Influence of the rigid alumina particles added to ZrO₂ ceramics stabilized with Y₂ O₃ for its mechanical properties

• Autorzy: Boniecki Marek , Gołębiewski Przemysław , Węglarz Helena , Piątkowska Anna , Romaniec Magdalena , Krzyżak Konrad

Identyfikatory

DOI

10.34769/g9x6-7e09

Warianty tytułu

PL

Wpływ sztywnych korundowych cząstek dodawanych do ceramiki ZrO₂ stabilizowanej Y₂ O₃ na jej właściwości mechaniczne

• Języki publikacji: EN

Abstrakty

EN

The effect of the phase added to ZrO₂ ceramics on its mechanical properties, and in partcular on the fracture toughness, was examined using the example of Al₂ O₃ - ZrO₂ composite where ZrO₂ was stabilized with 3 mol% of Y_2O3 . Composites of 20% wt. Al₂ O₃ - 80 wt.% ZrO₂ with different size of corundum grain were made. Vickers indenter crack resistance tests showed an increase of 21% in the value of this parameter for the samples with Al₂ O₃ grains of approx. 6.5 μm in comparison with pure ZrO₂ ceramics. On the basis of literature data and microscopic observations, authors present a thesis that this increase is caused by two factors, i.e. the increase of the phase transition range (from tetragonal to monoclinic phase) accompanying crack propagation and the effect of large Al₂ O₃ grains as bridges fastening the fracture surfaces.

PL

Wpływ fazy dodawanej do ceramiki ZrO₂ na jej właściwości mechaniczne w tym głównie na jej odporność na pękanie zbadano na przykładzie kompozytu Al₂ O₃ – ZrO₂ gdzie ZrO₂ było stabilizowane 3% mol Y₂ O₃ . Wykonano kompozyty 20% wag. Al₂ O₃ – 80% wag. ZrO₂ różniące się wielkością ziarna korundowego. Badania odporności na pękanie prowadzone metodą wgłębnika Vickersa wykazały wzrost wielkości tego parametru o 21% dla próbek z ziarnami Al₂ O₃ o wielkości ok. 6,5 µm w porównaniu z czystą ceramiką ZrO₂ . Na podstawie danych literaturowych oraz własnych obserwacji mikroskopowych postawiono tezę, że wzrost ten spowodowany jest przez dwa czynniki tj. zwiększenie się zakresu przemiany fazowej (z fazy tetragonalnej do jednoskośnej) towarzyszącej propagacji pęknięcia oraz działaniem dużych ziaren Al₂ O₃ jako mostków spinających powstające powierzchnie przełamu.

Słowa kluczowe

EN

ZrO2; ceramics; Y2O3; ceramic additives with a large Young's modulus; Al2O3 grain sizes; fracture toughness, bending strength

PL

ceramika; ZrO2; Y2O3; dodatki ceramiczne o dużym module Younga; wielkość ziaren Al2 O3; odporność na pękanie; wytrzymałość na zginanie

• Wydawca: Sieć Badawcza Łukasiewicz - Instytut Technologii Materiałów Elektronicznych
• Czasopismo: Materiały Elektroniczne
• Rocznik: 2019
• Tom: T. 47, nr 1-4
• Strony: 4--13
• Opis fizyczny: Bibliogr. 44 poz., rys., tab.

Twórcy

autor

Boniecki Marek

• Łukasiewicz Research Network - Institute of Electronic Materials Technology, 133 Wólczyńska Str., 01-919 Warsaw

autor

Gołębiewski Przemysław

• Łukasiewicz Research Network - Institute of Electronic Materials Technology, 133 Wólczyńska Str., 01-919 Warsaw

autor

Węglarz Helena

• Łukasiewicz Research Network - Institute of Electronic Materials Technology, 133 Wólczyńska Str., 01-919 Warsaw

autor

Piątkowska Anna

• Łukasiewicz Research Network - Institute of Electronic Materials Technology, 133 Wólczyńska Str., 01-919 Warsaw

autor

Romaniec Magdalena

• Łukasiewicz Research Network - Institute of Electronic Materials Technology, 133 Wólczyńska Str., 01-919 Warsaw

autor

Krzyżak Konrad

• Łukasiewicz Research Network - Institute of Electronic Materials Technology, 133 Wólczyńska Str., 01-919 Warsaw

Bibliografia

• [1] Okada A.: Automotive and industrial applications of structural ceramics in Japan, J.Eur.Ceram.Soc., 2008, 28, 1097-1104.
• [2] Okada A.: Ceramic technologies for automotive industry: Current status and perspectives, Mater.Sci.Eng.B, 2009, 161, 182-187.
• [3] Manicone FP.F., Iommetti P.R., Raffaelli L.: An overview of zirconia ceramics: Basic properties and clinical applications, J.of Dentistry, 2007, 35, 819-826.
• [4] Krell A., Hutzler T., Klimke J. : Transmission physics and consequences for materials selection, manufacturing, and applications, J.Eur.Ceram.Soc., 2009, 29, 207-221.
• [5] Wiederhorn S.M.: Subcritical crack growth in ceramics, in Fracture Mechanics of Ceramics, v.2 ed. By Bradt R.C., Hasselman D.P.H., Lange F.F., Plenum Press, New York, London, 1974, 613-646.
• [6] Konopka K., Maj M., Kurzydłowski J.K.: Studies of the effect of metal particles on the fracture toughness of ceramic matrix composites, Materials Characterization, 2003, 51, 5, December, 335-340.
• [7] Ostertag C.P.: Influence of fiber and grain bridging on crack profiles in SiC fiber-reinforced alumina-matrix composites, Mater.Sci.Eng. A, 1999, 260, 124-131.
• [8] Bocanegra-Bernal M.H., Echeberia J., Ollo J.,et al.: A comparison of the effects of multi-wall and single- -wall carbon nanotube additions on the properties of zirconia toughened alumina composites, Carbon, 2011, 49, 5, 1599-1607.
• [9] Boniecki M., Gołębiewski P., Wesołowski W., et al.: Alumina/zirconia composites toughened by the addition of graphene flakes, Ceram. Int., 2017, 43, 10066-10070.
• 10] Liu J., Yan H., Reece M.J., Jiang K.: Toughening of zirconia/alumina composites by the addition of graphene platelets, J.Eur.Ceram.Soc., 2012, 32, 4185-4193.
• [11] Shin J-H., Hong S-H.: Fabrication and properties of reduced graphene oxide reinforced yttria-stabilized zirconia composite ceramics, J.Eur.Ceram.Soc., 2014, 34, 1297-1302.
• [12] Fei Ch., Jin D., Tyeb K., et al.: Field assisted sintering of graphene reinforced zirconia ceramics, Ceram.Int., 2015, 41, 6113-6116.
• [13] Li J-F., Watanabe R.: Fracture toughness of Al2 O3 - particle-dispersed Y2 O3 - partially stabilized zirconia, J.Am.Ceram.Soc., 1995, 78, 1079-1082.
• [14] Lee J-K., Kim M-J., Lee E-G.: Influence of dispersed- -alumina particle size on the fracture toughness of 3 mol% yttria-stabilized zirconia polycrystals (3Y-TZP), J.Mater.Sci.Lett., 2002, 21, 259-261.
• [15] Vleugels J., Van der Biest O.: Development and characterization of Y2 O3 – stabilized ZrO2 (Y-TZP) composites with TiB2 , TiN, TiC, and TiC0.5N0.5, J.Am. Ceram.Soc., 1999, 82 [10] 2717 – 2720.
• [16] Basu B., Vleugels J., Van der Biest O.: Processing and mechanical properties of ZrO2 – TiB2 composites, J.Eur.Ceram.Soc., 2005, 25, 3629-3637.
• [17] Haberko K., Pędzich Z. Róg G., Bućko M.M., Faryna M.: The TZP matrix-WC particulate composites, Eur.J.Solid State Inorg. Chem., 1995, 32, 593-601.
• [18] Pędzich Z., Haberko K.: Toughening mechanism in the TZP - WC particulate composites, Key Eng.Mater., 1997, 132-136, 2076-2079.
• [19] Pędzich Z., Haberko K., Piekarczyk J., Faryna M., Lityńska L.: Zirconia matrix-tungsten carbide particulate composites manufactured by hot-pressing technique, Mater. Lett., 1998, 70-75.
• [20] Pędzich Z.: The reliability of particulate composites in the TZP/WC system, J.Eur.Ceram.Soc., 2004, 24, 3427-3430.
• [21] Pędzich Z.: Fracture of oxide matrix composites with different phase arrangement, Key Eng. Mater., 2009, 409, 244-251.
• [22] Pędzich Z.: Tungsten Carbide as an reinforcement in structural oxide-matrix composites, INTECH open science/open minds, chapter 4 (Tungsten Carbide - Processing and Applications), (2012), 81-102, (http:// dx.doi.org/10.5772/51183).
• [23] Űnal N., Kern F., Ővecoglu M.L., Gadow R.: Influence of WC particles on the microstructural and mechanical properties of 3 mol % Y2 O3 stabilized ZrO2 matrix composites produced by hot pressing, J.Eur.Ceram.Soc., 2011, 31, 2267- 2275.
• [24] Bamba N., Choa Y-Ho, Sekino T., Niihara K.: Mechanical properties and microstructure for 3 mol% yttria doped zirconia/silicon carbide nanocomposites, J.Eur.Ceram.Soc., 2003, 23, 773-780.
• [25] Zhan G.-D., Lai T.-R., Shi J.-L., Yen T.-S., Zhou Y. Zhang Y.: Microstructure and mechanical properties of yttria-stabilized tetragonal zirconia polycrystals containing dispersed TiC particles, J.Mater.Sci., 1996, 31, 2903-2907.
• [26] Stevens R.: Zirconia and zirconia ceramics. Introduction to zirconia. Magnesium Electron Publication. 113, July (1986), 56 pages.
• [27] Cutler R.A., Reynolds J.R., Jones A.: Sintering and characterization of polycrystalline monoclinic, tetragonal and cubic zirconia, J.Am.Ceram.Soc., 1992, 73[8], 2173-2183.
• [28] Govila R.K.: Strength characterization of yttria- -partially stabilized zirconia, J.Mater.Sci., 1995, 30, 2656-2667.
• [29] Anstis G.R, Chantikul P., Lawn B.R., Marchall D.B.: A critical evaluation of indentation techniques for fracture toughness, J.Am.Ceram.Soc., 1981, 64, 533-538.
• [30] Niihara K.: A fracture mechanics analysis of indentation-induced Palmqvist crack in ceramics, J.Mater. Sci. Lett., 1983, 2, 221-223.
• [31] Boniecki M.: unpublished data, 2018.
• [32] Bozkurt F., Schmidova E.: Fracture toughness evaluation of S355 steel using circumferentialy notched round bars, Periodica Polytechnica Transportation Engineering, 2018, 1-5, https://doi.org/10.3311/PPtr.11560.
• [33] Munro R.G.: Evaluated material properties for a sintered α – alumina, J.Am.Ceram.Soc., 1997, 80 (8), 1919-1928.
• [34] https://accuratus.com/silicar.html.
• [35] Vallauri D., Adrian I.C.A., Chrysanthou A.: TiC – TiB2 composites: A review of phase relationships, processing and properties, J. Eur.Ceram. Soc., 2008, 28, 1697 – 1713.
• [36] Małek O., Lauwers B., Perez Y., De Baets P., Vleugels J.: Processing of ultrafine ZrO2 toughened WC composites, J.Eur. Ceram.Soc., 2009, 29, 3371-3378.
• [37] Selsing J.: Internal stresses in ceramics, J.Am.Ceram. Soc., 1961, 44,419.
• [38] Budiansky B., Hutchinson J.W., Lambropoulus J.C.: Continuum theory of dilatant transformation toughening in ceramics, Int.J.Solids Struct., 1983, 19, 337-355.
• [39] Evans A.G., Cannon R.M.: Toughening of brittle solids by martensitic transformation, Acta Metall., 986, 34, 761-800.
• [40] PN-EN ISO 15732, October 2007. Fine ceramics (advanced ceramics, advanced technical ceramics). Test method for fracture thoughness of monolithic ceramics at room temperature by single edge precracked beam (SEPB) method (ISO 15732:2003) (Eq. 8).
• [41] Chantikul P., Anstis G.R., Lawn B.R, Marshall D.B.: A critical evaluation of indentation techniques for measuring fracture toughness: II, Strength method, J.Am.Ceram.Soc., 1981, 64 [9], 539-543.
• [42] PN – EN 843-1, December 2007. Advanced technical ceramics - Monolithic ceramics - Mechanical properties at room temperature - Part 1: Determination of flexural strength.
• [43] PN-EN 843-2, December 2007. Advanced technical ceramics - Monolithic ceramics - Mechanical properties at room temperature - Part 2: Determination of the Young's modulus, shear modulus and Poisson's ratio.
• [44] Boniecki M., Gołębiewski P., Wesołowski W. i inni: Kompozyt Al2 O3 -ZrO2 wzmocniony płatkami grafenowymi/Al2 O3 -ZrO2 composite reinforced with graphene platelets, Materiały Elektroniczne/Electronic Materials, 2016, 44, 1, 20-28.

Uwagi

PL

Opracowanie rekordu ze środków MNiSW, umowa Nr 461252 w ramach programu "Społeczna odpowiedzialność nauki" - moduł: Popularyzacja nauki i promocja sportu (2020).