)00276-8.
  • 4. Mills, P. & Chaudhari, R. (1997). Multiphase catalytic reactor engineering and design for pharmaceuticals. Cat. Today 37(4), 367 - 404. DOI: 10,1016/ S0920-5861(97)00028-X.
  • 5. Blaser, H. (2000). Heterogeneous catalysis for fine chemicals production. Cat. Today 60(1 - 3), 161 - 165. DOI: 10,1016/S0920-5861(00)00332-1.
  • 6. Millini, R., Massaro, E., Perego, G. & Bellussi, G. (1992). Framework composition of titanium silicalite 1. J. Catal. 137(2), 497 - 503.
  • 7. Wróblewska, A. & Milchert, E. (2002). Synthesis of titanium-silicalite catalysts. Pol. J. App.Chem. 46(3 - 4), 151 - 175.
  • 8. Khouw, C., Dartt, C., Labinger, J. & Davis, M. (1994). Studies on the catalytic oxidation of alkanes and alkenes by titanium silicalites. J. Catal. 149, 195 - 205.
  • 9. Notari, B. (1987). Innovation in Zeolite Material Scienece. Stud. Surf. Sci. Catal. 37, 413.
  • 10. Hauptman, S. (1985). Organische Chemie. Leibziger: VEB deutscher Verlag für Grundstoffindustrie.
  • 11. Koch, M., Wark, M. & Schulz-Ekloff, G. (1999). Report to Bayer AG. Germany: University of Bremen.
  • 12. Kooyman, P. (1993). A Study On Titanium-Silicalite-1 And Related Systems. Delft: Technische Universiteit.
  • 13. Notari, B. (1988). Innovation In Zeolite Materials Science. 37, 413.
  • 14. Clerici, M. (1991). Oxidation of saturated hydrocarbons with hydrogen peroxide, catalyzed by titanium silicalite. Appl. Catal. 68(1 - 2), 249 - 261.
  • 15. Tatsumi, T., Nakamura, M., Negeshi, S. & Tominaga, H (1990). Shape-selective oxidation of alkenes with hydrogen peroxide catalyzed by titanosilicalite. J. Chem. Soc., Chem. Commun. 476 - 477.
  • 16. Huybrechts, D., Bruyker, L. & Jacobs, P. (1990). Oxyfunctionalization of alkenes with hydrogen peroxide on titanium silicalite. Nature 345, 240.
  • 17. Romano, U., Esposito, A., Maspero, F., Neri, F. & Clerici, M. (1990). New Developments In Selective Oxidation. Stud. Surf. Sci. Catal. 55, 33.
  • 18. Clerici, M. & Ingllina, P. (1993). Epoxidation of lower olefins with hydrogen peroxide and titanium silicalite. J. Catal. 140, 71.
  • 19. Goutier, S. & Tuel, A. (1994). Oxidation of aniline over TS-1, the titanium substituted silicalite -1. Appl. Catal. A 118(2), 173 - 186.
  • 20. Van der Waal J. (1998). Prof. Thesis Univ. Delft, The Niderlandy.
  • 21. Van der Waal, J., Rigutto, M. & Van Bekkum, H. (1997). Zeolite titanium beta as a selective catalyst in the epoxidation of bulky alkenes. Appl. Catal. A 167(2), 331 - 342. DOI: 10.1016/S0926-860X(97)00323-2.
  • 22. Corey, E. & Schmidt, G. (1979). Useful procedures for the oxidation of alcohols involving pyridinium dichromate in aprotic media. Tetrahedron Lett. 5, 399 - 402.
  • 23. Wu, P., Tatsumi, T., Komatsu, T. & Yashima, T. (2001). A novel titano-silicalite with MWW structure: I. Hydrothermal synthesis, elimination of extraframework titanium, and characterizations. J. Phys. Chem. B 105(15), 2897 - 2905. DOI: 10.1021/jp002816S.
  • 24. Degnan, T. (2003). The implications of the fundamentals of shape selectivity for the development of catalysts for the petroleum and petrochemical industries. J. Catal. 216(1-2), 32 - 46. DOI: 10.1016/S0021-9517(02)00105-7.
  • 25. Fan, W., Wu, P., Namba, S. & Tatsumi, T. (2006). Synthesis and catalytic properties of a new titanosilicate molecular sieve with the structure analogous to MWW-type lamellar precursor. J. Catal. 243(1), 183 - 191. DOI: 10.1016/jat.2006.07.003.
  • 26. Wu, P., Tatsumi, T., Komatu, T. & Yashima, T. (2002). A novel titanosilicate with MWW structure: II. Catalytic properties In The selective oxidation of alkenes. J. Catal. 202(2), 245 - 255. DOI: 10.1006/jat.2001.3278.
  • 27. Wu, P. & Tatsumi, T. (2002). Preparation of B-free Ti-MWW through reversible structural conversion. Chem. Commun. 1026 - 1027. DOI: 10.1039/b201170k.
  • 28. Wu, P., Liu, Y., He, M. & Tatsumi, T. (2004). A novel titanosilicalite with MWW structure. Catalytic properties In selective epoxidation of diallyl ether with hydrogen peroxide. J. Catal. 228(1), 183 - 191. DOI: 10.1016/jat.2004.09.001.
  • 29. Song, F., Liu, Y., Wu, H. & He, M. (2006). A novel titanosilicate with MWW structure: Highly effective liquidphase ammoximation of cycloheksanone. J. Catal. 237(2), 359 - 367. DOI: 10.1016/j.jcat.2005.11.018.
  • 30. Vayssilov, G. (1997). Structural and physicochemical features of titanium siliclites. Catal. Rev. 39, 209.
  • 31. Saxton, R. (1999). Crystalline microporous titanium silicalites. Top. Catal. 9(1 - 2), 43 - 57. DOI: 10.1023/A:1019102320274.
  • 32. Camblor, M., Corma, A., Martinez, A. & Perez-Pariente, J. (1992). Synthesis of titaniumsilicoaluminate isomorphous to zeolite beta and its application as a catalyst for the selective oxidation of large organic molecules. J. Chem. Soc. 8, 589 - 590.
  • 33. Wu, P., Tatsumi, T., Komatsu, T. & Yashima, T. (2001). A novel titanosilicate with MWW structure. I. Hydrothermal synthesis, elimination of extraframework titanium, and characterizations. J.Phys. Chem. B 105(15), 2897 - 2905. DOI: 10.1021/jp002816s.
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-article-BPS2-0050-0072
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