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Natural radionuclides (NORM) in a Moroccan river affected by former conventional metal mining activities

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Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
The main aim of this work was to determine the levels of multiple natural radionuclides in an aquatic system (Moulouya river, Morocco) impacted by multiple abandoned Zinc and Lead mines. 238U, 234U, 232Th, 230Th and 210Po were determined by alpha-particle spectrometry in water and sediment samples collected along the river and in samples from three pit lakes of abandoned mines, located in the Upper Moulouya catchment area. The results enabled the analysis of the different levels of impact of former mining activities, depending on the natural radionuclides. While the activity concentration of U-isotopes in Moulouya river water was slightly elevated in the vicinity of abandoned mine wastes, other natural radionuclides (Th-isotopes and 210Po) levels were typical of a natural environment. This fact is clearly reflected in the magnitude and range observed in the distribution coefficients for the different radionuclides analyzed.
Rocznik
Strony
45--51
Opis fizyczny
Bibliogr. 22 poz.
Twórcy
  • Applied Nuclear Physics Group, Applied Physics II Department, ETSA, Universidad de Sevilla, Av Reina Mercedes 2, 41012, Seville, Spain
autor
  • Applied Nuclear Physics Group, Applied Physics II Department, ETSA, Universidad de Sevilla, Av Reina Mercedes 2, 41012, Seville, Spain
  • Applied Nuclear Physics Group, Applied Physics II Department, ETSA, Universidad de Sevilla, Av Reina Mercedes 2, 41012, Seville, Spain
  • Applied Nuclear Physics Group, Applied Physics II Department, ETSA, Universidad de Sevilla, Av Reina Mercedes 2, 41012, Seville, Spain
  • Applied Nuclear Physics Group, Applied Physics II Department, ETSA, Universidad de Sevilla, Av Reina Mercedes 2, 41012, Seville, Spain
autor
  • Geosciences of Natural Resources Laboratory, IbnTofail University, Faculty of Sciences, BP 133, 14000, Kénitra, Morocco
  • Laboratory of Polymers, Radiations and Environment, IbnTofail University, Faculty of Sciences, BP 133, 14000, Kénitra, Morocco
  • Applied Nuclear Physics Group, Applied Physics II Department, ETSA, Universidad de Sevilla, Av Reina Mercedes 2, 41012, Seville, Spain
  • Spanish National Accelerator Center (CNA), Universidad de Sevilla-Junta de Andalucía-CSIC, Seville, Spain
Bibliografia
  • 1. Barbero, L., Gázquez, M. J., Bolívar, J. P., Casas-Ruiz, M., Hierro, A., Baskaran, M., et al. (2014). Mobility of Po and U-isotopes under acid mine drainage conditions: An experimental approach with samples from Río Tinto area (SW Spain). Journal of Environmental Radioactivity, 138, 384-389. https://doi.org/10.1016/j.jenvrad.2013.11.004.
  • 2. Bounakhla, M., Embarch, K., Tahri, M., Baghdad, B., Naimi, M., Bouabdli, A., et al. (2012). PGAA metals analysis in tailings in Zaida abandoned mine, high Moulouya, Morocco. Journal of Radioanalytical and Nuclear Chemistry, 291(1), 129-135. https://doi.org/10.1007/s10967-011-1321-6.
  • 3. Broecker, J. N. (1974). Chemical oceanography. New York. New York: Harcourt-Brace- Jovanovich.
  • 4. Carvalho, F. P., Oliveira, J. M., Lopes, I., & Batista, A. (2007). Radionuclides from past uranium mining in rivers of Portugal. Journal of Environmental Radioactivity, 98(3), 298-314. https://doi.org/10.1016/j.jenvrad.2007.05.007.
  • 5. Casacuberta, N., Lehritani, M., Mantero, J., Masqué, P., Garcia-Orellana, J., & Garcia- Tenorio, R. (2012). Determination of U and Th á-emitters in NORM samples through extraction chromatography by using new and recycled UTEVA resins. Applied Radiation and Isotopes, 70(4), 568-573. https://doi.org/10.1016/j.apradiso.2011.11.063.
  • 6. Coward, J. B., & Osmond, J. K. (1974). Uranium-234 and 238 in the Carrizo sandstone aquifer of south Texas. Isotope techniques in groundwater hydrology, proceedings symposium: Vol. 2, (pp. 131-149). Vienna: International Atomic Energy Agency.
  • 7. Díaz-Francés, I., Mantero, J., Manjón, G., Díaz, J., & García-Tenorio, R. (2013). 210Po and 238U isotope concentrations in commercial bottled mineral water samples in Spain and their dose contribution. Radiation Protection Dosimetry, 156(3), 1-7.
  • 8. Flynn, W. W. (1968). The determination of low levels of polonium-210 in environmental samples. Analytical Chemistry Acta, 43(2), 221-227.
  • 9. González-Labajo, J., Bolívar, J. P., & García-Tenorio, R. (2001). Natural radioactivity in waters and sediments from a Spanish mining river. Radiation Physics and Chemistry, 61(3-6), 643-644. https://doi.org/10.1016/S0969-806X(01)00359-0.
  • 10. Hallstadius, L. (1984). A method for the electrodeposition of actinides. Nuclear Instruments and Methods in Physics Research, 223(2-3), 266-267. https://doi.org/10.1016/0167-5087(84)90659-8.
  • 11. Holm, E., & Fukai, R. (1977). Method for multi-element alpha-spectrometry of actinides and its application to environmental radioactivity studies. Talanta, 24(11), 659-664. https://doi.org/10.1016/0039-9140(77)80061-1.
  • 12. Huang, Y.-J., Chen, Ch.-F., Huang, Y.-Ch., Yue, Q.-J., Zhong, Ch.-M., & Tan, Ch.-J. (2015). Natural radioactivity and radiological hazards assessment of bone-coal from a vanadium mine in central China. Radiation Physics and Chemistry, 107, 82-88. https://doi.org/10.1016/j.radphyschem.2014.10.001.
  • 13. Iavazzo, P., Adamo, P., Boni, M., Hillier, S., & Zampella, M. (2012). Mineralogy and chemical forms of lead and zinc in abandoned mine wastes and soils: An example from Morocco. Journal of Geochemical Exploration, 113, 56-67. https://doi.org/10.1016/j.gexplo.2011.06.001.
  • 14. Kossoff, D., Dubbin, W. E., Alfredsson, M., Edwards, S. J., Macklin, M. G., & Hudson- Edwards, K. A. (2014). Mine tailings dams: Characteristics, failure, environmental impacts, and remediation. Applied Geochemistry, 51, 229-245.
  • 15. Ku, T. L. (1976). The Uranium Series method of age determination. Annual Review of Earth and Planetary Sciences, 4, 347-380.
  • 16. Lee, M. H., & Lee, C. W. (2001). Radiochemical analysis of uranium isotopes in soil and sediment samples with extraction chromatography. Talanta, 54(1), 181-186. https://doi.org/10.1016/S0039-9140(00)00666-4.
  • 17. Makhoukh, M., Sbaa, M., Berrahou, A., & Vanclooster, M. (2011). Contribution à l’étude de l’impact d’un site minier abandonné dans la haute Moulouya sur la qualité de l'Oued Moulouya, Maroc. Afrique Science: Revue Internationale des Sciences et Technologie, 7(3), 33-48.
  • 18. Mantero, J., Lehritane, M., Hurtado, S., & García-Tenorio, R. (2010). Radioanalytical determination of actinoids in refractory matrices by alkali fusion. Journal of Radioanalytical and Nuclear Chemistry, 286(2), 557-563. https://doi.org/10.1007/s10967-010-0782-3.
  • 19. Martínez-Aguirre, A., & García-León, M. (1992). Uranium and Radium isotopes in the Guadalquivir river, southern Spain. Radiation Protection Dosimetry, 45(1-4), 249-252. https://doi.org/10.1093/rpd/45.1-4.249.
  • 20. Michalik, B., Brown, J., & Krajewski, P. (2013). The fate and behavior of enhanced natural radioactivity with respect to environmental protection. Environmental Impact Assessment Review, 38, 163-171. https://doi.org/10.1016/j.eiar.2012.09.001.
  • 21. Persson, B. R. R., & Holm, E. (2011). Polonium-210 and lead-210 in the terrestrial environment: A historical review. Journal of Environmental Radioactivity, 102, 420-429. https://doi.org/10.1016/j.jenvrad.2011.01.005.
  • 22. Saç, M. M., Ortabuk, F., Kumru, M. N., Içhedef, M., & Sert, Ş. (2012). Determination of radioactivity and heavy metals of Bakirçay river in Western Turkey. Applied Radiation and Isotopes, 70(10), 2494-2499.
Uwagi
Opracowanie rekordu ze środków MNiSW, umowa Nr 461252 w ramach programu "Społeczna odpowiedzialność nauki" - moduł: Popularyzacja nauki i promocja sportu (2020).
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-ad6b6c77-fa76-4f1d-943d-1386a590375d
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