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Preparation and environmental toxicity of non-sintered ceramsite using coal gasification coarse slag

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Identyfikatory
Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
In this study, non-sintered ceramsite was prepared using coal gasification coarse slag obtained from a methanol plant. The basic performance and heavy metal leaching toxicity were analyzed. The results showed that seven out of nine non-sintered ceramsite groups were in accordance with the national standard of compressive strength (5 MPa), while only three groups met the national standard of water absorption index of less than 22%. The heavy metal concentrations in these three groups were found to be lower than that specified in National Class IV of surface water environment standards. The concentration of Cr was found to be 16.45 μg/L, which represents only 1% of the IV standard. The optimum mixing ratio, which showed high compressive strength (6.76 MPa) and low water absorption (20.12%), was found to be 73% coal gasification coarse slag, 15% cement, and 12% quartz sand. The characterization using Fourier transform infrared spectroscopy showed that the formation of gelatin in ceramsite enhances the performance of the ceramsite base and increases the immobilization of heavy metal. The study proved that the preparation of non-sintered ceramsite using coal gasification coarse slag reduces its environmental risk and achieves efficient utilization of the slag. Therefore, it can be concluded that it is a feasible and environmental friendly method for the disposal of coal slag.
Rocznik
Strony
84--90
Opis fizyczny
Bibliogr. 34 poz., tab., wykr.
Twórcy
autor
  • School of Chemical & Environmental Engineering, China University of Mining & Technology (Beijing), Beijing, China
autor
  • School of Chemical & Environmental Engineering, China University of Mining & Technology (Beijing), Beijing, China
autor
  • School of Chemical & Environmental Engineering, China University of Mining & Technology (Beijing), Beijing, China
autor
  • School of Chemical & Environmental Engineering, China University of Mining & Technology (Beijing), Beijing, China
autor
  • Department of Civil Engineering, New Mexico State University, Las Cruces, United States
autor
  • Shanghai Municipal Engineering Design Institute (Group) CO., LTD, Shanghai, China
autor
  • School of Chemical & Environmental Engineering, China University of Mining & Technology (Beijing), Beijing, China
autor
  • School of Chemical & Environmental Engineering, China University of Mining & Technology (Beijing), Beijing, China
Bibliografia
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  • 6. Civeira, M.S., Pinheiro, R.N., Gredilla, A., de Vallejuelo, S.F., Oliveira, M.L., Ramos, C.G., Taffarel, S.R., Kautzmann, R.M., Madariaga, J.M. & Silva, L.F. (2016). The properties of the nano-minerals and hazardous elements: Potential environmental impacts of Brazilian coal waste fi re, Science of the Total Environment, 544, pp. 892-900.
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  • 13. Jianhuan, H. (2013). The leaching characteristics of heavy metals from municipal solid waste fly ash and experimental study on cement solidification, South China University of Technology, Guangzhou. (in Chinese)
  • 14. Ismail, I., Bernal, S.A., Provis, J.L., San Nicolas, R., Hamdan, S. & van Deventer, J.S.J. (2014). Modification of phase evolution in alkali-activated blast furnace slag by the incorporation of fly ash, Cement and Concrete Composites, 45, pp. 125-135.
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  • 19. Li, Z., Zhang, H., Zhao, P., He, X. & Duan, X. (2018). Manufacturing of ultra-light ceramsite from slate wastes in Shangri-la, China, Journal of the Korean Ceramic Society, 55, 1, pp. 36-43.
  • 20. Liu, X., Zhao, X., Yin, H., Chen, J. & Zhang, N. (2018). Intermediatecalcium based cementitious materials prepared by MSWI fly ash and other solid wastes: hydration characteristics and heavy metals solidification behavior, Journal of Hazardous Materials, 349, pp. 262-271.
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  • 24. Steffan, J.J., Brevik, E.C., Burgess, L.C. & Cerda, A. (2018). The effect of soil on human health: an overview, European Journal of Soil Science, 69, 1, pp. 159-171.
  • 25. Wang, F.H., Zhang, F., Chen, Y.J., Gao, J. & Zhao, B. (2015). A comparative study on the heavy metal solidification/stabilization performance of four chemical solidifying agents in municipal solid waste incineration fly ash, Journal of Hazardous Materials, 300, pp. 451-458.
  • 26. Wu, S., Huang, S., Ji, L., Wu, Y. & Gao, J. (2014). Structure characteristics and gasification activity of residual carbon from entrained-flow coal gasification slag, Fuel, 122, pp. 67-75.
  • 27. Wu, S., Huang, S., Wu, Y. & Gao, J. (2015). Characteristics and catalytic actions of inorganic constituents from entrained-flow coal gasification slag, Journal of the Energy Institute, 88, 1, pp. 93-103.
  • 28. Xie, K., Li, W. & Zhao, W. (2010). Coal chemical industry and its sustainable development in China, Energy, 35, 11, pp. 4349-4355.
  • 29. Xu, H. (2012). Study on the development and application in BAD of the new unburned fly ash ceramsite, Harbin Institude of Technology, Harbin. (in Chinese)
  • 30. Yao, Z.T., Ji, X.S., Sarker, P.K., Tang, J.H., Ge, L.Q., Xia, M.S. & Xi, Y.Q. (2015). A comprehensive review on the applications of coal fly ash, Earth-Science Reviews, 141, pp. 105-121.
  • 31. Yu, C. (2004). The study of manufacture of fly ash haydite and treating oily waste water with fly ash haydite, Beijing University of Chemical Technology, Beijing. (in Chinese)
  • 32. Zhang, Z., Provis, J.L., Reid, A. & Wang, H. (2015). Mechanical, thermal insulation, thermal resistance and acoustic absorption properties of geopolymer foam concrete, Cement and Concrete Composites, 62, pp. 97-105.
  • 33. Zishu, L., Xu, H., Fang, M., Shan, Q. & Shanwen, X. (2012). The study on manufacture of unbruned fly ash ceramsite with sludge applied to BAF, Environmental Engineering, 30, S2, pp. 262-266. (in Chinese)
  • 34. Zou Zhengyu, L.Y. (2013). Preparation of non-sintered ceramsite from coal fly ash and its performance on heavy metals removal, Chinese Journal of Environmental Engineering, 7, 10, pp. 4054-4060. (in Chinese)
Uwagi
Opracowanie rekordu w ramach umowy 509/P-DUN/2018 ze środków MNiSW przeznaczonych na działalność upowszechniającą naukę (2019).
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-ac660275-1f57-4891-b74a-e3f88271e16b
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