Styrene epoxidation over heterogeneous manganese (III) complexes

• Autorzy: Kuźniarska-Biernacka I. , Lisinska-Czekaj A. , Czekaj D. , Alves M. J. , Fonseca A. M. , Neves I. C.

Identyfikatory

DOI

DOI: 10.1515/amm-2016-0242

• Języki publikacji: EN

Abstrakty

EN

The manganes (III) complex functionalised with 2,3-dihydropyridazine has been encapsulated in the supercages of the NaY zeolite using two different procedures, flexible ligand and in situ complex. The parent zeolite and the encapsulated manganese (LTI) complexes were screened as catalysts for styrene oxidation by using t-BOOH as the oxygen source in acetonitrile. Under the optimized conditions, the catalysts exhibited moderate activity with high selectivity to benzaldehyde.

Słowa kluczowe

EN

styrene epoxidation; heterogeneous manganes

• Wydawca: Institute of Metallurgy and Materials Science of Polish Academy of Sciences ; Committee of Materials Engineering and Metallurgy of Polish Academy of Sciences
• Czasopismo: Archives of Metallurgy and Materials
• Rocznik: 2016
• Tom: Vol. 61, iss. 3
• Strony: 1477--1482
• Opis fizyczny: Bibliogr. 31 poz., rys., tab., wykr.

Twórcy

autor

Kuźniarska-Biernacka I.

• Departamento de Química, Centro de Química, Universidade do Minho, 4710-057 Braga, Portugal
• Departamento de Química E Bioquímica Faculdade de Ciencias da Universidade do Porto, Rua de Campo Alegre, 4169-007 Porto, Portugal

autor

Lisinska-Czekaj A.

• University of Silesia, Destitute of Technology and Mechatronics, 41-200 Sosnowiec, 12 Żytnia str., Poland

autor

Czekaj D.

• University of Silesia, Destitute of Technology and Mechatronics, 41-200 Sosnowiec, 12 Żytnia str., Poland

autor

Alves M. J.

• Departamento de Química, Centro de Química, Universidade do Minho, 4710-057 Braga. Portugal

autor

Fonseca A. M.

• Departamento de Química, Centro de Química, Universidade do Minho, 4710-057 Braga. Portugal

autor

Neves I. C.

• Departamento de Química, Centro de Química, Universidade do Minho, 4710-057 Braga. Portugal

Bibliografia

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Uwagi

EN

IKB thanks to Foundation for the Science and Technology (FCT, Portugal), for the contract under “Programa Ciencia 2007” and for the contract under the project "n-STeP - Nanostructured systems for Tail" (NORTE-07-0124- FEDER-000039, supported by Norte (ON.2). FCT and FEDER (European Fund for Regional Development)-COMPETE-QREN-EU for financial support to the Research Centres, CQ/UM [PEst-C/QUI/UI0686/2013 (F-COMP-01-0124- FEDER-037302). This work is funded also by FEDER funds through the Operational Programme for Competitiveness Factors - COMPETE and by National Funds through FCT - Foundation for Science and Technology under the grant PEST-C/EQB/LA0006/2013/37285.