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A comparison of uranium recovery from low-grade ore by bioleaching and acid leaching

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Warianty tytułu
Języki publikacji
EN
Abstrakty
EN
The objective of this work was to compare the bioleaching with the acid leaching of uranium under similar process conditions within 65 days. The low-grade uranium ore used in the experiments was collected from Radoniow’s ‘small’ dump, Poland. Bioleaching and acid leaching studies were carried out in identical columns. The isolated bacterial consortium from the Radoniow’s mine was used for the bioleaching process. A solution of sulphuric acid and H2O2 as oxidizing agent was used for the acid leaching. The extraction of uranium under acid leaching conditions reached maximum of 64±13 % w/w after 31 days. The bioleaching of uranium achieved a maximum extraction of 75±15 % w/w after 55 days. In this study an attempt was made to demonstrate the relationship between the shrinking-core model and the experimental data by plotting the fractional conversion of uranium against time.
Rocznik
Strony
136--149
Opis fizyczny
Bibliogr. 35 poz., rys., tab.
Twórcy
  • Institute of Nuclear Chemistry and Technology, Dorodna 16 Street, 03-195 Warsaw, Poland
  • Institute of Nuclear Chemistry and Technology, Dorodna 16 Street, 03-195 Warsaw, Poland
Bibliografia
  • ABHILASH, PANDEY B.D., 2013, Microbially assisted leaching of uranium – a review, Mineral Processing and Extractive Metallurgy Review: An International Journal, 34 (2), 81-113.
  • ABHILASH, PANDEY B.D., NATARAJAN K.A., 2015, Microbiology for minerals, metals, materials and the environment, CRC Press Taylor & Francis Group.
  • ABZALOV M.Z., 2012, Sandstone-hosted uranium deposits amenable for exploitation by in situ leaching, Technologies Applied Earth Science, 121 (2), 55-64.
  • ASLAM K.M., ASLAM M., 1970, Bacteria aided water leaching of uranium ores, Nucleus (Karachi), 7 (1-2), 28-36.
  • BARANSKA J.A., SADOWSKI Z., 2013, Bioleaching of uranium minerals and biosynthesis of UO2 nanoparticles, Physicochemical Problems of Mineral Processing, 49(1), 71-79.
  • BHARGAVA S.K., RAM R., POWNCEBY M., GROCOTT S., RING B., TARDIO J., JONES L., 2015, A review of acid leaching of uraninite, Hydrometallurgy, 151, 10-24.
  • BOSECKER K., 1997, Bioleaching: metal solubilization by microorganisms, Federal Institute for Geosciences and Natural Resources (BGR), Hannover (Germany), FEMS Microbiology Reviews, 20, 591-604.
  • BURES J., PETRAN M., ZACHAR J., 1967, Electrophysiological Methods in Biological Research, Third edition, Academia Publishing House of the Czechoslovak Academy of Sciences Praue, Academic Press New York and London, New York, 735-736.
  • CHAJDUK E., BARTOSIEWICZ I., PYSZYNSKA M., CHWASTOWSKA J., POLKOWSKA-MOTRENKO H., 2013, Determination of uranium and selected elements in Polish dictyonema shales and sandstones by ICP-MS, Journal of Radioanalytical and Nuclear Chemistry, 295, 1913-1919.
  • CHMIELEWSKI A.G., WAWSZCZAK D., BRYKAŁA M., 2016, Possibility of uranium and rare metal recovery in the Polish copper mining industry, Hydrometallurgy 159, 12-18.
  • DOMANSKA-SIUDA J., 2010, New data on secondary uranium minerals from the Western Sudetes (Poland) - preliminary report, Mineralogy Special Papers, 37, 77.
  • DREWNIAK L., 2014, Uranium storages in the Sudety Mountains – high ionizing radiation and its limitation, Nuclear safety and radiation protection (in Polish: Bezpieczeństwo Jądrowe i Ochrona Radiologiczna), National Atomic Energy Agency, 4 (in Polish).
  • EASTAUGH N., WALSH V., CHAPLIN T., SIDDALL R., 2008, Pigment Compendium, A Dictionary and Optical Microscopy of Historical Pigments, ISBN: 978-0-7506-8980-9, Elsevier.
  • FRACKIEWICZ K., KIEGIEL K., HERDZIK-KONIECKO I., CHAJDUK E., ZAKRZEWSKA-KOLTUNIEWICZ G., WOLKOWICZ S., CHWASTOWSKA J., BARTOSIEWICZ I., 2012, Extraction of uranium from low-grade Polish ores: dictyonemic shales and sandstones, Nukleonika, 58 (4), 451-459.
  • GAJDA D., KIEGIEL K., ZAKRZEWSKA-KOLTUNIEWICZ G., CHAJDUK E., BARTOSIEWICZ I., WOLKOWICZ S., 2015, Mineralogy and uranium leaching of ores from Triassic Peribaltic sandstones, Journal of Radioanalytical and Nuclear Chemistry, 303, 521-529.
  • GHORBANI Y., BECKER M., MAINZA A.N., FRANZIDIS J-P., PETERSEN J., 2011, Large particle effect in chemical/biochemical heap leach processes - A review, Minerals Engineering, 24, 1172-1184.
  • HABASHI F., 1999, Kinetics of Metallurgical Processes. Department of Mining and Metallurgy, Laval University, Quebec City.
  • HAMIDIAN H., 2011, Microbial Leaching of Uranium Ore, Nuclear Power-Deployment, Operation and Sustainability, ISBN: 978-953-307-474-0, InTech.
  • HUNTER E., 2013, On the leaching behavior of uranium – bearing resources in carbonate bicarbonate solution by gaseous oxidants, Faculty and the Board of Trustees of the Colorado School of Mines, USA, PhD thesis?
  • JASKOLSKI S., 1967a, Polymetallic oxide and sulphide mineralization in gneissose granites of the Izera Mountains (Lower Silesia) and its origin, Geological Review (in Polish: Przegląd Geologiczny), 43, 7–78 (in Polish with English summary).
  • JASKOLSKI S., 1967b, Polymetallic mineralization in gneissose granites at Radoniów, Geological Review (in Polish: Przegląd Geologiczny), 15, 238–239 (in Polish with English summary).
  • KACZMAREK, A., 1959, Uranium potential of the Izera Mts., Unpublished industrial report. Archiv of the AGH University of Science and Technology, Cracow, 54–160 (in Polish).
  • KACZMAREK L., 1959, Uranium potential of the Karkonosze Granite and its eastern envelope, Unpublished industrial report. Archiv of the AGH University of Science and Technology, Cracow, 15-48 (1959) (in Polish).
  • LEVENSPEL O., 1999, Chemical Reaction Engineering, 3rd Edition, Wiley, New York.
  • MISHRA A., PRADHAN N., KAR R.N., SUKLA L.B., MISHRA B.K., 1997, Microbial recovery of uranium using native fungal strains, FEMS Microbiology Reviews, 20 (3-4), 591-604.
  • MISHRA A., PRADHAN N., KAR R.N., SUKLA L.B., MISHRA B.K., 2009, Microbial recovery of uranium using native fungal strains, Hydrometallurgy, 95, 175-177.
  • MUNOZ J.A., GONZALEZ F., BALLESTER A., BLAZQUEZ M.L., 1993, Bioleaching of Spanish uranium ore, FEMS Microbiology Reviews, 11, 109-120.
  • MUNOZ J.A., BLAZQUEZ M.L., BALLESTER A., GONZALEZ F., 1995, A study of the bioleaching of a Spanish uranium ore. Part III: Column experiments, Hydrometallurgy, 38, 79-97.
  • OTHUSITSE N., MUZENDA E., 2015, Predictive Models of Leaching Processes: A Critical Review, 7th International Conference on Latest Trends in Engineering & Technology (ICLTET'2015), Irene, Pretoria (South Africa).
  • PIESTRZYNSKI A., PIECZONKA J., MIELNICZUK W., CHRUSCIEL E., JODLOWSKI P., 1996, Effects of uranium mining on the contamination of some areas in Poland, in: Planning for environmental restoration of radioactively contaminated sites in central and eastern Europe, Volume 1; Identification and characterization of contaminated sites, IAEA-Vienna, TECDOC-865, 193-216.
  • QUI G., LI Q., YU R., SUN Z., LIU Y., CHEN M., YIN H., ZHANG Y., LIANG Y., XU L., SUN L., LIU X., 2011, Column bioleaching of uranium embedded in granite porphyry by a mesophilic acidophilic consortium, Bioresource Technology, 102, 4697-4702.
  • REWERSKI B., MIELNICKA S., BARTOSIEWICZ I., POLKOWSKA-MOTRENKO H., SKŁODOWSKA A., 2013, Uranium post-mining wastes as a potential reserve source of uranium for nuclear energy plants, Physicochemical Problems of Mineral Processing, 49 (1), 5-11.
  • SILVERMAN M.P., LUNDGREN D.G., 1959, Studies on the chemoautotrophic iron bacterium Ferrobacillus Ferrooxidans II, Manometric Studies, Bacteriol, 78(3), 326-331.
  • TIAN J., CHI R., YIN J., 2010, Leaching process of rare earths from weathered crust elution-deposited rare earth ore, Transactions of Nonferrous Metals Society of China, 20, 892-896.
  • WAWSZCZAK D., DEPTULA A., ŁADA W., SMOLINSKI T., OLCZAK T., BRYKALA M., WOJTOWICZ P., ROGOWSKI M., MIŁKOWSKA M., CHMIELEWSKI A.G., 2014, Studies of leaching of copper ores and flotation wastes, Journal of Radioanalytical and Nuclear Chemistry, 300 (1), 243-247.
Uwagi
Opracowanie ze środków MNiSW w ramach umowy 812/P-DUN/2016 na działalność upowszechniającą naukę (zadania 2017).
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-688c026c-3883-4f63-8f7b-43e538402680
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