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TiO2/Al–MCM-41 mesoporous materials were prepared via sol-gel method by loading titania onto Al–MCM-41 mesoporous molecular sieve by hydrothermal treatment from coal-series kaolin as raw material. The TiO2/Al–MCM-41 mesoporous materials were characterized by XRD, FT-IR, HRTEM, N2 adsorption-desorption and the photocatalytic degradation of methyl orange solution under visible light irradiation. The results showed that the TiO2/Al–MCM-41 mesoporous materials possessed a high surface area of 369.9 – 751.3 m2/g and a homogeneous pore diameters of 2.3 – 2.8 nm. The titania crystalline phase was anatase, and the particles size of TiO2 increased with TiO2 content. The Al–MCM-41 mesoporous materials exhibited excellent photodegradation activity under visible-light irradiation for methyl orange.
Słowa kluczowe
Wydawca
Czasopismo
Rocznik
Tom
Strony
372--377
Opis fizyczny
Bibliogr. 26 poz., rys., tab., wykr.
Twórcy
autor
- School of Materials Science and Engineering, Nanjing University of Science and Technology, Jiangsu Nanjing 210094, P. R. China
- School of Materials Science and Engineering, Nanjing University of Science and Technology, Jiangsu Nanjing 210094, P. R. China
autor
- School of Materials Engineering, Yancheng Institute of Technology, Jiangsu Yancheng, 224051, P. R. China
autor
- School of Materials Science and Engineering, Nanjing University of Science and Technology, Jiangsu Nanjing 210094, P. R. China
autor
- College of Materials Science and Engineering, Nanjing University of Technology, Jiangsu Nanjing 210009, P. R. China
autor
- School of Materials Engineering, Yancheng Institute of Technology, Jiangsu Yancheng, 224051, P. R. China
autor
- School of Materials Engineering, Yancheng Institute of Technology, Jiangsu Yancheng, 224051, P. R. China
Bibliografia
- [1] MA H. Z., WANG B., WANG Y., J. Hazard. Mater., 145 (2007), 417.
- [2] TOYA T., KAMESHIMA Y., NAKAJIMA A., OKAD K., Ceram. Int., 32 (2006), 789.
- [3] WU Q. S., LI S. P., SU S. S., Chemical Industry Engineering and Progress, 28 (2009), 130 (in Chinese).
- [4] WU Q. S., LI S. P., SU S. S., Chemical Industry Engineering and Progress, 28 (2009), 458 (in Chinese).
- [5] TUEL A., HUBERT-PTALZGRAT L. G., J. Catal., 217 (2003), 343.
- [6] LIHITKAR N. B., ABYANEH M. K., SAMUEL V., PASRICHA R., GOSAVI S. W., KULKARNI, S. K., J. Colloid Interface Sci., 314 (2007), 310.
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- [8] BECK J. S. et al., Am. Chem. Soc., 114 (1992), 10834.
- [9] WANG L. J., LI D., WANG R., HE Y., QI Q., ZHANG T., Sens. Actuators, B: Chem, 133 (2008), 622.
- [10] CHEN H. Y., XI H. X., CAI X. Y., YU Q., Microporous Mesoporous Mater., 118 (2009), 396.
- [11] YANG H. M., DENG Y. H., DU C. F., Colloids Surf., A, 339 (2009), 111.
- [12] SADJADI M. FARHADYAR S., N., ZARE K., Superlattices Microstruct., 46 (2009), 77.
- [13] AKPAN U. G., HAMEED B. H., J. Hazard. Mater., 170 (2009), 520.
- [14] XIE Y., LI Y. Z., ZHAO X. J., J. Mol. Catal. A: Chem, 277 (2007), 119.
- [15] XIAO Y., DANG L. Q., AN L. Z., BAI S. Y., LEI Z. B., 29 (2008), 31.
- [16] LI S. P., WU Q. S., J. Mater. Sci. Eng., 27 (2009), 233 (in Chinese).
- [17] LI S. P., WU Q. S., Chin. Environ. Eng., 28 (2010), 403 (in Chinese).
- [18] WU Q. S., LI S. P., J. Wuhan University Tech. (Mater Sci. Ed.), 26 (2009), 514.
- [19] MOENKE H. H. W.. Silica, the three dimensional silicates, borosilicates and beryllium silicates. The Infrared Spectra of Minerals, Mineralogical Society. London, 1974.
- [20] KUBICKI J. D., BLAKE G. A., APITZ S. E., Am. Mineral., 81 (1996), 789.
- [21] KIYOSHI O., AKIRA S., TAKAHIRO T., SHIGEO H., ATSUO Y., KENNETH J. D. M., Microporous Mesoporous Mater., 21 (1998), 289.
- [22] XU H. L. et al., J. Phys. Chem. Solids, 72 (2010), 24.
- [23] HSIEN Y.H., CHANG C. F., CHEN Y. H., CHENG S., Appl. Catal. B, 31 (2001), 241.
- [24] YUAN S., SHENG Q. R., ZHANG J. L., Microporous Mesoporous Mater., 110 (2008), 501.
- [25] FAN X. X. et al., J. Mol. Catal. A: Chem., 284 (2008), 155.
- [26] HUANG J. H. et al., Microporous Mesoporous Mater., 110 (2008), 543.
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-7f56650d-d5b1-4e38-a990-1060267d658d