Semi-quantitative analysis study of the impact of microwave treatment on fly ash

• Autorzy: Ma Xian Yun , Nie Yi Miao , Guo Jia Le , Chen Yang , Chang Zhen Jia , Wang Ling , Liu Shu Xian , Wang Long

Identyfikatory

DOI

10.37190/ppmp/174897

• Języki publikacji: EN

Abstrakty

EN

Pre-processing provides an effective way for fly ash's high value-added utilization. However, the shortcomings of pre-processing methods such as grinding and flotation are apparent with many disadvantages that make it more challenging to use efficiently. Microwave heating helps the SiO₂-Al.₂O₃ bond break, not only can make the structural change of the material can also promote the chemical reaction process. In the article, XRD, SEM, FT-IR, ammonia nitrogen adsorption, and other methods were used to analyze the changes in the properties of fly ash before and after microwave pre-treatment, the change in adsorption performance of fly ash before and after microwave treatment was analyzed. The study found that under microwave conditions of 600 W and 15 min, the adsorption rate of ammonia nitrogen by fly ash reached a maximum of 29.67%. The intensity of mullite and amorphous diffraction peaks decreased after 20 min at 600 W. The Si-O-(Si, Al) and Si-O-(Si) bonds showed significant changes at 15 min and 20 min under 600 W conditions. Based on the results, the microwave conditions were selected at 600 W for different periods, and semi-quantitative analysis was carried out by XRD-Rietveld, infrared peak fitting, and nuclear magnetic resonance. The XRD-Rietveld analysis showed that the amorphous phase content reached 46.18% at 15 min. In the infrared peak fitting, the fitting area at 1300-900 cm^-1 and 600-400 cm^-1 peaks at 56.92% at 25 min and 17.5% at 15 min, respectively. The silicon-oxygen network's degree of connection and polymerization was reduced after 15 min of microwave treatment for the nuclear magnetic resonance analysis. By combining specific surface area measurements, it was discovered that the maximum specific surface area attained a value of 3.122 m²/g at 15 min.

Słowa kluczowe

EN

microwave; fly ash; semi-quantitative analysis; adsorption; XRD refinement; infrared fitting; NMR

• Wydawca: Oficyna Wydawnicza Politechniki Wrocławskiej
• Czasopismo: Physicochemical Problems of Mineral Processing
• Rocznik: 2023
• Tom: Vol. 59, iss. 6
• Strony: art. no. 174897
• Opis fizyczny: Bibliogr. 44 poz., rys., tab., wykr.

Twórcy

autor

Ma Xian Yun

• College of Mining Engineering, North China University of Science and Technology, Tangshan 063210, China
• Hebei Province Key Laboratory of Mining Exploitation and Security Technology, Tangshan 063210, China

autor

Nie Yi Miao

• College of Mining Engineering, North China University of Science and Technology, Tangshan 063210, China
• Hebei Province Key Laboratory of Mining Exploitation and Security Technology, Tangshan 063210, China

autor

Guo Jia Le

• College of Mining Engineering, North China University of Science and Technology, Tangshan 063210, China
• Hebei Province Key Laboratory of Mining Exploitation and Security Technology, Tangshan 063210, China

autor

Chen Yang

• College of Mining Engineering, North China University of Science and Technology, Tangshan 063210, China
• Hebei Province Key Laboratory of Mining Exploitation and Security Technology, Tangshan 063210, China

autor

Chang Zhen Jia

• College of Mining Engineering, North China University of Science and Technology, Tangshan 063210, China
• Hebei Province Key Laboratory of Mining Exploitation and Security Technology, Tangshan 063210, China

autor

Wang Ling

• College of Mining Engineering, North China University of Science and Technology, Tangshan 063210, China
• Hebei Province Key Laboratory of Mining Exploitation and Security Technology, Tangshan 063210, China

autor

Liu Shu Xian

• College of Mining Engineering, North China University of Science and Technology, Tangshan 063210, China
• Hebei Province Key Laboratory of Mining Exploitation and Security Technology, Tangshan 063210, China

autor

Wang Long

• College of Mining Engineering, North China University of Science and Technology, Tangshan 063210, China
• Hebei Province Key Laboratory of Mining Exploitation and Security Technology, Tangshan 063210, China
• State Key Laboratory of Clean Utilization of Complex Nonferrous Metal Resources, Kunming 650093, China

Bibliografia

• AELST, J.V., HAOUAS, M., GOBECHIYA, E. and HOUTHOOFD, K., 2014. Hierarchization of USY Zeolite by NH4OH. A Postsynthetic Process Investigated by NMR and XRD. The Journal of Physical Chemistry, C. Nanomaterials and Interfaces, 118(39), 22573-22582.
• ALAKENT, B., KAYAÖZKIPER, K., and SOYERUZUN, S., 2022. Global interpretation and generalizability of boosted regression models for the prediction of methylene blue adsorption by different clay minerals and alkali activated materials. Chemosphere, 308(P1), 136248.
• AL-DAHRI, T., ABDULRAZAK, A., and ROHANI, S., 2022. Preparation and characterization of Linde-type A zeolite (LTA) from coal fly ash by microwave-assisted synthesis method: its application as adsorbent for removal of anionic dyes. International Journal of Coal Preparation and Utilization, 42(7).
• BERNARD, E., LOTHENBACH, B., GERMAN, A., and RENTSCH, D., 2023. Effect of aluminate and carbonate in magnesia silicate cement. Cement and Concrete Composites, 139, 105010.
• CHEN, C.Y., ZHONG, C., ZHANG, Y., and LI, A., 2022. Structural and dynamic properties of MgO–Al2O3–SiO2 glasses from molecular dynamics simulations and NMR. Ceramics International, 48(15).
• CHEN, W., SONG, G.Q., LIN, Y.Y., and QIAO, J.T., 2022. Synthesis and catalytic performance of Linde-type A zeolite (LTA) from coal fly ash utilizing microwave and ultrasound collaborative activation method. Catalysis Today, 397-399.
• DAS, D., and ROUT, P.K., 2023. A review of coal fly ash utilization to save the environment. Water, Air, & Soil Pollution, 234(2), 1-23.
• DINDI, A., DANG, V., QUANG, D.V., and VEGA, L.F., 2019. LOURDES F. Vega, R.M. Abu-Zahra. Applications of fly ash for CO2 capture, utilization, and storage. Journal of CO2 Utilization, 29, 82-102.
• EI-FEKY, M.S., KOHAIL, M., MAHER, A., and SERAG, M.I., 2020. Effect of microwave curing as compared with conventional regimes on the performance of alkali activated slag pastes. Construction and Building Materials, 233(117268).
• ELKARRACH, K., OMOR, A., ATIA, F., and LAIDI, O., 2023. Mohamed, Merzouki Mohammed. Treatment of tannery effluent by adsorption onto fly ash released from thermal power stations: Characterisation, optimization, kinetics, and isotherms. Heliyon, 9(4), e12687.
• FRANUS, M., PANEK, R., MADEJ, J., and FRANUS, W., 2019. The properties of fly ash derived lightweight aggregates obtained using microwave radiation. Construction and Building Materials, 227(116677).
• GHANI, S.M., RABAT, N.E., RAHIM, A.R.A., JOHARI, K., SIYAL, A.A., and KUMERESEN, R., 2023. ABDUL Rahim Abdul Rahman, Amine Infused, et al. Fly ash grafted acrylic acid/acrylamide hydrogel for carbon dioxide (CO2) adsorption and its kinetic analysis. Gels, 9(3).
• GOPALAN, A., RAMESH, S., NIRMALA, P., GOVINDARAJ, D.R., SAHOO, S., SHIFANI, S.A., and JAYADHAS, S. A., 2022. Investigation of insulation properties using microwave nondevastating methodology to predict the strength of polymer materials. Advances in Materials Science and Engineering, 3, 1-9.
• GULTEKIN, A. and RAMYAR, K., 2023. Investigation of high-temperature resistance of natural pozzolan-based geopolymers produced with oven and microwave curing. Construction and Building Materials, 365(2), 130059.
• HAN, Q.C., TANG, J. and LU, J.G.Z., 2003. Standard specification for fly ash and raw or calcined natural pozzolan for use as a mineral admixture in concrete (ASTMC 618). Coal Ash China, 2, 44–45.
• HOSSEINPOUR, S., MEHRIZI, M.H., HASHEMIPOUR, H., and FARPOOR, M.H., 2023. Adsorptive removal of phosphorus from aqueous solutions using natural and modified coal solid wastes. Water Science and Technology: A Journal of the International Association on Water Pollution Research, 87(6).
• IOANA, A., PAUNESCU, L., NICOLAE, C., POLLIFRONI, M., DEONISE, D., and PETCU, F.S., 2022. Glass foam from flat glass waste produced by the microwave irradiation technique. Micromachines, 13(4), 550.
• JAIN, S., BANTHIA, N., and TROCZYNSKI, T., 2022. Conditioning of simulated cesium radionuclides in NaOH-activated fly ash-based geopolymers. Journal of Cleaner Production, 380, 134984.
• KUNECKI, P., WDOWIN, M., and HANC, E., 2023. Fly ash-derived zeolites and their sorption abilities in relation to elemental mercury in a simulated gas stream. Journal of Cleaner Production, 391, 136181.
• LUO, S.Q., GE, Y.L., and PAN, C.G., 2023. Microstructures of fly ash activated by microwave and early properties of flyashcement slurry. Materials Reports, 1-17.
• LV, Y., 2018. Experience in the operation of water chemical titration. Northern Chinese Fisheries, (02), 17-19.
• MAJID, B. 2021. Application of fly ash and fine limestone powder in cement and concrete. Journal of Progress in Civil Engineering, 3(7).
• MA, P.C., LI, X., WEN, Z.Y., MENG, F.H., and LI, Z., 2021. Research progress on active excitation and mechanism of fly ash. Inorganic Chemicals Industry, 53(10), 28-35.
• MARJANOVIĆ, N., KOMLJENOVIĆ, M., BAŠČAREVIĆ, Z., and NIKOLIĆ, V., 2014. Improving reactivity of fly ash and properties of ensuing geopolymers through mechanical activation. Construction and Building Materials, 57, 151-162.
• MATHAPATI, M.K., AMATE, K., PRASAD, D., JAYAVARDHANA, M.L., and RAJU, T.H., 2021. A review on fly ash utilization. Materials Today Proceedings, 50(2).
• MA, X.Y., NIE, Y.M., CHEN, Y., LI, T., HUANG, H., LIU, S.X., WANG, L., and WANG, L., 2022. Synthesis of fly ashbased zeolite molecular sieve and research status of its structural properties. Metal Mine, (08), 82-93.
• MEDYKOWSKA, M., WIŚNIEWSKA, M., SZEWCZUK, K.K., and PANEK, R., 2022. Simultaneous removal of inorganic and organic pollutants from multicomponent solutions by the use of zeolitic materials obtained from fly ash waste. Clean Technologies and Environmental Policy, 25(3).
• MOISILI, P.E. and JEN, T.C., 2022. Microwave-assisted sol–gel template-free synthesis and characterization of silica nanoparticles obtained from South African coal fly ash. Nanotechnology Reviews, 11(1), 3042-3052.
• NGUYEN, H.T., NGUYEN, H.T., and AHMED, S.F., 2023. Emerging waste-to-wealth applications of fly ash for environmental remediation: A review. Environmental Research, 227:115800.
• NIE, Y.M., XIA, M.H., BAI, L.M., LIU, S.X., ZHANG, J.X., and NIU, F.S., 2012. Analysis method of ~(27)Al, ~(29) Si solid high-resolution nuclear magnetic resonance pattern analysis of silicon (aluminum) salt mineral crystals. Bulletin of the Chinese Ceramic Society, 31(05), 1200-1203.
• OLUYINKA, O.A., PATEL, A.V., SHAH, B., and BAGIA, M., 2020. Microwave and fusion techniques for the synthesis of mesoporous zeolitic composite adsorbents from bagasse fly ash: sorption of p-nitroaniline and nitrobenzene. Applied Water Science, 10(12).
• PANITSA, O.A., KIOUPIS, D., and KAKALI, G., 2022. Thermal and microwave synthesis of silica fume-based solid activator for the one-part geopolymerization of fly ash. Environmental Science and Pollution Research International, 29(39).
• PRAIPIPAT, P., NGAMSURACH, P., and ROOPKHAN, N., 2023. Zeolite A powder and beads from sugarcane bagasse fly ash modified with iron(III) oxide-hydroxide for lead adsorption. Scientific Reports, 13(1).
• RUSĂNESCU, C.O., and RUSĂNESCU, M., 2023. Application of fly ash obtained from the incineration of municipal solid waste in agriculture. Applied Sciences, 13(5), 3246.
• SHI, S., LI, H., ZHOU, Q. Z., ZHANG, H.Z., and BAI, Y., 2023. Alkali-activated fly ash cured with pulsed microwave and thermal oven: A comparison of reaction products, microstructure and compressive strength. Cement and Concrete Research, 166(8).
• SINGH, K., KUMAR, A., SINGH, A.K., and AGARWAL, A., 2023. Fly ash and TiO2 modified fly ash as adsorbing materials for effective removal of methylene blue and malachite green from aqueous solutions. Journal of the Indian Chemical Society, 100(3), 100942.
• TANG, T., CAI, L.X., YOU, K., and LIU, M., 2020. Effect of microwave pre-curing technology on carbide slag-fly ash autoclaved aerated concrete (CS-FA AAC): Porosity rough body formation, pore characteristics and hydration products. Construction and Building Materials, 263(29), 120112.
• UM, N. and JEON, T.W., 2021. Pretreatment method for the utilization of the coal ash landfilled in ash ponds. Process Safety and Environmental Protection, 153(9).
• VALEEV, D. and KONDRATIEV, A., 2022. Current state of coal fly ash utilization: Characterization and application. Materials, 16(1), 27.
• YAKABOYLU, G.A., BAKER, D., WAYDA, B., and SABOLSKY, K., 2019. Microwave-assisted pretreatment of coal fly ash for enrichment and enhanced extraction of rare-earth elements. Energy & Fuels, 33(11).
• YILDIZ, K., and ATAKAN, M., 2020. Improving microwave healing characteristic of asphalt concrete by using fly ash as a filler. Construction and Building Materials, 262(120448), 1-9.
• ZHANG, L.J., YUAN, H., PENG, L., PENG, J.H., LI, S.W., CHEN, K.H., YIN, S.H., ZHANG, L.B., 2020. Comparison of microwave and conventional heating routes for kaolin thermal activation. Journal of Central South University, 27, 2494-2506.
• ZHOU, Q., JIANG, X.G., QIU, Q. L., ZHAO, Y.M., and LONG, L., 2022. Ling. Synthesis of high-quality NaP1 zeolite from municipal solid waste incineration fly ash by microwave-assisted hydrothermal method and its adsorption capacity. The Science of the Total Environment, 855(8), 158741.
• ZUMA, M.C., NOMNGONGO, P.N. and MKETO, N., 2021. Simultaneous determination of REEs in coal samples using the combination of microwave-assisted ashing and ultrasound-assisted extraction methods followed by ICP-OES analysis. Minerals, 11(10), 1103.