Spatial Distribution of Carbonaceous Aerosol in the Southeastern Baltic Sea Region (Event of Grass Fires)

• Autorzy: Dudoitis V. , Byčenkienė S. , Plauškaitė K. , Bozzetti C. , Fröhlich R. , Mordas G. , Ulevičius V.

Identyfikatory

DOI

10.1515/acgeo-2016-0018

• Języki publikacji: EN

Abstrakty

EN

The aerosol chemical composition in air masses affected by large vegetation fires transported from the Kaliningrad region (Russia) and southeast regions (Belarus and Ukraine) during early spring (March 2014) was characterized at the remote background site of Preila, Lithuania. In this study, the chemical composition of the particulate matter was studied by high temporal resolution instruments, including an Aerosol Chemical Speciation Monitor (ACSM) and a seven-wavelength aethalometer. Air masses were transported from twenty to several hundred kilometres, arriving at the measurement station after approximately half a day of transport. The concentration-weighted trajectory analysis suggests that organic aerosol particles are mainly transported over the Baltic Sea and the continent (southeast of Belarus). Results show that a significant fraction of the vegetation burning organic aerosol is transformed into oxidised forms in less than a half-day. Biomass burning aerosol (BBOA) was quantified from the ACSM data using a positive matrix factorization (PMF) analysis, while its spatial distribution was evaluated using air mass clustering approach.

Słowa kluczowe

EN

ACSM; air masses; organic aerosol; nitrate; sulphate; ammonium; chloride

PL

ACSM; masy powietrza; aerozol organiczny; azotan; siarczan; amon; chlorek

• Wydawca: Instytut Geofizyki PAN ; Springer
• Czasopismo: Acta Geophysica
• Rocznik: 2016
• Tom: Vol. 64, no. 3
• Strony: 711--731
• Opis fizyczny: Bibliogr. 49 poz.

Twórcy

autor

Dudoitis V.

• SRI Center for Physical Sciences and Technology, Vilnius, Lithuania

autor

Byčenkienė S.

• SRI Center for Physical Sciences and Technology, Vilnius, Lithuania

autor

Plauškaitė K.

• SRI Center for Physical Sciences and Technology, Vilnius, Lithuania

autor

Bozzetti C.

• Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI), Villigen, Switzerland

autor

Fröhlich R.

• Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI), Villigen, Switzerland

autor

Mordas G.

• SRI Center for Physical Sciences and Technology, Vilnius, Lithuania

autor

Ulevičius V.

• SRI Center for Physical Sciences and Technology, Vilnius, Lithuania

Bibliografia

• Abdalmogith, S.S., and R.M. Harrison (2005), The use of trajectory cluster analysis to examine the long-range transport of secondary inorganic aerosol in the UK, Atmos. Environ. 39, 35, 6686-6695, DOI: 10.1016/j.atmosenv.2005. 07.059.
• Amiridis, V., E. Giannakaki, D.S. Balis, E. Gerasopoulos, I. Pytharoulis, P. Zanis, S. Kazadzis, D. Melas, and C. Zerefos (2010), Smoke injection heights from agricultural burning in Eastern Europe as seen by CALIPSO, Atmos. Chem. Phys. 10, 23, 11567-11576, DOI: 10.5194/acp-10-11567-2010.
• Bahreini, R., M.D. Keywood, N.L. Ng, V. Varutbangkul, S. Gao, R.C. Flagan, J.H. Seinfeld, D.R. Worsnop, and J.L. Jimenez (2005), Measurements of secondary organic aerosol from oxidation of cycloalkenes, terpenes, and mxylene using an aerodyne aerosol mass spectrometer, Environ. Sci. Technol. 39, 15, 5674-5688, DOI: 10.1021/es048061a.
• Beverland, I.J., T. Tunes, M. Sozanska, R.A. Elton, R.M. Agius, and M.R. Heal (2000), Effect of long-range transport on local PM10 concentrations in the UK, Int. J. Environ. Heal. Res. 10, 3, 229-238, DOI: 10.1080/ 09603120050127176.
• Blum, U., K.H. Fricke, K.P. Müller, J. Siebert, and G. Baumgarten (2005), Longterm lidar observations of polar stratospheric clouds at Esrange in northern Sweden, Tellus B 57, 5, 412-422, DOI: 10.1111/j.1600-0889.2005.00161.x.
• Bond, T.C., S.J. Doherty, D.W. Fahey, P.M. Forster, T. Berntsen, B.J. DeAngelo, M.G. Flanner, S. Ghan, B. Kärcher, D. Koch, S. Kinne, Y. Kondo, P.K. Quinn, M.C. Sarofim, M.G. Schultz, M. Schulz, C. Venkataraman, H. Zhang, S. Zhang, N. Bellouin, S.K. Guttikunda, P.K. Hopke, M.Z. Jacobson, J.W. Kaiser, Z. Klimont, U. Lohmann, J.P. Schwarz, D. Shindell, T. Storelvmo, S.G. Warren, and C.S. Zender (2013), Bounding the role of black carbon in the climate system: A scientific assessment, J. Geophys. Res. 118, 11, 5380-5552, DOI: 10.1002/jgrd.50171.
• Byčenkienė, S., V. Ulevičius, V. Dudoitis, and J. Pauraitė (2013), Identification and characterization of black carbon aerosol sources in the East Baltic region, Adv. Meteorol. 2013, DOI: 10.1155/2013/380614.
• Byčenkienė, S., V. Dudoitis, and V. Ulevičius (2014), The use of trajectory cluster analysis to evaluate the long-range transport of black carbon aerosol in the South-Eastern Baltic region, Adv. Meteorol. 2014, DOI: 10.1155/2014/ 137694.
• Dall’Osto, M., S. Hellebust, R.M. Healy, I.P. O’Connor, I. Kourtchev, J.-R. Sodeau, J. Ovadnevaite, D. Ceburnis, C.-D. O’Dowd, and J.-C. Wenger (2014), Apportionment of urban aerosol sources in Cork (Ireland) by synergistic measurement techniques, Sci. Total Environ. 493, 197-208, DOI: 10.1016/ j.scitotenv.2014.05.027.
• Draxler, R.R., and G.D. Rolph (2014), HYSPLIT (HYbrid Single-Particle Lagrangian Integrated Trajectory) model access via NOAA ARL READY website, NOAA Air Resources Laboratory, Silver Spring, USA, http://ready.arl. noaa.gov/HYSPLIT.php.
• Du, S.Y., and L.A. Rodenburg (2007), Source identification of atmospheric PCBs in Philadelphia/Camden using positive matrix factorization followed by the potential source contribution function, Atmos. Environ. 41, 38, 8596-8608, DOI: 10.1016/j.atmosenv.2007.07.042.
• Fröhlich, R., V. Crenn, A. Setyan, C.A. Belis, F. Canonaco, O. Favez, V. Riffault, J.G. Slowik, W. Aas, M. Aijälä, A. Alastuey, B. Artiñano, N. Bonnaire, C. Bozzetti, M. Bressi, C. Carbone, E. Coz, P.L. Croteau, M.J. Cubison, J.K. Esser-Gietl, D.C. Green, V. Gros, L. Heikkinen, H. Herrmann, J.T. Jayne, C.R. Lunder, M.C. Minguillón, G. Močnik, C.D. O’Dowd, J. Ovadnevaite, E. Petralia, L. Poulain, M. Priestman, A. Ripoll, R. SardaEstève, A. Wiedensohler, U. Baltensperger, J. Sciare, and A.S.H. Prévôt (2015), ACTRIS ACSM intercomparison – Part 2: Intercomparison of ME-2 organic source apportionment results from 15 individual, co-located aerosol mass spectrometers, Atmos. Meas. Tech. Discuss. 8, 1559-1613, DOI: 10.5194/amtd-8-1559-2015.
• Gildemeister, A.E., P.K. Hopke, and E. Kim (2007), Sources of fine urban particulate matter in Detroit, MI, Chemosphere 69, 7, 1064-1074, DOI: 10.1016/ j.chemosphere.2007.04.027.
• Goode, J.G., R.J. Yokelson, R.A. Susott, and D.E. Ward (1999), Trace gas emissions from laboratory biomass fires measured by open-path Fourier transform infrared spectroscopy: Fires in grass and surface fuels, J. Geophys. Res. 104, D17, 21237-21245, DOI: 10.1029/1999JD900360.
• Hamed, A., J. Joutsensaari, S. Mikkonen, L. Sogacheva, M. Dal Maso, M. Kulmala, F. Cavalli, S. Fuzzi, M.C. Facchini, S. Decesari, M. Mircea, K.E.J. Lehtinen, and A. Laaksonen (2007), Nucleation and growth of new particles in Po Valley, Italy, Atmos. Chem. Phys. 7, 2, 355-376, DOI: 10.5194/acp-7- 355-2007.
• Heringa, M.F., P.F. DeCarlo, R. Chirico, T. Tritscher, J. Dommen, E. Weingartner, R. Richter, G. Wehrle, A.S.H. Prévôt, and U. Baltensperger (2011), Investigations of primary and secondary particulate matter of different wood combustion appliances with a high-resolution time-of-flight aerosol mass spectrometer, Atmos. Chem. Phys. 11, 12, 5945-5957, DOI: 10.5194/acp- 11-5945-2011.
• Hildebrandt, L., E. Kostenidou, N. Mihalopoulos, D.R. Worsnop, N.M. Donahue, and S.N. Pandis (2010), Formation of highly oxygenated organic aerosol in the atmosphere: Insights from the Finokalia Aerosol Measurement Experiments, Geophys. Res. Lett. 37, 23, L23801, DOI: 10.1029/2010GL045193.
• Hoh, E., and R.A. Hites (2004), Sources of toxaphene and other organochlorine pesticides in North America as determined by air measurements and potential source contribution function analyses, Environ. Sci. Technol. 38, 15, 4187- 4194, DOI: 10.1021/es0499290.
• IPCC (2013), Climate Change 2013: The Physical Science Basis, Working Group I Contribution to the 5th Assessment Report, Intergovernmental Panel on Climate Change, Bern, Switzerland.
• Jeong, U., J. Kim, H. Lee, J. Jung, Y.J. Kim, C.H. Song, and J.H. Koo (2011), Estimation of the contributions of long range transported aerosol in East Asia to carbonaceous aerosol and PM concentrations in Seoul, Korea using highly time resolved measurements: a PSCF model approach, J. Environ. Monit. 13, 7, 1905-1918, DOI: 10.1039/c0em00659a.
• Kabashnikov, V.P., A.P. Chaikovsky, T.L. Kucsera, and N.S. Metelskaya (2011), Estimated accuracy of three common trajectory statistical methods, Atmos. Environ. 45, 31, 5425-5430, DOI: 10.1016/j.atmosenv.2011.07.006.
• Kroll, J.H., and J.H. Seinfeld (2008), Chemistry of secondary organic aerosol: Formation and evolution of low-volatility organics in the atmosphere, Atmos. Environ. 42, 16, 3593-3624, DOI: 10.1016/j.atmosenv.2008.01.003.
• Kulmala, M., and V.M. Kerminen (2008), On the formation and growth of atmospheric nanoparticles, Atmos. Res. 90, 2-4, 132-150, DOI: 10.1016/ j.atmosres.2008.01.005.
• Kulmala, M., M. Dal Maso, J.M. Mäkelä, L. Pirjola, M. Väkevä, P. Aalto, P. Miikkulainen, K. Hämeri, and C.D. O’Dowd (2001), On the formation, growth and composition of nucleation mode particles, Tellus B 53, 4, 479-490, DOI: 10.1034/j.1600-0889.2001.530411.x.
• Kulmala, M., A. Asmi, H.K. Lappalainen, U. Baltensperger, J.-L. Brenguier, M.C. Facchini, H.-C. Hansson, Ø. Hov, C.D. O’Dowd, U. Pöschl, A. Wiedensohler, R. Boers, O. Boucher, G. de Leeuw, H.A.C. Denier van der Gon, J. Feichter, R. Krejci, P. Laj, H. Lihavainen, U. Lohmann, G. McFiggans, T. Mentel, C. Pilinis, I. Riipinen, M. Schulz, A. Stohl, E. Swietlicki, E. Vignati, C. Alves, M. Amann, M. Ammann, S. Arabas, P. Artaxo, H. Baars, D.C.S. Beddows, R. Bergström, J.P. Beukes, M. Bilde, J.F. Burkhart, F. Canonaco, S.L. Clegg, H. Coe, S. Crumeyrolle, B. D’Anna, S. Decesari, S. Gilardoni, M. Fischer, A.M. Fjaeraa, C. Fountoukis, C. George, L. Gomes, P. Halloran, T. Hamburger, R.M. Harrison, H. Herrmann, T. Hoffmann, C. Hoose, M. Hu, A. Hyvärinen, U. Hõrrak, Y. Iinuma, T. Iversen, M. Josipovic, M. Kanakidou, A. Kiendler-Scharr, A. Kirkevåg, G. Kiss, Z. Klimont, P. Kolmonen, M. Komppula, J.-E. Kristjánsson, L. Laakso, A. Laaksonen, L. Labonnote, V.A. Lanz, K.E.J. Lehtinen, L.V. Rizzo, R. Makkonen, H.E. Manninen, G. McMeeking, J. Merikanto, A. Minikin, S. Mirme, W.T. Morgan, E. Nemitz, D. O’Donnell, T.S. Panwar, H. Pawlowska, A. Petzold, J.J. Pienaar, C. Pio, C. Plass-Duelmer, A.S.H. Prévôt, S. Pryor, C.L. Reddington, G. Roberts, D. Rosenfeld, J. Schwarz, Ø. Seland, K. Sellegri, X.J. Shen, M. Shiraiwa, H. Siebert, B. Sierau, D. Simpson, J.Y. Sun, D. Topping, P. Tunved, P. Vaattovaara, V. Vakkari, J.P. Veefkind, A. Visschedijk, H. Vuollekoski, R. Vuolo, B. Wehner, J. Wildt, S. Woodward, D.R. Worsnop, G.-J. van Zadelhoff, A.A. Zardini, K. Zhang, P.G. van Zyl, V.-M. Kerminen, K.S. Carslaw, and S.N. Pandis (2011), General overview: European integrated project on Aerosol Cloud Climate and Air Quality Interactions (EUCAARI) – integrating aerosol research from nano to global scales, Atmos. Chem. Phys. 11, 24, 13061-13143, DOI: 10.5194/acp-11-13061-2011.
• Labonne, M., F.-M. Bréon, and F. Chevallier (2007), Injection height of biomass burning aerosols as seen from a spaceborne lidar, Geophys. Res. Lett. 34, 11, L11806, DOI: 10.1029/2007GL029311.
• Mauderly, J.L., and J.C. Chow (2008), Health effects of organic aerosols, Inhal. Toxicol. 20, 3, 257-288, DOI: 10.1080/08958370701866008.
• Ng, N.L., M.R. Canagaratna, Q. Zhang, J.L. Jimenez, J. Tian, I.M. Ulbrich, J.H. Kroll, K.S. Docherty, P.S. Chhabra, R. Bahreini, S.M. Murphy, J.H. Seinfeld, L. Hildebrandt, N.M. Donahue, P.F. DeCarlo, V.A. Lanz, A.S.H. Prévôt, E. Dinar, Y. Rudich, and D.R. Worsnop (2010), Organic aerosol components observed in Northern Hemispheric datasets from Aerosol Mass Spectrometry, Atmos. Chem. Phys. 10, 10, 4625-4641, DOI: 10.5194/acp-10-4625-2010.
• Ng, N.L., S.C. Herndon, A. Trimborn, M.R. Canagaratna, P.L. Croteau, T.B. Onasch, D. Sueper, D.R. Worsnop, Q. Zhang, Y.L. Sun, and J.T. Jayne (2011), An Aerosol Chemical Speciation Monitor (ACSM) for routine monitoring of the composition and mass concentrations of ambient aerosol, Aerosol Sci. Technol. 45, 7, 780-794, DOI: 10.1080/02786826.2011. 560211.
• Ovadnevaitė, J., K. Kvietkus, and A. Maršalka (2006), 2002 summer fires in Lithuania: Impact on the Vilnius city air quality and the inhabitants health, Sci. Total Environ. 356, 1-3, 11-21, DOI: 10.1016/j.scitotenv.2005.04.013.
• Paatero, P. (1997), Least squares formulation of robust non-negative factor analysis, Chemometr. Intell. Lab. Syst.. 37, 1, 23-35, DOI: 10.1016/S0169-7439(96) 00044-5.
• Pratt, K.A., S.M. Murphy, R. Subramanian, P.J. DeMott, G.L. Kok, T. Campos, D.C. Rogers, A.J. Prenni, A.J. Heymsfield, J.H. Seinfeld, and K.A. Prather (2011), Flight-based chemical characterization of biomass burning aerosols within two prescribed burn smoke plumes, Atmos. Chem. Phys. 11, 24, 12549-12565, DOI: 10.5194/acp-11-12549-2011.
• Putaud, J.P., F. Raes, R. van Dingenen, E. Brüggemann, M.C. Facchini, S. Decesari, S. Fuzzi, R. Gehrig, C. Hüglin, P. Laj, G. Lorbeer, W. Maenhaut, N. Mihalopoulos, K. Müller, X. Querol, S. Rodriguez, J. Schneider, G. Spindler, H. ten Brink, K. Tørseth, and A. Wiedensohler (2004), A European aerosol phenomenology – 2: Chemical characteristics of particulate matter at kerbside, urban, rural and background sites in Europe, Atmos. Environ. 38, 16, 2579-2595, DOI: 10.1016/j.atmosenv.2004.01.041.
• Putaud, J.P., R. van Dingenen, A. Alastuey, H. Bauer, W. Birmili, J. Cyrys, H. Flentje, S. Fuzzi, R. Gehrig, H.C. Hansson, R.M. Harrison, H. Herrmann, R. Hitzenberger, C. Hüglin, A.M. Jones, A. Kasper-Giebl, G. Kiss, A. Kousa, T.A.J. Kuhlbusch, G. Löschau, W. Maenhaut, A. Molnar, T. Moreno, J. Pekkanen, C. Perrino, M. Pitz, H. Puxbaum, X. Querol, S. Rodriguez, I. Salma, J. Schwarz, J. Smolik, J. Schneider, G. Spindler, H. ten Brink, J. Tursic, M. Viana, A. Wiedensohler, and F. Raes (2010), A European aerosol phenomenology – 3: Physical and chemical characteristics of particulate matter from 60 rural, urban, and kerbside sites across Europe, Atmos. Environ. 44, 10, 1308-1320, DOI: 10.1016/j.atmosenv.2009.12.011.
• Reid, J.S., R. Koppmann, T.-F. Eck, and D.P. Eleuterio (2005), A review of biomass burning emissions. Part II: Intensive physical properties of biomass burning particles, Atmos. Chem. Phys. 5, 3, 799-825, DOI: 10.5194/acp-5-799-2005.
• Rizzo, M.J., and P.A. Scheff (2007), Fine particulate source apportionment using data from the USEPA speciation trends network in Chicago, Illinois: Comparison of two source apportionment models, Atmos. Environ. 41, 29, 6276- 6288, DOI: 10.1016/j.atmosenv.2007.03.055.
• Saarikoski, S., M. Sillanpää, M. Sofiev, H. Timonen, K. Saarnio, K. Teinilä, A. Karppinen, J. Kukkonen, and R. Hillamo (2007), Chemical composition of aerosols during a major biomass burning episode over northern Europe in spring 2006: Experimental and modelling assessments, Atmos. Environ. 41, 17, 3577-3589, DOI: 10.1016/j.atmonsenv.2006.12.053.
• Salvador, P., B. Artiñano, D.G. Alonso, X. Querol, and A. Alastuey (2004), Identification and characterisation of sources of PM10 in Madrid (Spain) by statistical methods, Atmos. Environ. 38, 3, 435-447, DOI: 10.1016/j.atmosenv. 2003.09.070.
• Sato, K., A. Takami, T. Isozaki, T. Hikida, A. Shimono, and T. Imamura (2010), Mass spectrometric study of secondary organic aerosol formed from the photo-oxidation of aromatic hydrocarbons, Atmos. Environ. 44, 8, 1080- 1087, DOI: 10.1016/j.atmosenv.2009.12.013.
• Sciare, J., K. Oikonomou, H. Cachier, N. Mihalopoulos, M.O. Andreae, W. Maenhaut, and R. Sarda-Estève (2005), Aerosol mass closure and reconstruction of the light scattering coefficient over the Eastern Mediterranean Sea during the MINOS campaign, Atmos. Chem. Phys. 5, 2253-2265, DOI: 10.5194/ acp-5-2253-2005.
• Sillanpää, M., A. Frey, R. Hillamo, A.S. Pennanen, and R.O. Salonen (2005), Organic, elemental and inorganic carbon in particulate matter of six urban environments in Europe, Atmos. Chem. Phys. 5, 11, 2869-2879, DOI: 10.5194/acp-5-2869-2005.
• Takami, A., T. Miyoshi, A. Shimono, N. Kaneyasu, S. Kato, Y. Kajii, and S. Hatakeyama (2007), Transport of anthropogenic aerosols from Asia and subsequent chemical transformation, J. Geophys. Res. 112, D22, D22S31, DOI: 10.1029/2006JD008120.
• Takegawa, N., T. Miyakawa, Y. Kondo, J.L. Jimenez, Q. Zhang, D.R. Worsnop, and M. Fukuda (2006), Seasonal and diurnal variations of submicron organic aerosol in Tokyo observed using the Aerodyne aerosol mass spectrometer, J. Geophys. Res. 111, D11, D11206, DOI: 10.1029/2005JD006515.
• Ulevičius, V., G. Mordas, and K. Plauškaitė (2002), Evolution of aerosol particle size distribution in the coastal environment: effect of relative humidity, SO2 and NO2, Environ. Chem. Phys. 24, 1, 13-17.
• Ulevičius, V., S. Byčenkienė, V. Remeikis, A. Garbaras, S. Kecorius, J. Andriejauskienė, D. Jasinevičienė, and G. Mocnik (2010), Characterization of pollution events in the East Baltic region affected by regional biomass fire emissions, Atmos. Res. 98, 2-4, 190-200, DOI: 10.1016/j.atmosres.2010.03. 021.
• van Dingenen, R., F. Raes, J.P. Putaud, U. Baltensperger, A. Charron, M.C. Facchini, S. Decesari, S. Fuzzi, R. Gehrig, H.C. Hansson, R.M. Harrison, C. Hüglin, A.M. Jones, P. Laj, G. Lorbeer, W. Maenhaut, F. Palmgren, X. Querol, S. Rodriguez, J. Schneider, H. ten Brink, P. Tunved, K. Tørseth, B. Wehner, E. Weingartner, A. Wiedensohler, and P. Wåhlin (2004), A European aerosol phenomenology – 1: Physical characteristic of particulate matter at kerbside, urban, rural and background sites in Europe, Atmos. Environ. 38, 16, 2561-2577, DOI: 10.1016/j.atmosenv.2004.01.040.
• Virkkula, A., T. Mäkelä, R. Hillamo, T. Yli-Tuomi, A. Hirsikko, K. Hämeri, and I.K. Koponen (2007), A simple procedure for correcting loading effects of Aethalometer data, J. Air Waste Manag. Assoc. 57, 10, 1214-1222, DOI: 10.3155/1047-3289.57.10.1214.
• Wang, Z.B., M. Hu, D.L. Yue, L.Y. He, X.F. Huang, Q. Yang, J. Zheng, R.Y. Zhang, and Y.H. Zhang (2013), New particle formation in the presence of a strong biomass burning episode at a downwind rural site in PRD, China, Tellus B 65, 19965, DOI: 10.3402/tellusb.v65i0.19965.
• Yttri, K.E., W. Aas, A. Bjerke, J.N. Cape, F. Cavalli, D. Ceburnis, C. Dye, L. Emblico, M.C. Facchini, C. Forster, J.E. Hanssen, H.C. Hansson, S.G. Jennings, W. Maenhaut, J.P. Putaud, and K. Tørseth (2007), Elemental and organic carbon in PM10: a one year measurement campaign within the European Monitoring and Evaluation Programme EMEP, Atmos. Chem. Phys. 7, 22, 5711-5725, DOI: 10.5194/acp-7-5711-2007.

Uwagi

PL

Opracowanie ze środków MNiSW w ramach umowy 812/P-DUN/2016 na działalność upowszechniającą naukę