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Comparison of beta (LSC) and gamma (HPGe) spectrometric methods for lead-210 in chronological study

Identyfikatory
Warianty tytułu
Konferencja
Conference Proceedings of the 12th International Conference “Methods of Absolute Chronology” May 11-13th, 2016, Gliwice-Paniówki, Poland
Języki publikacji
EN
Abstrakty
EN
The sediments of two lakes located in the Baltic Uplands, the western part of the East European Plain (East Lithuania and North East Poland), were studied. Activity concentration of 210Pb was determined using two nuclear analytical techniques: determination of 210Pb in equilibrium with its beta emitting daughter 210Bi using liquid scintillation counter (LSC), and direct determination of 210Pb (and other radionuclides) by low-background gamma-ray spectrometer with a well type HPGe detector. For the 210Pb determination by LSC the methodology of lead separation based on the anion exchange resin in Cl– form (Eichrom) was used. Several steps of radiochemical procedures and respective parameters were investigated additionally. The optimized procedures for LSC method were used for case study with two lake cores. The activity concentration of 210Pb in lake sediment samples based on both nuclear analytical techniques (LSC and HPGe) were compared. 210Pb dating of cores was performed according to Constant Rate of 210Pb Supply (CRS) model with some modifications. Both techniques in the range of uncertainties gave similar results. From two considered lakes, the more eutrophic one exhibited higher sediment mass accumulation rate (MAR) values.
Wydawca
Czasopismo
Rocznik
Strony
34--43
Opis fizyczny
Bibliogr. 36 poz., rys.
Twórcy
  • Laboratory of Nuclear Geophysics and Radioecology, State Research Institute Nature Research Centre, Akademijos str. 2, Vilnius, Lithuania
autor
  • Laboratory of Nuclear Geophysics and Radioecology, State Research Institute Nature Research Centre, Akademijos str. 2, Vilnius, Lithuania
  • Laboratory of Nuclear Geophysics and Radioecology, State Research Institute Nature Research Centre, Akademijos str. 2, Vilnius, Lithuania
  • Department of Geomorphology, Faculty of Geography and Regional Studies, University of Warsaw, Krakowskie Przedmiescie 30, 00-927 Warsaw, Poland
Bibliografia
  • 1. Appleby PG, 2001. Chronostratigraphic techniques in recent sediments. In: Last WL and Smol JP, Eds., Tracking environmental changes using lake sediments. Volume 1:Basin analysis, coring and chronological techniques, development in paleoenvironmental research. Kluwer Academic Publishers, 576.
  • 2. Appleby PG, Richardson N and Nolan PJ, 1991. 241Am dating of lake sediments. Hydrobiologia214: 35–42, .
  • 3. Appleby PG and Oldfield F, 1978. The calculation of lead-210 dates assuming a constant rate of supply of unsupported 210Pb to the sediment. Catena5: 1–8.
  • 4. Barlas Simsek F and Cagatay MN, 2014. Geochronology of lake sediments using 210Pb with double energetic window method by LSC: an application to Lake Van. Applied Radiation and Isotopes93: 126–133, .
  • 5. Begy RC, Timar-Gabor A, Somlai J and Cosma C, 2011. A sedimentation study of St. Ana Lake (Romania) applying the 210Pb and 137Cs dating methods. Geochronometria38(2): 93–100, .
  • 6. Bhatki KS, 1977. The radiochemistry of bismuth. National Research Council Report, NAS-NS-3057. Washington D.C.: National Academy of Sciences, 151.
  • 7. Dušauskiene-Duž R, 1997. Ecological and geochemical role of radionuclides (90Sr and 210Pb) in Lake Druksiai ecosystem – water cooler of the Ignalina NPP (Lithuania). Environmental Physics19(2): 11–19.
  • 8. Ebaid YY and Khater AE, 2006. Determination of 210Pb in Environmental Samples. Journal of Radioanalytical and Nuclear Chemistry270(3): 609–619, .
  • 9. Farmer JG, Graham MC, Yafa C, Cloy JM, Freeman AJ and MacKenzie AB, 2006. Use of 206Pb/207Pb ratios to investigate the surface integrity of peat cores used to study the recent depositional history and geochemical behaviour of inorganic elements in peat bogs. Global Planetary Change53: 240–248, .
  • 10. Figgins PE, 1961. The Radiochemistry of Polonium. National Research Council Report, NAS-NS-3037. Washington D.C.: National Academy of Sciences, 74.
  • 11. Gibson WM, 1961. The Radiochemistry of Lead. National Research Council Report, NAS-NS-3040. Washington D. C.: National Academy of Science,160.
  • 12. Goldberg ED, 1963. Geochronology with 210Pb in radioactive dating. IAEA Contribution1510: 121–131.
  • 13. Happel S, Le Berre M, Johanson L and Bombard A, 2006. Validation of an Improved Method for the Separation and Measurement of Pb-210 and Po-210. Users Group Meeting, Bratislava - Slovakia, 10th November 2006.
  • 14. Jia G, Belli M, Blasi M, Marchetti A, Rosamilia S and Sansone U, 2001. Determination of 210Pb and 210Po in Mineral and Biological Environmental Samples. Journal of Radioanalytical and Nuclear Chemistry247(3): 491–499, .
  • 15. Jia G, Belli M, Liu S, Sansone U, Xu C, Rosamilia S, Xiao X, Gaudino S, Ching L and Yang H, 2006. The fractional and determination procedures for the speciation of 210Pb and 210Po in soil samples. Analytica Chimica Acta562: 51–58.
  • 16. Jia G and Torri G, 2007. Determination of 210Pb and 210Po in Soil or Rock Samples Containing Refractory Matrices. Applied Radiation and Isotopes65: 1–8, .
  • 17. Kim CK, Martin P and Fajgelj A, 2008. Quantification of measurement uncertainty in the sequential determination of 210Pb and 210Po by liquid scintillation counting and alpha-particle spectrometry. Accreditation and Quality Assurance13(12): 691–702, .
  • 18. Krishnaswami S, Lal D, Martin JM and Meybeck M, 1971. Geochronology of lake sediments. Earth and Planetary Science Letters11: 407–14, .
  • 19. Krzywicki T, Smolska E and Szwarczewski P, 2007. Etapy rozwoju sandru olecko-rajgrodzkiego na tle faz recesyjnych zlodowacenia Wisly w nawiązaniu do wybranych cech strukturalnoteksturalnych osadów (Stages development of Olecko-Rajgrod outwash - relation to vistula glacier recession marginal limits and structural and textural features of the sediments).Słupskie Prace Geograficzne4: 79–92 (in Polish).
  • 20. Koide M, Soutar A and Goldberg ED, 1972. Marine geochronology with 210Pb. Earth and Planetary Science Letters14(3): 442–446, .
  • 21. Lehto J and Hou X, 2011. Chemistry and Analysis of Radionuclides. John Wiley & Sons, New York: 426.
  • 22. Lozano JC, Blanco Rodriguez P, Vera Tome F and Leal-Cidoncha E, 2012. Improvement of a method for the sequential determination of 210Pb, 226Ra and uranium isotopes by LSC and alpha-particle spectrometry. Applied Radiation and Isotopes70: 609–611, .
  • 23. Mabit L, Benmansour M, Abril JM, Walling DE, Meusburger K, Iuran AR, Bernard C, Tarjan S, Owens PN, Blake, WH and Alewell C, 2014. Fallout 210Pb as a soil sediment tracer in catchment sediment budget investigations: a review. Earth-Science Reviews138: 335–351, .
  • 24. Mabit L, Benmansour M and Walling DE, 2008. Comparative advantages and limitations of the fallout radionuclides 137Cs,210Pbex and 7Be for assessing soil erosion and sedimentation. Journal of Environmental Radioactivity99: 1799–1807, .
  • 25. MacKenzie AB, Hardie SML, Farmer JG, Eades LJ and Pulford ID, 2011.Analytical and sampling constraints in 210Pb dating.Science Total Environmental409: 1298–1304, .
  • 26. Marčiulioniene D, Mažeika J, Lukšiene B, Jefanova O, Mikalauskienė R and Paškauskas R, 2015. Anthropogenic radionuclide fluxes and distribution in bottom sediments of the cooling basin of the Ignalina Nuclear Power. Journal of Environmental Radioactivity145: 48–57, .
  • 27. Mažeika J, Dušauskiene-Duž R and Radzevičius R, 2004. Sedimentation in the eastern Baltic Sea: lead-210 dating and trace element data implication. Baltica17(2): 79–92.
  • 28. O’Reilly J, Leon Vintro L, Mitchell PI, Donohue I, Leira M, Hobbs W and Irvine K, 2011. 210Pb dating of a lake sediment core from Lough Carra (Co. Mayo, western Ireland): use of paleolimnological data for chronology validation below the 210Pb dating horizon. Journal of Environmental radioactivity102: 495–499, .
  • 29. Pennington W, Cambray RS and Fisher EM, 1973. Observations on lake sediments using 137Cs fallout as a tracer. Nature242: 324–326, .
  • 30. Polikarpov GG, 1966. Radioecology of Aquatic Organisms. Reinhold, New York: xxviii+314 (in Russian).
  • 31. Smith JN, 2001. Why should we believe 210Pb geochronologies? Journal of Environmental Radioactivity55: 121–123, .
  • 32. Taner PA, Pan SM, Mao SY and Yu KN, 2000. γ-Ray spectrometric and α-counting method comparison for the determination of Pb-210 in estuarine sediments. Applied Spectroscopy54: 1443–1446, .
  • 33. Villa M, Moreno HP and Manjon G, 2005. Determination of 226Ra and 224Ra in Sediments Samples by Liquid Scintillation Counting. Radioactivity Measurements39(5): 543–550, .
  • 34. Villa M, Hurtado S, Manjon G and Garcia-Tenorio R, 2007. Calibration and measurement of 210Pb using two independent techniques. Radiation Measurements42: 1552–1560, .
  • 35. Walling DE, He Q and Appleby PG, 2002. Conversion models. In: Zapata F, eds. Handbook for the assessment of soil erosion and sedimentation using environmental radionuclides. Kluwer Academic Publishers, 111–162.
  • 36. Zaborska A, Carrol J, Papucci C and Pempkowiak J, 2007. Intercomparison of alpha and Gamma Spectrometry Techniques Used in 210Pb Geochronology. Journal of Environmental Radioactivity93: 38–50, .
Uwagi
Opracowanie rekordu w ramach umowy 509/P-DUN/2018 ze środków MNiSW przeznaczonych na działalność upowszechniającą naukę (2018).
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-52967bd1-d9a1-45a1-94ac-83dcbd90d9b9
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