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Polycyclic aromatic hydrocarbons in crude oils from Poland

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Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
The content of 17 polycyclic aromatic hydrocarbons (PAHs) in oil samples derived from all three oil-bearing regions of Poland, i.e. from the Carpathians, the Carpathian Foredeep and the Polish Lowlands (the Fore-Sudetic-Wielkopolska, the Western Pomeranian and the Peribaltic areas), were determined. The concentrations of PAHs determined in these crude oils varied from 22.85 to 332.45 ppm. The average content of PAHs in crude oils from the Carpathians and the Carpathian Foredeep (191.18 ppm) was several times higher than that in crude oils from the Polish Lowlands (44.70 ppm); there was throughout, though, a relatively small variability in the content of perylene, varying from 0.50 to 0.80 ppm. Of PAH compounds determined, the largest share was occupied by 3-cyclic hydrocarbons (an average of 72%) and 4-cyclic (about 24%), whereas the content of 5- and 6-cyclic hydrocarbons did not exceed 3%. Phenanthrene and fluorene were prevailing PAH compounds. The diverse PAH composition in oil samples from the Polish Lowlands compared to those from the Carpathians and the Carpathian Foredeep seems to have resulted more from the composition of original organic matter than from the course of geochemical and biochemical processes (which occur during biomass decay) and the subsequent migration of these compounds in rock formations.
Słowa kluczowe
Rocznik
Strony
81--86
Opis fizyczny
Bibliogr.26 poz., rys., tab., wykr.
Twórcy
  • Polish Geological Institute, Rakowiecka 4, PL-00-975 Warszawa, Poland
  • Polish Geological Institute, Rakowiecka 4, PL-00-975 Warszawa, Poland
Bibliografia
  • 1. BEAK S. O., FIELD R. A., GOLDSTONE M. E., KIRK P. W., LESTER J. N. and PERRY R. (1991) - A review of atmospheric polycyclic aromatic hydrocarbons: sources, fate and behaviour. Water, Air, Soil Pollut., 54: 279-297.
  • 2. BENCE A., KVENVOLDEN K. and KENNICUTT M. (1996) – Organic geochemistry applied to environmental assessments of Prince William Sound Alaska, after the Exxon Waldez oil spill - a review. Org. Geochem., 24 (1): 7-42.
  • 3. BEHYMER T. and HITES R. (1988) - Photolysis of polycyclic aromatic hydrocarbons adsorbed on fly ash. Environ. Sc. Technol., 22 (11): 1311-1319.
  • 4. BOJAKOWSKA I. and SOKOŁOWSKA G. (1998) - Geochemical blackground of multicyclic aromatic hydrocarbons in forest soils (in Polish only). Prz. Geol., 46 (10): 1083-1085.
  • 5. BOJAKOWSKA I. and SOKOŁOWSKA G. (1999) - Geochemia wielopierścieniowych węglowodorów aromatycznych w kaustobiolitach występujących w Polsce. Centr. Arch. Geol. Państw. Inst. Geol. Warszawa.
  • 6. BOJAKOWSKA I., SOKOŁOWSKA G. and GLIWICZ T. (1999) - Geochemia wielopierścieniowych węglowodorów aromatycznych. In: Atlas Geochemiczny Legnicko-Głogowskiego Okręgu Miedziowego: 21-24. Państw. Inst. Geol. Warszawa.
  • 7. CAPACCIONI B., MARTINI M. and MANGANI F. (1995) - Light hydrocarbons in hydrothermal and magmatic fumaroles: hints of catalytic and thermal reactions. Bull. Volcanol., 56 (8): 593-600.
  • 8. JIANG C., ALEKSANDER R., KAGI R. and MURRAY A. (1998) - Polycyclic aromatic hydrocarbons in ancient sediments and their relationships to paleoclimate. Org. Geochem., 29 (5-7): 1721-1735.
  • 9. CZEPIEC I. and KOTARBA M. (1998) - Paleoecology and organic matter in the Late Badenian and Early Sarmatian marine basin of the Polish part of the Carpathian Foredeep (in Polish with English summary). Prz. Geol., 40 (8/2): 732-736.
  • 10. DEPOWSKI S. (1987) - Ropa naftowa i gaz ziemny. In: Budowa Geologiczna Polski. Złoża surowców mineralnych: 49-98. Wyd. Geol. Warszawa.
  • 11. EVANS K. M., GILL R. A. and ROBOTHAM P. W. (1990) - The source, composition and flux of polycyclic aromatic hydrocarbons in sediments of the River Derwent, Derbyshire, U.K. Water, Air, Soil Pollut., 51: 1-12.
  • 12. HARVEY R. (1998) - Environmental chemistry of PAHs. In: PAHs and Related Compounds: 1-54. Springer-Verlag. Berlin, Heidelberg. ten HAVEN H., LAFARGUEB E. and KOTARBA M. (1993) - Oil/oil and oil/source rock correlations in the Carpathian Foredeep and overthrust, south-east Poland. Org. Geochem., 20 (7): 935-959.
  • 13. HOWSAM M. and JONES K. (1998) - Sources of PAHs in the environment. In: PAHs and Related Compounds: 137-174. Springer-Verlag. Berlin, Heidelberg.
  • 14. KARNKOWSKI P. (1993) - Złoża gazu ziemnego i ropy naftowej w Polsce, 1. Niż Polski. Tow. Geosynoptyków “Geos”.
  • 15. KOTARBA M., WIĘCŁAW D. and KOWASKI A. (1998) - Origin of hydrocarbons from selected areas of the Devonian and Zechstein basins of the Polish Lowlands: geochemical evidence. Pr. Państw. Inst. Geol., 165: 261-272.
  • 16. KOZIŃSKI J. and SAADE R. (1998) - Effect of biomass burning on the formation of soot particles and heavy hydrocarbons. An experimental study. Fuel, 77 (4): 225-237.
  • 17. McGRODDY and FARRINGTON (1995) - Sediment porewater partioning of polycyclic aromatic hydrocarbons in three cores from Boston Harbor, Massachusetts. Environ. Sc. Technol., 29 (6): 1542-1550.
  • 18. MALISZEWSKA-KORDYBACH B. and TERELAK H. (1996) - Evaluation of the content of polycyclic aromatic hydrocarbons in soils from rural region of Poland (Lublin Province). II Inter. Sym. Exhb. Environmental Contamination in Central and Eastern Europe: 81-83. Warsaw.
  • 19. OLLIVON D., GARBON B. and CHESTERIKOFF A. (1995) - Analysis of distribution of some polycyclic aromatic hydrocarbons in sediments and suspended matter in the river Seine (France). Water, Air, Soil Pollut., 81: 135-152.
  • 20. PU F., PHILP R., ZHENXI L. and GUANGGUO Y. (1990) - Geochemical characteristics of aromatic hydrocarbons of crude oils and source rocks from different sedimentary environments. Org. Geochem., 16 (1-3): 427-435.
  • 21. RAMANAMPISOA L. and RADKE M. (1995) - Extractable aromatic hydrocarbons in a short-term organic cycle of the Kimmeridge Clay Formation, Vorkshire (U.K.): relationship to primary production and thermal maturity. Org. Geochem., 23 (9): 803-817.
  • 22. REQUEJO A., SASSEN R., MCDONALD T., DENOUX G., KENNICUTT M. and BROOKS J. (1996) - Polynuclear aromatic hydrocarbons (PAH) as indicators of the source and maturity of marine crude oils. Org. Geochem., 29 (5/7): 1737-1744.
  • 23. SILLIMAN J., MEYERS P. and EADIE B. (1998) - Perylen: an indicator of alteration processes or precursor materials? Org. Geochem., 24 (10/11): 1017-1033.
  • 24. SIMONEIT B. and FETZER J. (1996) - High molecular weight polycyclic aromatic hydrocarbons in hydrothermal petroleums from the Gulf of California and Northeast Pacific Ocean. Org. Geochem., 24 (10/11): 1065-1077.
  • 25. SMITH J., GEORGE S. and BATTS B. (1995) - The geosynthesis of alkylaromatics. Org. Geochem., 23 (1): 71-80.
  • 26. TANCELL P., RHEAL M., PEMBERTON R. and BRAVEN J. (1995) - Survival of polycyclic aromatic hydrocarbons during diesel combustion. Environ. Sc. Technol., 29: 2871-2878.
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-article-BAT3-0012-0033
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