Influence of nitrogen configuration on the electrochemical properties of carbonized poly(acrylonitrile)-ionic liquid as anode materials in lithium ion batteries

• Autorzy: Wang Lei , Meng Yanshuang , Du Mengqi , Wang Gongrui , Xia Jun , Zhu Fuliang , Zhang Yue

Identyfikatory

DOI

10.2478/msp-2020-0062

• Języki publikacji: EN

Abstrakty

EN

A sequence of N-doped carbon materials has been synthesized using poly(acrylonitrile)-ionic liquid copolymers as carbon precursors. The nitrogen content and configuration in carbon materials has been changed regularly within a certain range by adjusting the proportion of ionic liquids. We found that the capacity and rate performance increased dramatically after the introduction of ionic liquids, which was attributed to incorporation of higher amount pyridinic-N, pyrrolic-N into the carbon materials. Besides, with the increase of the graphitic-N, the initial Coulombic efficiency decreased from 58.5 % to 53.47 % and the RSEI raised from 66.34 W to 140.96 W, which was attributed to the higher cohesive energy of Li dimmer than adsorption energy of graphitic-N with Li, since more lithium clusters during the formation of SEI film were formed. The electrochemical tests also revealed the negative role of graphitic-N in the capacity. Therefore, this work provides a feasible method to design the nitrogen content and configuration of the N-doped carbon materials.

Słowa kluczowe

EN

graphitic-N; poly(acrylonitrile)-ionic liquid copolymers; carbon materials; lithium-ion batteries

• Wydawca: De Gruyter
• Czasopismo: Materials Science Poland
• Rocznik: 2020
• Tom: Vol. 38, No. 4
• Strony: 518--525
• Opis fizyczny: Bibliogr. 43 poz., rys., tab.

Twórcy

autor

Wang Lei

• School of Materials Science and Engineering, Lanzhou University of Technology, Lanzhou 730050, China

autor

Meng Yanshuang

• School of Materials Science and Engineering, Lanzhou University of Technology, Lanzhou 730050, China

autor

Du Mengqi

• School of Materials Science and Engineering, Lanzhou University of Technology, Lanzhou 730050, China

autor

Wang Gongrui

• School of Materials Science and Engineering, Lanzhou University of Technology, Lanzhou 730050, China

autor

Xia Jun

• School of Materials Science and Engineering, Lanzhou University of Technology, Lanzhou 730050, China

autor

Zhu Fuliang

• School of Materials Science and Engineering, Lanzhou University of Technology, Lanzhou 730050, China
• State Key Laboratory of Advanced Processing and Recycling of Non-ferrous Metals, Lanzhou 730050, China

autor

Zhang Yue

• Department of Mechanical and Industrial Engineering, Texas A&M University-Kingsville, Kingsville, Texas, 78363, USA

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Uwagi

Opracowanie rekordu ze środków MNiSW, umowa Nr 461252 w ramach programu "Społeczna odpowiedzialność nauki" - moduł: Popularyzacja nauki i promocja sportu (2021).