The effect of substrate roughness on the surface structure of TiO2, SiO2, and doped thin films prepared by the sol-gel method

• Autorzy: Krzak-Roś J. , Filipiak J. , Pezowicz C. , Baszczuk A. , Miller M. , Kowalski M. , Będziński R.
• Języki publikacji: EN

Abstrakty

EN

Pure and calcium-doped silica and titanium dioxide thin films were prepared by the sol-gel method. Two different metallic substrates, i.e. stainless steel (316L) and titanium alloy (Ti6Al4V), were used for thin film deposition. Physicochemical properties and roughness of the thin films derived were investigated using the Raman spectroscopy, X-ray diffraction analysis, scanning electron microscopy and Taylor-Hobson's surface analyser. It is suggested that the synthesized coatings display physicochemical and surface properties suitable for materials used for implant.

Słowa kluczowe

EN

thin films; coatings; sol-gel method; roughness

PL

cienkie warstwy; powłoki; metoda zol-żel; chropowatość

• Wydawca: Oficyna Wydawnicza Politechniki Wrocławskiej
• Czasopismo: Acta of Bioengineering and Biomechanics
• Rocznik: 2009
• Tom: Vol. 11, nr 2
• Strony: 21--29
• Opis fizyczny: Bibliogr. 25 poz., rys., tab.

Twórcy

autor

Krzak-Roś J.

autor

Filipiak J.

autor

Pezowicz C.

autor

Baszczuk A.

autor

Miller M.

autor

Kowalski M.

autor

Będziński R.

• Institute of Materials Science and Applied Mechanics, Wrocław University of Technology

Bibliografia

• [1] BOWERS K.T., KELLER J.C., RANDOLPH B.A., WICK D.G., MICHAELS C.M., Optimization of surface micromorphology for enhanced osteoblast responses in vitro, Int. J. Oral Maxillofac. Implants, 1992, 7(3), 302–310.
• [2] BRUNETTE D.M., The effects of implant surface topography on the behaviour of cells, Int. J. Oral Maxillofac. Implants, 1988, 3, 231–246.
• [3] ANSELME K., BIGERELLE M., NOEL B., DUFRESNE E., JUDAS D., IOST A., HARDOUIN P., Qualitative and quantitative study of human osteoblast adhesion on materials with various surface roughnesses, J. Biomed. Mater. Res., 2000, 49, 155–66.
• [4] KONONEN M., HORNIA M., KIVILAHTI J., HAUTANIEMI J., THESLEFF I., Effect of surface processing on the attachment, orientation, and proliferation of human gingival fibroblasts on titanium, J. Biomed. Mater. Res., 1992, 26, 1325–1341.
• [5] MURRAY D.W., RAE T., RUSHTON N., The influence of the surface energy and roughness of implants on bone resorption, JBJS (Br), 1989, 71-B (4), 632–637.
• [6] SATSANGI A., SATSANGI N., GLOVER R., SATSANGI R.K, ONG J.L., Osteoblast response to phospholipid modified titanium surface, Biomaterials, 2003, 24, 4585–4589.
• [7] GŁUSZEK J., Tlenkowe powłoki ochronne otrzymywane metodą sol–gel, Wrocław, 1998.
• [8] KRZAK-ROŚ J., GRYGIER D., BASZCZUK A., BĘDZIŃSKI R., Mechanical and physico-chemical properties of titanium dioxide thin films, Engineering of Biomaterials, 2007, X(67-68), 35–37.
• [9] OCHSENBEIN A., CHAI F., WINTER S., TRAISNEL M., BREME J., HILDEBRAND H.F., Osteoblast responses to different oxide coatings produced by the sol–gel process on titanium substrates, Acta Biomaterialia, 2008, 4, 1506–1517.
• [10] GRYGIER D., DUDZIŃSKI W., WIKTORCZYK T., HAIMANN K., Effect of silica precursors-type on mechanical properties of sol–gel coatings, Acta Bioeng. Biomech., 2008, 10(1), 27–35.
• [11] ZHU X., CHEN J., SCHEIDELER L., REICHL R., GEIS-GERSTORFER J., Effects of topography and composition of titanium surface oxides on osteoblast responses, Biomaterials, 2004, 25, 4087–4103.
• [12] FALARAS P., XAGAS A.P., Roughness and fractality of nanostructured TiO2 films prepared via sol–gel techniques, J. Mat. Science, 2002, 37, 3855–3860.
• [13] TING C.C., CHEN S.Y., Influence of ligand groups in Ti precursors on phase transformation and microstructural evolution of TiO2 thin films prepared by the wet chemical process, J. Mater. Res., 2001, 16 (6), 1712–1719.
• [14] PN-ISO 4288: 1997 + Ap1: 1999, Wymagania geometryczne wyrobów. Struktura geometryczna powierzchni. Zasady i procedury oceny struktury geometrycznej powierzchni metodą profilową.
• [15] OHSAKA T., IZUMI F., FUJIKI Y., Raman spectrum of anatase, TiO2, J. Raman Spectrosc., 1978, 7, 321–324.
• [16] WANG Z., SAXENA S.K., Raman spectroscopic study on pressure-induced amorphization in nanocrystalline anatase (TiO2), Solid State Communications, 2001, 118, 75–78.
• [17] TOMPSETT G.A., BOWMAKER G.A., COONEY R.P., METSON J.B., RODGERS K.A., SEAKINS J.M., The Raman spectrum of brookite, TiO2 (Pbca, Z = 8), J. Raman Spectrosc., 1995, 26(1), 57–62.
• [18] HU Y., TAI H.L., HUANG C.L., Effect of brookite phase on the anatase–rutile transition in titania nanoparticles, J. European Ceramic Society, 2003, 23, 691–696.
• [19] DJAOUED Y., BRUNING R., BERSANI D., LOTTICI P.P., BADILESCU S., Sol–gel nanocrystalline brookite-rich titania films, Materials Letters, 2004, 58, 2618–2622.
• [20] NOWICKI B., Struktura geometryczna. Chropowatość i falistość powierzchni, WNT, Warszawa, 1991.
• [21] ŻEBROWSKI H., KOWALSKI M., Pomiary i analiza stereometryczna (3D) powierzchni po obróbce strumieniowo-ściernej. Zagadnienia inżynierii powierzchni w obróbce skrawaniem, Inżynieria powierzchni, 1999.
• [22] DELIGIANNI D.D., KATSALA N., LADAS S., SOTIROPOULOU D., AMEDEE J., MISSIRLIS Y.F., Effect of surface roughness of the titanium alloy Ti6Al4V on human bone marrowcell response and on protein adsorption, Biomaterials, 2001, 22, 1241–1251.
• [23] BĘDZIŃSKI R., FILIPIAK J., PEZOWICZ C., KRZAK-ROŚ J., KOWALSKI M., Influence of substrate roughness on TiO2 and SiO2, coating topography produced by the sol–gel process, Engineering of Biomaterials, 2008, 11 (81–84), 87–89.
• [24] MECHIAKH R., MERICHE F., KREMER R., BENSAHA R., BOUDINE B., BOUDRIOUA A., TiO2 thin films prepared by sol–gel method for waveguiding application: Correlation between the structural and optical properties, Optical Materials, 2007, (30), 645–651.
• [25] TRISI P., RAO W., REBAUDI A., A histometric comparison of smooth and rough titanium implants in human low-density jawbone, Int. J. Oral Maxillofac. Implants., 1999, 14(5), 689–698.