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The homogeneous stirred reactor designed for kinetic studies of the combustion of hydrocarbons with intensive internal recirculation in high temperature combustion chamber is described. The originality of our reactor lies in its construction which allows to intensively mix fuel and flue gases, measure gas temperature as well as obtain samples which can be used to investigate diffusion flames. The cylindrical construction enables to use the reactor in laboratory cylindrical electrically heated ovens. The CFD analysis of the reactors, the mixing parameters (turbulent Peclet number and mixing level) and the volume average temperature in the reactors were elaborated on the basis of the typical dimensions of classical reactors to kinetics research as well as the own reactor design. The results of the analysis allow to reveal advantages of our construction.
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Czasopismo
Rocznik
Tom
Strony
397--410
Opis fizyczny
Bibliogr. 16 poz., rys., tab.
Bibliografia
- 1. Dagaut P., Cathonnet M., Rouan J.P., Foulatier R., Quilgars A., Boettner J.C., Gaillard F., James H., 1986. A jetstirred reactor for kinetic studies of homogeneous gas-phase reactions at pressures up to ten atmospheres (1 MPa). J. Phys. E: Sci. Instrum., 19, 207-209. DOI: 10.1088/0022-3735/19/3/009.
- 2. FLUENT 6.3 User’s Guide. Lebanon NH: Fluent Inc., 2006.
- 3. Gil I, Tomeczek J., 2008 Investigation of combustion mechanism in CH4/CO2/O2/N2 system in the high temperature furnace. Thermodynamics in the science and economy. Oficyna Wydawnicza Politechniki Wrocławskiej, Wrocław (in Polish).
- 4. Gil I., 2009. Influence flue gases recirculation on the methane combustion in the high temperature furnaces. Conferences in VSB Technical University of Ostrava. Ostrava, Czech Republic.
- 5. Gil I., 2009. Modeling methane combustion in the high temperature furnaces with recirculation flue gases. International Conference on Optimization using Exergy Based Methods and Computation Fluid Dynamics. Berlin, Germany.
- 6. Gil I., 2010. Investigation of gaseous hydrocarbon combustion mechanism in air diluted by combustion products in the high temperature furnace. PhD thesis. Silesian University of Technology, Katowice.
- 7. Hill Ch.G. Jr., 1999. An introduction to chemical engineering kinetics & reaction design. John Willey and Sons, Inc., New York.
- 8. Joannon E., Cavaliere A., Faravellic T., Ranzic E., Sabiab P., Tregrossia A., 2005. Analysis of process parameters for steady operations in methane mild combustion technology, Proc. Combust. Inst., 30, 2605-2612. DOI: 10.1016/j.proci.2004.08.190.
- 9. Launder B.E., Spalding, D.B., 1972. Mathematical models of turbulences. Academic Press, New York. DOI: 10.1002/zamm.19730530619.
- 10. Levenspiel O., 1977. Chemical Reaction Engineering. 3rd edition, John Willey and Sons, Inc., New York.
- 11. Longwell J.P., Weiss M.A., 1955. High temperature reaction rates in hydrocarbon combustion. Ind. Eng. Chem., 47, 1634-1639. DOI: 10.1021/ie50548a049.
- 12. Malte P.C., Pratt D.T., 1975. Measurement of atomic oxygen and nitrogen oxides in jet-stirred combustion. Fifteenth Symposium (International) on Combustion, 15, 1061-1070. DOI:10.1016/S0082-0784(75)80371-7.
- 13. Miller J.A., Bowman C.T., 1989. Mechanism and modeling of nitrogen chemistry in combustion. Prog. Energy and Comb. Sci., 15, 287-338. DOI: 10.1016/0360-1285(89)90017-8.
- 14. NIST-JANAF thermochemical tables, 1998. 4th edition, Chase M.W., Jr. American Chemical Society, American Institute of Physics for the National Institute of Standards and Technology. Washington, D.C.
- 15. Sazhin S.S., Sazhina E.M., Faltzi-Saravelou O., Wild P., 1996. The P-1 model for thermal radiation transfer: advantages and limitations. Fuel, 75, 289-294. DOI: 10.1016/0016-2361(95)00269-3.
- 16. Siegel R., Howell R., 1992. Thermal radiation heat transfer. Hemisphere Publishing Corporation, Washington DC.
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-article-BPK6-0026-0007