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A methodology to determine the full energy peak efficiency (FEPE) for precise gamma spectrometry measurements of environmental samples with high-purity germanium (HPGe) detector, valid when this efficiency depends on the energy of the radiation E, the height of the cylindrical sample H, and its density ρ is introduced. The methodology consists of an initial calibration as a function of E and H and the application of a self-attenuation factor, depending on the density of the sample ρ, in order to correct for the different attenuation of the generic sample in relation to the measured standard. The obtained efficiency can be used in the whole range of interest studied, E = 120–2000 keV, H = 1–5 cm, and ρ = 0.8–1.7 g/cm3, being its uncertainty below 5%. The efficiency has been checked by the measurement of standards, resulting in a good agreement between experimental and expected activities. The described methodology can be extended to similar situations when samples show geometric and compaction differences.
Czasopismo
Rocznik
Tom
Strony
47--59
Opis fizyczny
Bibliogr. 17 poz., rys.
Twórcy
autor
- Group of Environmental Radioactivity, Applied Physics Department, CEIMAR, University of Cadiz, Avda. Rep. Saharaui s/n, Puerto Real 11510, Cádiz, Spain, Tel.: +34 956 483 419, Fax: +34 956 015 101
autor
- Group of Environmental Radioactivity, Applied Physics Department, CEIMAR, University of Cadiz, Avda. Rep. Saharaui s/n, Puerto Real 11510, Cádiz, Spain, Tel.: +34 956 483 419, Fax: +34 956 015 101
autor
- Group of Environmental Radioactivity, Applied Physics Department, CEIMAR, University of Cadiz, Avda. Rep. Saharaui s/n, Puerto Real 11510, Cádiz, Spain, Tel.: +34 956 483 419, Fax: +34 956 015 101
autor
- Group of Environmental Radioactivity, Applied Physics Department, CEIMAR, University of Cadiz, Avda. Rep. Saharaui s/n, Puerto Real 11510, Cádiz, Spain, Tel.: +34 956 483 419, Fax: +34 956 015 101
Bibliografia
- 1. Debertin, K., & Helmer, R. G. (1988). Gamma and X-ray spectrometry with semiconductor detectors. Amsterdam: Elsevier Science Ltd.
- 2. Knoll, G. F. (2010). Radiation detection and measurement (4th ed.). New York: John Wiley & Sons. 3. Casas-Ruiz, M., Ligero, R. A., & Barbero, L. (2012). Estimation of annual effective dose due to natural and man-made radionuclides in the metropolitan area of the Bay of Cadiz (SW of Spain). Radiat. Prot. Dosim., 150(1), 60–70.
- 4. Ligero, R. A., Casas-Ruiz, M., Barrera, M., Barbero, L., & Meléndez, M. J. (2010). An alternative radiometric method for calculating the sedimentation rates: Application to an intertidal region (SW of Spain). Appl. Radiat. Isot., 68, 1602–1609.
- 5. Ligero, R. A., Barrera, M., & Casas-Ruiz, M. (2005). Levels of 137Cs in muddy sediments of the seabed of the Bay of Cádiz, Spain. Part I: Vertical and spatial distribution of activities. J. Environ. Radioact., 80, 75–86.
- 6. Ligero, R. A., Barrera, M., & Casas-Ruiz, M. (2005). Levels of 137Cs in muddy sediments on the seabed in the Bay of Cádiz, Spain. Part II: Model of vertical migration of 137Cs. J. Environ. Radioact., 80, 87–103.
- 7. International Organization for Standardization. (1995). Guide to the expression of uncertainty in measurement. Geneva, Switzerland: ISO.
- 8. Bolívar, J. P., García-Tenorio, R., & García-León, M. (1994). A generalized transmission method for gamma-efficiency determination in soil samples. Nucl. Geophys., 8(5), 485–492.
- 9. Zikovsky, L. (1997). Variation of the detection efficiency of a Ge detector with the height of the sample in Marinelli beaker. J. Radioanal. Nucl. Chem., 224, 171–172.
- 10. Hubbell, J. H., & Seltzer, S. M. (1995). Tables of x-ray mass attenuation coefficients and mass energyabsorption coefficients 1 keV to 20 MeV for elements Z = 1 to 92 and 48 additional substances of dosimetric interest. Gaithersburg, MD: National Institute of Standards and Technology (NISTIR 5632). Available from http://physics.nist.gov/xaamdi.
- 11. Kitto, M. E. (1990). Mass attenuation coefficients of size-fractioned soil. J. Radioanal. Nucl. Chem.-Lett., 145(3), 175–182.
- 12. Cutshall, N. H., Larsen, I. L., & Olsen, C. R. (1983). Direct analysis of 210Pb in sediment samples: Selfabsorption correction. Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms, 206, 309–312.
- 13. Galloway, R. B. (1991). Correction for sample selfabsorption in activity determination by gamma spectrometry. Nucl. Instrum. Methods Phys. Res. Sect. AAccel. Spectrom. Dect. Assoc. Equip., 300(2), 367–373.
- 14. Haase, G., Tait, D., & Wiechen, A. (1993). Monte Carlo simulation of several gamma-emitting source and detector arrangements for determining corrections of self-attenuation and coincidence summation in gamma-spectrometry. Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip., 329(3), 483–492.
- 15. Pham, M. K., Sanchez-Cabeza, J. A., Povinec, P. P., Andor, K., Arnold, D., Benmansour, M., Bikit, I., Carvalho, F. P., Dimitrova, K., Edrev, Z. H., Engeler, C., Fouche, F. J., Garcia-Orellana, J., Gasco, C., Gastaud, J., Gudelis, A., Hancock, G., Holm, E., Legarda, F., Ikaheimonen, T. K., Ilchmann, C., Jenkinson, A. V., Kanisch, G., Kis-Benedek, G., Kleinschmidt, R., Koukouliou, V., Kuhar, B., LaRosa, J., Lee, S. -H., LePetit, G., Levy-Palomo, I., Liong Wee Kwong, L., Llaurado, M., Maringer, F. J., Meyer, M., Michalik, B., Michel, H., Nies, H., Nour, S., Oh, J. -S., Oregioni, B., Palomares, J., Pantelic, G., Pfi tzner, J., Pilvio, R., Puskeiler, L., Satake, H., Schikowski, J., Vitorovic,G., Woodhead, D., & Wyse, E. (2008). A new Certified Reference Material for radionuclides in Irish Seasediment (IAEA-385). Appl. Radiat. Isot., 66(11), 1711–1717.
- 16. Shakhashiro, A., Gondin da Fonseca Azeredo, A. M., Sansone, U., & Fajgelj, A. (2007). Matrix materials for proficiency testing: optimization of a procedure for spiking soil with gamma-emitting radionuclides. Anal. Bioanal. Chem., 387(7), 2509–2515.
- 17. Canberra Industries. (2013). Model S574 LabSOCS calibration software. Meriden CT, USA: Canberra Industries Inc. Available from http://www.canberra.com/products/insitu_systems/pdf/ISOCS-SSC40166.pdf.
Uwagi
PL
Opracowanie ze środków MNiSW w ramach umowy 812/P-DUN/2016 na działalność upowszechniającą naukę (zadania 2017).
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-6a2507e2-524f-4eea-9847-3049872a105c