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224Ra and the 224Ra/228Ra activity ratio in selected mineral waters from the Polish Carpathians

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Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
Mineral and therapeutic waters widely occurring in the Polish Carpathians contain a vast amount of biogenic elements. However, radioactive elements like radium isotopes are also found in these waters. This paper presents the first results of the activity concentration measurements of 224Ra in selected mineral waters of the Polish Carpathians. Additionally, the content of 226Ra and 228Ra, and the activity ratios of 224Ra/228Ra, 224Ra/226Ra and 226Ra/228Ra in the waters were determined. The work was based on a method for the simultaneous determination of 224Ra, 226Ra and 228Ra in water samples using the a/b liquid scintillation spectrometer. The results show that the activity concentrations of 224Ra, 226Ra and 228Ra in the mineral waters are comparable and vary from ca. 220 mBq/L to above 1500 mBq/L. The activity ratios of 224Ra/228Ra, 224Ra/226Ra and 226Ra/228Ra are variable within the ranges of 0.68 to 1.48, 0.65 to 1.48, and 0.78 to 2.05, respectively. The committed effective dose resulting from the intake of 224Ra through the water consumption is far lower than that from 226Ra and 228Ra.
Słowa kluczowe
Rocznik
Strony
771--778
Opis fizyczny
Bibliogr. 33 poz., tab., rys., wykr.
Twórcy
autor
  • AGH University of Science and Technology, Faculty of Geology, Geophysics and Environmental Protection, al. A. Mickiewicza 30, 30-059 Kraków, Poland
autor
  • AGH University of Science and Technology, Faculty of Geology, Geophysics and Environmental Protection, al. A. Mickiewicza 30, 30-059 Kraków, Poland
autor
  • Hanoi University of Mining and Geology, Faculty of Oil and Gas, Vietnam
autor
  • AGH University of Science and Technology, Faculty of Physics and Applied Computer Science, al. A. Mickiewicza 30, 30-059 Kraków, Poland
Bibliografia
  • 1. Asikainen, M., Kahlos, H., 1979. Anomalously high concentrations of uranium, radium and radon in water from drilled well in the Helsinki region. Geochimica et Cosmochimica Acta, 44: 1681-1686.
  • 2. Bayés, J.C., Gómez, E., Garcias, F., Casas, M., Cerdá, V., 1996. Radium determination in mineral waters. Applied Radiation and Isotopes, 47: 849-853.
  • 3. Brown, E., Firestone, R., Shirley, V., 1986. Table of Radioactive Isotopes. John Wiley & Sons, New York, Chichester, Brisbane, Toronto, Singapore.
  • 4. Currie, L.A., 2008. Detection and quantification capabilities in nuclear analytical measurement. In: Analysis of Environmental Radionuclides (ed. S.P. Povinec): 49-136. Elsevier.
  • 5. Davidson, M.R., Dickson, B.L., 1986. A porous flow model for steady-state transport of radium in ground water. Water Resources Research, 22: 34-44.
  • 6. Euratom, 2013. Council Directive 2013/51/Euratom of 22 October 2013 laying down requirements for the protection of the health of the general public with regard to radioactive substances in water intended for human consumption.
  • 7. Godoy, J.M., da Amaral, E.C., Luiza, M., Godoy, D.P., 2001. Natural radionuclides in Brazilian mineral water and consequent doses to the population. Journal of Environmental Radioactivity, 53: 175-182.
  • 8. Grundl, T., Cape, M., 2006. Geochemical factors controlling radium activity in sandstone aquifer. Ground Water, 44: 518-527.
  • 9. Horrocks, D.L., 1974. Application of Liquid Scintillation Counting. Academic Press, New York.
  • 10. ICRP, 1995. Age-Dependent Doses to Members of the Public From Intake of Radionuclides - Part 5 Compilation of Ingestion and Inhalation Dose Coefficients. International Commission on Radiological Protection, Publication 72, Ann. ICRP 26 (1).
  • 11. King, P., Michel, J., Moore, W., 1982. Ground water geochemistry of 228 Ra, 226 Ra and 222 Rn. Geochimica et Cosmochimica Acta, 46: 1173-1182.
  • 12. Langmuir, D., 1997. Aqueous Environmental Chemistry. Prentice Hall. Upper Saddle River, New Jersey.
  • 13. Langmuir, D., Melchior, D., 1985. The geochemistry of Ca, Sr, Ba and Ra sulfates in some deep brines from Palo Duro Basin, Texas. Geochimica et Cosmochimica Acta, 49: 2423-2432.
  • 14. Lucivjansky, L., 1999. Natural radioactivity of water in Slovakia. Slovak Geological Magazine, 5: 53-61.
  • 15. Manjón, G., Vioque, I., Moreno, H., García-Tenorio, R., García-León, M., 1996. Determination of 226Ra and 224Ra in drinking waters by liquid scintillation counting. Applied Radiation and Isotopes, 48: 535-540.
  • 16. Martin, P., Akber, R.A., 1999. Radium isotopes as indicators of adsorption-desorption interactions and barite formation in groundwater. Journal of Environmental Radioactivity, 46: 271-286.
  • 17. Nguyen, D.C., Niewodniczański J., Dorda J., Ochoński A., Chruściel E., Tomza I., 1997. Determination of radium isotopes in mine waters through a- and b-activities measured by liquid scintillation spectrometry. Journal of Radioanalytical & Nuclear Chemistry, 222: 69-74.
  • 18. Nguyen, D.C., Duliński, M., Jodłowski, P., Nowak, J., Różański, K., Śleziak, M., Wachniew, P., 2011. Natural radioactivity in groundwater - a review. Isotopes in Environmental and Health Studies, 47: 415-437.
  • 19. Nguyen, D.C., Rajchel, L., Nowak, J., Jodłowski, P., 2012. Radium isotopes in the Polish Outer Carpathian mineral waters of various chemical composition. Journal of Environmental Radioactivity, 112: 38-44.
  • 20. Nguyen, D.C., Kopeć, M., Nowak J., 2016. Factors controlling 226Ra,228Ra and their activity ratio in groundwater - an application in Polish Carpathian mineral waters. Geology, Geophysics & Environment, 42: 337-351.
  • 21. Osmond, J.K., Cowart, J.B., 1976. The theory and uses of natural uranium isotopic variations in hydrology. Atomic Energy Review, 14: 621-679.
  • 22. Oszczypko, N., Uchman, A., Malata, E., 2006. Rozwój paleotektoniczny basenów Karpat zewnętrznych i pienińskiego pasa skałkowego (in Polish). Instytut Nauk Geologicznych Uniwersytetu Jagiellońskiego, Kraków.
  • 23. Plewa, M., Plewa S., 1992. Petrofizyka (in Polish). Wyd. Geol., Warszawa.
  • 24. Rajchel, L., 2012. Carbonated waters and waters containing carbon dioxide of the Polish Carpathians (in Polish with English summary). Wydawnictwo AGH, Kraków.
  • 25. Rajchel, L., Czop, M., 2012. Hydrogeochemical modelling of chloride mineral water from Rabka spa (Carpathians Mountains, Poland). Geological Quarterly, 56 (4): 681-690.
  • 26. Ruberu, S.R., Liu, Y.G., Perera, S.K., 2005. Occurrence of 224Ra, 226Ra, 228Ra, gross alpha, and uranium in California groundwater. Health Physics, 89: 667-678.
  • 27. Sturchio, N.C., Bohlke, J.K., Markun, F.J., 1992. Radium isotope geochemistry of thermal water, Yellowstone National Park, Wyoming, USA. Geochimica et Cosmochimica Acta, 57: 1203-1214.
  • 28. Szabo, Z., DePaul, V.T., Fischer, J.M., Kraemer, T.F., Jacobsen, E., 2012. Occurrence and geochemistry of radium in water from principal drinking-water aquifer system of the United States. Applied Geochemistry, 37: 729-752.
  • 29. Vesterbacka, P., Turtiainen, T., Heinävaara, S., Arvela, H., 2006. Activity concentrations of 226Ra and 228Ra in drilled well water in Finland. Radiation Protection Dosimetry, 121: 406-421.
  • 30. Walencik-Łata, A., Kozłowska, B., Dorda, J., Przylibski, T.A., 2016. The detailed analysis of natural radionuclides dissolved in spa water of the Kłodzko Valley, Sudety Mountains, Poland. Science of the Total Environment, 569-570:1174-1184.
  • 31. Waller, G., Steininger, G., 2007. Radium isotopes and 222Rn in Austrian drinking waters, Journal of Radioanalytical and Nuclear Chemistry, 274: 511-516.
  • 32. Waller, G., Wagner, R., Katzlberger, Ch., 2008. Natural radionuclides in Austrian mineral water and their sequential measurement by fast methods. Journal of Environmental Radioactivity, 99: 1090-1094.
  • 33. WHO, 2008. Guidelines for Drinking-Water Quality. World Health Organization, Geneva.
Uwagi
Opracowanie rekordu w ramach umowy 509/P-DUN/2018 ze środków MNiSW przeznaczonych na działalność upowszechniającą naukę (2018).
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-8905e4a4-0b97-4f27-9089-19620f5c3fd9
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