Preparation and characterization of titania powders obtained via hydrolysis of titanium tetraisopropoxide

• Autorzy: Grzeskowiak M , Wrobel R. J. , Grzechulska J. , Przepiorski J

Identyfikatory

DOI

10.2478/s13536-013-0163-z

• Języki publikacji: EN

Abstrakty

EN

TiO2 powders were prepared through the hydrolysis of titanium isopropoxide followed by calcination at temperatures of 200 °C to 600 °C. The obtained powders were characterized by N2 adsorption-desorption and X-ray powder diffraction. The results confirmed strong dependence between specific surface area of the TiO2 powders and both the conditions of the hydrolysis process and the calcination temperature. While calcination temperature strongly affected crystallinity of the product, no significant influence of the hydrolysis conditions on this parameter was observed. TiO2 powders prepared at various conditions were examined as catalysts for photodegradation of Acid Red 18 in water. Photoactivities of the prepared powders were influenced by both the amount of water used to hydrolyze the TiO2 precursor and the temperature of calcination process. TiO2 samples calcined at 500 °C appeared to be the most active and the photocatalytic activities of the prepared materials increased along with the amount of water used for the hydrolysis process.

Słowa kluczowe

EN

titanium dioxide; titanium tetraisopropoxide; hydrolysis; photocatalysis; azo-dye

• Wydawca: De Gruyter
• Czasopismo: Materials Science Poland
• Rocznik: 2014
• Tom: Vol. 32, No. 1
• Strony: 71--79
• Opis fizyczny: Bibliogr. 44 poz., rys., tab., wykr.

Twórcy

autor

Grzeskowiak M

• West Pomeranian University of Technology, Institute of Chemical and Environment Engineering, ul. Pułaskiego 10, 70-322 Szczecin, Poland

autor

Wrobel R. J.

• West Pomeranian University of Technology, Institute of Chemical and Environment Engineering, ul. Pułaskiego 10, 70-322 Szczecin, Poland

autor

Grzechulska J.

• West Pomeranian University of Technology, Institute of Chemical and Environment Engineering, ul. Pułaskiego 10, 70-322 Szczecin, Poland

autor

Przepiorski J

• West Pomeranian University of Technology, Institute of Chemical and Environment Engineering, ul. Pułaskiego 10, 70-322 Szczecin, Poland

Bibliografia

• [1] MACWAN D.P., DAVE P.N., CHATURVEDI S., J. Mater. Sci., 46 (2011), 3669 – 3686.
• [2] WANG X., SHUI M., LI R., SONG Y., Mater. Res. Bull., 43 (2008), 2476 – 2484.
• [3] KATOCH A., KIM H., HWANG T., KIM S.S., J. Sol-Gel Sci. Techn., 61 (2012), 77 – 82.
• [4] DIEBOLD U., Surf. Sci. Rep., 48 (2003), 53 – 229.
• [5] HANAOR D.A.H., SORRELL C.C., J. Mater. Sci., 46 (2011), 855 – 874.
• [6] PAN X., MA X., Mater. Lett., 58 (2004), 513 – 515.
• [7] GAO B., YAP P.S., LIM T.M., LIM T.-T., Chem. Eng. J., 171 (2011), 1098 – 1107.
• [8] ZHEREBTSOV A.D., SYUTKIN S.A., PERVUSHIN V.Y., KUZNETSOV G.F., KLESHCHEV D.G., GERMAN V.A., VIKTOROV V.V., KOLMOGORTSEV A.M., SERIKOV A.S., Russ. J. Inorg. Chem.+, 55 (2010), 1197 – 1201.
• [9] CARP O., HUISMAN C.L., RELLER A., Prog. Solid State Ch., 32 (2004), 33 – 177.
• [10] DANESHVAR N., RASOULIFARD M.H., KHATAEE A.R., HOSSEINZADEH F., J. Hazard. Mater., 143 (2007), 95 – 101.
• [11] FUJISHIMA A., RAO T.N., TRYK D.A., J. Photoch. Photobio. C, 1 (2000), 1 – 21.
• [12] MAHMOODI N.M., ARAMI M., LIMAEE N.Y., GHARANJIG K., NOURMOHAMMADIAN F., Mater. Res. Bull., 42 (2007), 797 – 806.
• [13] YANG S., TANG W., ISHIKAWA Y., FENG Q., Mater. Res. Bull., 46 (2011), 531 – 537.
• [14] MAHSHID S., ASKARI M., GHAMSARI S.M., J. Mater. Process. Tech., 189 (2007), 296 – 300.
• [15] GABLENZ S., V¨OLTZKE D., ABICHT H.-P., NEUMANN-ZDRALEK J., J. Mater. Sci. Lett., 17 (1998), 537 – 539.
• [16] KHALIL K.M.S., ZAKI M.I., Powder Technol., 92 (1997), 233 – 239.
• [17] SU C., HONG B.-Y., TSENG C.-M., Catal. Today, 96 (2004), 119 – 126.
• [18] BISCHOFF B.L., ANDERSON M.A., Chem. Mater., 7 (1995), 1772 – 1778.
• [19] DUNUWILA D.D., GAGLIARDI C.D., BERGLUND K.A., Chem. Mater., 6 (1994), 1556 – 1562.
• [20] KHALIL K.M.S., BAIRD T., ZAKI M.I., EL-SAMAHY A.A., AWAD A.M., Colloid Surface A, 13 (1998), 231 –232.
• [21] KIM J.Y., JUNG H.S., NO J.H., KIM J.-R., HONG K.S., J. Electroceram., 16 (2006), 447 – 451.
• [22] KUBELKA P., J. Opt. Soc. Am., 38 (1948), 448 – 456.
• [23] LV K., YU J., DENG K., LI X., LI M., J. Phys. Chem. Solids, 71 (2010), 519 – 522.
• [24] KARAMI A., J. Iran. Chem. Soc., 7 (2010), 154 – 160.
• [25] MAHSHID S., ASKARI M., GHAMSARI S.M., AFSHAR N., LAHUTI S., J. Alloy. Compd., 478 (2009), 586 – 587.
• [26] AGAFONOV A.V., VINOGRADOV A.V., J. Sol-Gel Sci. Techn., 49 (2009), 180 – 185.
• [27] HORVAT B., REˇCNIK A., DRAˇZI´C G., J. Cryst. Growth, 347 (2012), 19 – 24.
• [28] HAFIZAH N., SOPYAN I., Int. J. Photoenergy, (2009) article ID 962783, DOI: 10.1155/2009/962783.
• [29] QOURZAL S., ASSABBANE A., AIT-ICHOU Y., J. Photoch. Photobio. A, 163 (2004), 317 – 321.
• [30] SHOKOOHI R., VATANPOOR V., ZARRABI M., VATANI A., E-J. Chem., 7 (2010), 65 – 72.
• [31] BUBACZ K., CHOINA J., DOLAT D., MORAWSKI A.W., Pol. J. Environ. Stud., 19 (2010), 685 – 691.
• [32] SURESH S., SUGUMAR R.W., MAIYALAGAN T., Asian J. Chem., 23 (2011), 219 – 224.
• [33] GRZECHULSKA-DAMSZEL J., TOMASZEWSKA M., MORAWSKI A.W., Desalination, 241 (2009), 118 – 126.
• [34] WANG J.F., ZHAO J.H., LIU X.X., ZHANG S.H., WEI D.Y., HAN L., Appl. Mech. Mater., 189 (2012), 52 – 57.
• [35] MOZIA S., TOMASZEWSKA M., MORAWSKI A.W., Dyes Pigments, 75 (2007), 60 – 66.
• [36] MALEKI A., ZANDSALIMI Y., SHAHMORADI B., REZAIE R., PORDEL M.A., Sci. J. Kurdistan Univ. Med. Sci., 16 (2011), 101 – 108.
• [37] TRYBA B., J. Adv. Oxid. Technol., 10 (2007), 267 – 272.
• [38] SOUTSAS K., KARAYANNIS V., POULIOS I., RIGA A., NTAMPEGLIOTIS K., SPILIOTIS X., PAPAPOLYMEROU G., Desalination, 250 (2010), 345 – 350.
• [39] PATTERSON A.L., Phys. Rev., 56 (1939), 978 – 982.
• [40] INAGAKI M., NONAKA R., TRYBA B., MORAWSKI A.W., Chemosphere, 64 (2006), 437 – 445.
• [41] GREGG S.J., Stud. Surf. Sci. Catal., 10 (1982), 153 –164.
• [42] HU Y., TSAI H.-L., HUANG C.-L., J. Eur. Ceram. Soc., 23 (2003), 691 – 696.
• [43] ZHANG L., MENENDEZ-FLORES V.-M., MURAKAMI N., OHNO T., Appl. Surf. Sci., 258 (2012), 5803 – 5809.
• [44] KAPINUS E.I., KHALYAVKA T.A., SHIMANOVSKAYA V.V., VIKTOROVA T.I., STRELKO V.V., Int. J. Photoenergy, 5 (2003), 159 – 166.