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The accumulation of organic pollutants in Indonesian waters is challenging for water treatment, because high pollutant levels increase the burden on the water technology used. Membrane technology can be used to optimize the filtration of organic pollutants. However, this technique is still limited by the fouling phenomenon on the membrane surface. The aim of this study was to investigate the effect of humidity on the structure formation and antifouling properties of the fabricated polyethersulfone (PES)-polyethylene glycol hexadecyl ether (PEG-HE) membranes. The PES membrane was modified by adding the additive PEG-HE and printed using the vapor and non-solvent induced phase separation (VNIPS) technique with air humidity of 70% and 90%. Changes in membrane properties and performance were analyzed before and after modification. Overall, the results show that adding 3% PEG-HE additive and using the VNIPS technique have a favorable impact on the membrane, namely, increasing the hydrophilicity, as well as the number and size of pores. The PES membrane modified with PEGHE additives and 90% air humidity exhibited the highest stability in various aspects of analysis, such as a water contact angle of 55.11°, a pure water flux of 69.86 L/m2.h, a flux recovery ratio (FRR) of 91.91%, and humus acid rejection of 86.84%. In conclusion, the present research provides valuable insights into developing PES membranes with antifouling properties for filtering organic pollutants.
Słowa kluczowe
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28--36
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Bibliogr. 25 poz., rys., tab.
Twórcy
autor
- Department of Chemical Engineering, Universitas Syiah Kuala, Syekh Abdurauf As Sinkili 23111, Banda Aceh, Indonesia
autor
- Department of Chemical Engineering, Universitas Syiah Kuala, Syekh Abdurauf As Sinkili 23111, Banda Aceh, Indonesia
autor
- Department of Chemical Engineering, Universitas Syiah Kuala, Syekh Abdurauf As Sinkili 23111, Banda Aceh, Indonesia
autor
- Department of Chemical Engineering, Universitas Syiah Kuala, Syekh Abdurauf As Sinkili 23111, Banda Aceh, Indonesia
autor
- Department of Chemical Engineering, Universitas Syiah Kuala, Syekh Abdurauf As Sinkili 23111, Banda Aceh, Indonesia
autor
- Department of Chemical Engineering, Universitas Syiah Kuala, Syekh Abdurauf As Sinkili 23111, Banda Aceh, Indonesia
autor
- Department of Chemical Engineering, Universitas Syiah Kuala, Syekh Abdurauf As Sinkili 23111, Banda Aceh, Indonesia
autor
- Department of Chemical Engineering, Universitas Syiah Kuala, Syekh Abdurauf As Sinkili 23111, Banda Aceh, Indonesia
- Research Centre for Environmental and Natural Resources, Universitas Syiah Kuala, Jl. Hamzah Fansuri, No. 4, Darussalam, Banda Aceh 23111, Indonesia
- Atsiri Reserach Center-Pusat Unggulan Iptek (PUI), Universitas Syiah Kuala, Jl. Syeh A Rauf, No. 5, Banda Aceh 23111, Indonesia
Bibliografia
- 1. Alharbi, O.M.L., Basheer, A.A., Khattab, R.A., Ali, I., 2018. Health and environmental effects of persistent organic pollutants. Journal of Molecular Liquids 263, 442–453. https://doi.org/10.1016/j.molliq.2018.05.029.
- 2. Ambarita, A.C., Arahman, N., Mulyati, S., 2024. A synergistic approach to improving antifouling and antibacterial properties of Ag/DBR/PES membrane. South African Journal of Chemical Engineering 48, 30–39. https://doi.org/10.1016/j.sajce.2024.01.002.
- 3. Ambarita, A.C., Mulyati, S., Arahman, N., Rosnelly, Suhendrayatna, C.M., 2021. Modification of polyetersulfone (PES) membrane by using jernang (daemonorops draco blume) as a natural additive on humic acid fouling. IOP Conf. Ser.: Mater. Sci. Eng. 1087, 012056. https://doi. org/10.1088/1757-899X/1087/1/012056.
- 4. Amin, N.A.A.M., Mokhter, M.A., Salamun, N., Mohamad, M.F.B., Mahmood, W.M.A.W., 2023. Anti-fouling electrospun organic and inorganic nanofiber membranes for wastewater treatment. South African Journal of Chemical Engineering 44, 302–317. https://doi.org/10.1016/j.sajce.2023.02.002.
- 5. Anderson, L.E., DeMont, I., Dunnington, D.D., Bjorndahl, P., Redden, D.J., Brophy, M.J., Gagnon, G.A., 2023. A review of long-term change in surface water natural organic matter concentration in the northern hemisphere and the implications for drinking water treatment. Science of The Total Environment 858, 159699. https://doi.org/10.1016/j.scitotenv.2022.159699.
- 6. Arahman, N., Satria, S., Razi, F., Bilad, M.R., 2018. The effect of Ca and Mg ions on the filtration profile of sodium alginate solution in a polyethersulfone-2-(methacryloyloxy) ethylphosphorylchloline membrane. Water 10, 1207. https://doi.org/10.3390/w10091207.
- 7. Barambu, N.U., Bilad, M.R., Bustam, M.A., Huda, N., Jaafar, J., Narkkun, T., Faungnawakij, K., 2020. Development of polysulfone membrane via vapor-induced phase separation for oil/water emulsion filtration. Polymers 12, 2519. https://doi.org/10.3390/polym12112519.
- 8. Dias, T.F., Ghisi, E., 2024. Urban water consumption: A systematic literature review. Water 16, 838. https://doi.org/10.3390/w16060838.
- 9. Elhamarnah, Y., Alkhouzaam, A., Qiblawey, H., Nasser, M., 2024. Enhancing the properties and performance of polysulfone ultrafiltration membranes using citric acid based deep eutectic solvent additives. Journal of Environmental Chemical Engineering 12, 112110. https://doi.org/10.1016/j.jece.2024.112110.
- 10. El-Sawaf, A.K., Hemdan, M., Selim, H., Nassar, A.A., Mubarak, M.F., 2024. Revolutionizing water treatment: Enhanced flux and selectivity in polyethersulfone mixed matrix membrane through magnetic CuO-functionalized Fe3 O 4 nanoparticles for synthetic oily produced water remediation. Surfaces and Interfaces 46, 104142. https://doi.org/10.1016/j.surfin.2024.104142.
- 11. Fathanah, U., Muchtar, S., Aprilia, S., Lubis, M.R., Mulyati, S., Yusuf, M., 2024. Unlocking synergies of Mg(OH)2 and rice husk silica as dual additives for tailored pore properties, selectivity, and antifouling performances of PES membrane. South African Journal of Chemical Engineering 48, 22–29. https://doi.org/10.1016/j.sajce.2024.01.004.
- 12. Gul, A., Hruza, J., Yalcinkaya, F., 2021. Fouling and chemical cleaning of microfiltration membranes: A mini-review. Polymers 13, 846. https://doi.org/10.3390/polym13060846.
- 13. Haikal, R.D., Marom, A.Z., Aulia, M.P., Ambarita, A.C., Azwar, A., Fahrina, A., Bilad, M.R., Mulyati, S., Pasaoglu, M.E., Koyuncu, I., Arahman, N., 2023. Morphology and characteristics of polyethersulfone membrane modified with polyethylene glycol hexadecyl ether and nanocarbon. Appl. Chem. Eng. 7. https://doi.org/10.24294/ace.v7i1.2291.
- 14. Iyare, P.U., Ouki, S.K., Bond, T., 2020. Microplastics removal in wastewater treatment plants: a critical review. Environ. Sci.: Water Res. Technol. 6, 2664–2675. https://doi.org/10.1039/D0EW00397B.
- 15. Jarukas, L., Ivanauskas, L., Kasparaviciene, G., Baranauskaite, J., Marksa, M., Bernatoniene, J., 2021. Determination of organic compounds, fulvic acid, humic acid, and humin in peat and sapropel alkaline extracts. Molecules 26, 2995. https://doi.org/10.3390/molecules26102995.
- 16. Kallem, P., Othman, I., Ouda, M., Hasan, S.W., Al-Nashef, I., Banat, F., 2021. Polyethersulfone hybrid ultrafiltration membranes fabricated with polydopamine modified ZnFe2O 4 nanocomposites: Applications in humic acid removal and oil/water emulsion separation. Process Safety and Environmental Protection 148, 813–824. https://doi.org/10.1016/j.psep.2021.02.002.
- 17. Mat Nawi, N.I., Chean, H.M., Shamsuddin, N., Bilad, M.R., Narkkun, T., Faungnawakij, K., Khan, A.L., 2020. Development of hydrophilic PVDF membrane using vapour induced phase separation method for produced water treatment. Membranes 10, 121. https://doi.org/10.3390/membranes10060121.
- 18. Mukramah, S., Mulyati, S., Arahman, N., 2017. Influence of Brij58 on the characteristic and performance of PES membrane for water treatment process. IOP Conf. Ser.: Mater. Sci. Eng. 180, 012130. https://doi.org/10.1088/1757-899X/180/1/012130.
- 19. Mulyati, S., Riza, M., Muchtar, S., Ambarita, A.C., Amilia, Putri, E.F.A., Luthfiana, A., 2024. A high performance of polyvinylidene fluoride membrane modified with vanilin for humic acid removal. Case Studies in Chemical and Environmental Engineering 9, 100654. https://doi.org/10.1016/j.cscee.2024.100654.
- 20. Ngang, H.P., Ahmad, A.L., Low, S.C., Ooi, B.S.,2014. The influence of PEG additive on the morphology of PVDF ultrafiltration membranes and its antifouling properties towards proteins separation. Jurnal Teknologi 70. https://doi.org/10.11113/jt.v70.3430.
- 21. Rahman, N.A., Sotani, T., Matsuyama, H., 2008. Effect of the addition of the surfactant Tetronic 1307 on poly(ether sulfone) porous hollow‐fiber membrane formation. J of Applied Polymer Sci 108, 3411–3418. https://doi.org/10.1002/app.27940.
- 22. Raja, R.I., Rashid, K.T., Toma, M.A., AbdulRazak, A.A., Ahmed Shehab, M., Hernadi, K., 2024. A novel Polyethersulfone/Chamomile (PES/Chm) mixed matrix membranes for wastewater treatment applications. Journal of Saudi Chemical Society 28, 101805. https://doi.org/10.1016/j.jscs.2023.101805.
- 23. Ren, X., Ji, D., Wen, X., Bustamante, H., Daiyan, R., Foller, T., Khine, Y.Y., Joshi, R., 2022. Graphene oxide membranes for effective removal of humic acid. Journal of Materials Research 37, 3362–3371. https://doi.org/10.1557/s43578-022-00647-6.
- 24. Suryani, A.S., 2020. Development of clean water and sanitation during the Covid-19 pandemic. aspirations 11, 199–214. (in Indonesia) https://doi.org/10.46807/aspiration.v11i2.1757.
- 25. Yu, Y., Yang, Y., Yu, L., Koh, K.Y., Chen, J.P., 2021. Modification of polyvinylidene fluoride membrane by silver nanoparticles-graphene oxide hybrid nanosheet for effective membrane biofouling mitigation. Chemosphere 268, 129187. https://doi.org/10.1016/j.chemosphere.2020.129187.
Typ dokumentu
Bibliografia
Identyfikator YADDA
bwmeta1.element.baztech-3d065084-a299-4ee6-9440-5f772c1c4c7d
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